From Molecules to Frameworks to Superframework Crystals
Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy is proposed by which progressive levels of complexity are achieved through the building block approach whereby molecularly defined constructs...
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Published in | Advanced materials (Weinheim) Vol. 33; no. 42; pp. e2103808 - n/a |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
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Wiley Subscription Services, Inc
01.10.2021
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Abstract | Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy is proposed by which progressive levels of complexity are achieved through the building block approach whereby molecularly defined constructs at one level serve as constituent units of the next level, all being linked through strong bonds—”augmented reticular chemistry”. Specifically, current knowledge of linking metal complexes and organic molecules into reticular frameworks is applied here to linking the crystals of these frameworks into supercrystals (superframeworks). This strategy allows for the molecular control exercised on the molecular regime to be translated into higher augmentation levels to produce systems capable of dynamics and complex functionality far exceeding current materials.
A synthetic approach is presented to build macroscopic structures with the same precision applied in molecular chemistry. Molecules are linked into frameworks, and crystals of frameworks are in turn linked into superframeworks, an escalation of building blocks from molecules to crystals. This strategy is termed augmented reticular chemistry, from where new frontiers of photonics, dynamics, and systems chemistry emerge. |
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AbstractList | Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy is proposed by which progressive levels of complexity are achieved through the building block approach whereby molecularly defined constructs at one level serve as constituent units of the next level, all being linked through strong bonds—”augmented reticular chemistry”. Specifically, current knowledge of linking metal complexes and organic molecules into reticular frameworks is applied here to linking the crystals of these frameworks into supercrystals (superframeworks). This strategy allows for the molecular control exercised on the molecular regime to be translated into higher augmentation levels to produce systems capable of dynamics and complex functionality far exceeding current materials.
A synthetic approach is presented to build macroscopic structures with the same precision applied in molecular chemistry. Molecules are linked into frameworks, and crystals of frameworks are in turn linked into superframeworks, an escalation of building blocks from molecules to crystals. This strategy is termed augmented reticular chemistry, from where new frontiers of photonics, dynamics, and systems chemistry emerge. Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy is proposed by which progressive levels of complexity are achieved through the building block approach whereby molecularly defined constructs at one level serve as constituent units of the next level, all being linked through strong bonds-"augmented reticular chemistry". Specifically, current knowledge of linking metal complexes and organic molecules into reticular frameworks is applied here to linking the crystals of these frameworks into supercrystals (superframeworks). This strategy allows for the molecular control exercised on the molecular regime to be translated into higher augmentation levels to produce systems capable of dynamics and complex functionality far exceeding current materials. Abstract Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy is proposed by which progressive levels of complexity are achieved through the building block approach whereby molecularly defined constructs at one level serve as constituent units of the next level, all being linked through strong bonds—”augmented reticular chemistry”. Specifically, current knowledge of linking metal complexes and organic molecules into reticular frameworks is applied here to linking the crystals of these frameworks into supercrystals (superframeworks). This strategy allows for the molecular control exercised on the molecular regime to be translated into higher augmentation levels to produce systems capable of dynamics and complex functionality far exceeding current materials. |
Author | Diercks, Christian S. Hirschle, Patrick Ji, Zhe Freund, Ralph Wuttke, Stefan Yaghi, Omar M. |
Author_xml | – sequence: 1 givenname: Zhe orcidid: 0000-0002-8532-333X surname: Ji fullname: Ji, Zhe organization: University of California–Berkeley – sequence: 2 givenname: Ralph orcidid: 0000-0001-5156-6934 surname: Freund fullname: Freund, Ralph organization: Ludwig‐Maximilians‐Universität München – sequence: 3 givenname: Christian S. orcidid: 0000-0002-7813-0302 surname: Diercks fullname: Diercks, Christian S. organization: University of California–Berkeley – sequence: 4 givenname: Patrick surname: Hirschle fullname: Hirschle, Patrick organization: Ludwig‐Maximilians‐Universität München – sequence: 5 givenname: Omar M. orcidid: 0000-0002-5611-3325 surname: Yaghi fullname: Yaghi, Omar M. email: yaghi@berkeley.edu organization: UAE University – sequence: 6 givenname: Stefan orcidid: 0000-0002-6344-5782 surname: Wuttke fullname: Wuttke, Stefan email: stefan.wuttke@bcmaterials.net organization: Basque Foundation for Science |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34499785$$D View this record in MEDLINE/PubMed |
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Snippet | Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic strategy... Abstract Building chemical structures of complexity and functionality approaching the level of biological systems is an ongoing challenge. A general synthetic... |
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SubjectTerms | augmented reticular chemistry Bonding strength Carbon Dioxide - chemistry Chemical bonds Complexity Coordination Complexes - chemistry Coordination compounds Crystal structure Electrons Light Materials science Metal-Organic Frameworks - chemistry metal–organic frameworks Organic chemistry Oxidation-Reduction Porosity supercrystals superframeworks Surface Properties |
Title | From Molecules to Frameworks to Superframework Crystals |
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