MOF‐Derived Ni/ZIF‐8/ZnO Arrays on Carbon Fiber Cloth for Efficient Adsorption‐Catalytic Oxidation
The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon fiber cloth (CFC) serves as the zinc source to ensure that the Ni/ZIF‐8/ZnO nanoreactor is constructed. The Ni/ZIF‐8/ZnO/CFC nanoreactor effici...
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Published in | Small (Weinheim an der Bergstrasse, Germany) Vol. 19; no. 50; pp. e2303928 - n/a |
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Abstract | The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon fiber cloth (CFC) serves as the zinc source to ensure that the Ni/ZIF‐8/ZnO nanoreactor is constructed. The Ni/ZIF‐8/ZnO/CFC nanoreactor efficiently activates peroxymonosulfate (PMS) for bisphenol A (BPA) degradation owing to its high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. Experimental and theoretical calculations clearly show that the introduction of Ni is beneficial for improving the adsorption of BPA and the activation of PMS. The synergistic mechanism of BPA adsorption–PMS activation is also investigated, and the degradation pathway of BPA is examined. Moreover, a filter catalytic unit is constructed using Ni/ZIF‐8/ZnO/CFC to achieve a continuous zero discharge of BPA, which is convenient for nanocatalyst recycling. This study aims to develop a new strategy for the removal of emerging organic pollutants from water using a system with strong adsorption and catalytic capabilities.
The novel Ni/ZIF‐8/ZnO nanoreactor array is grown on carbon fiber cloth (CFC). The efficient activated peroxymonosulfate (PMS) performance of Ni/ZIF‐8/ZnO/CFC results from the high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. |
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AbstractList | Abstract
The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon fiber cloth (CFC) serves as the zinc source to ensure that the Ni/ZIF‐8/ZnO nanoreactor is constructed. The Ni/ZIF‐8/ZnO/CFC nanoreactor efficiently activates peroxymonosulfate (PMS) for bisphenol A (BPA) degradation owing to its high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. Experimental and theoretical calculations clearly show that the introduction of Ni is beneficial for improving the adsorption of BPA and the activation of PMS. The synergistic mechanism of BPA adsorption–PMS activation is also investigated, and the degradation pathway of BPA is examined. Moreover, a filter catalytic unit is constructed using Ni/ZIF‐8/ZnO/CFC to achieve a continuous zero discharge of BPA, which is convenient for nanocatalyst recycling. This study aims to develop a new strategy for the removal of emerging organic pollutants from water using a system with strong adsorption and catalytic capabilities. The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon fiber cloth (CFC) serves as the zinc source to ensure that the Ni/ZIF‐8/ZnO nanoreactor is constructed. The Ni/ZIF‐8/ZnO/CFC nanoreactor efficiently activates peroxymonosulfate (PMS) for bisphenol A (BPA) degradation owing to its high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. Experimental and theoretical calculations clearly show that the introduction of Ni is beneficial for improving the adsorption of BPA and the activation of PMS. The synergistic mechanism of BPA adsorption–PMS activation is also investigated, and the degradation pathway of BPA is examined. Moreover, a filter catalytic unit is constructed using Ni/ZIF‐8/ZnO/CFC to achieve a continuous zero discharge of BPA, which is convenient for nanocatalyst recycling. This study aims to develop a new strategy for the removal of emerging organic pollutants from water using a system with strong adsorption and catalytic capabilities. The novel Ni/ZIF‐8/ZnO nanoreactor array is grown on carbon fiber cloth (CFC). The efficient activated peroxymonosulfate (PMS) performance of Ni/ZIF‐8/ZnO/CFC results from the high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon fiber cloth (CFC) serves as the zinc source to ensure that the Ni/ZIF‐8/ZnO nanoreactor is constructed. The Ni/ZIF‐8/ZnO/CFC nanoreactor efficiently activates peroxymonosulfate (PMS) for bisphenol A (BPA) degradation owing to its high density of active sites, high adsorbability, and dispersibility structure, which concentrates catalytic and adsorptive sites within a confined space. Experimental and theoretical calculations clearly show that the introduction of Ni is beneficial for improving the adsorption of BPA and the activation of PMS. The synergistic mechanism of BPA adsorption–PMS activation is also investigated, and the degradation pathway of BPA is examined. Moreover, a filter catalytic unit is constructed using Ni/ZIF‐8/ZnO/CFC to achieve a continuous zero discharge of BPA, which is convenient for nanocatalyst recycling. This study aims to develop a new strategy for the removal of emerging organic pollutants from water using a system with strong adsorption and catalytic capabilities. |
Author | Yang, Zhen Wang, Ruoding Wang, Yue Liu, Zifan Ge, Yu Yang, Weiben Yin, Zhonglong Liu, Fuqiang |
Author_xml | – sequence: 1 givenname: Yue surname: Wang fullname: Wang, Yue organization: Nanjing Normal University – sequence: 2 givenname: Yu surname: Ge fullname: Ge, Yu organization: Nanjing Normal University – sequence: 3 givenname: Ruoding surname: Wang fullname: Wang, Ruoding organization: Nanjing Normal University – sequence: 4 givenname: Zifan surname: Liu fullname: Liu, Zifan organization: Nanjing Normal University – sequence: 5 givenname: Zhonglong surname: Yin fullname: Yin, Zhonglong organization: Nanjing Normal University – sequence: 6 givenname: Zhen surname: Yang fullname: Yang, Zhen organization: Nanjing Normal University – sequence: 7 givenname: Fuqiang surname: Liu fullname: Liu, Fuqiang organization: Nanjing University – sequence: 8 givenname: Weiben orcidid: 0000-0002-8521-255X surname: Yang fullname: Yang, Weiben email: yangwb007@njnu.edu.cn organization: Nanjing Normal University |
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Snippet | The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a carbon... Abstract The catalytic oxidation of toxic organic pollutants in water requires enhanced efficiency for commercial applications. A ZnO nanorod array grown on a... |
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SubjectTerms | Adsorption Adsorptivity Arrays Bisphenol A Carbon fibers Catalytic oxidation Cloth Confined spaces Degradation nanoreactors Nanorods Nanotechnology organic pollutants Oxidation peroxymonosulfate Pollutants Zinc oxide |
Title | MOF‐Derived Ni/ZIF‐8/ZnO Arrays on Carbon Fiber Cloth for Efficient Adsorption‐Catalytic Oxidation |
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