High Water Adsorption MOFs with Optimized Pore‐Nanospaces for Autonomous Indoor Humidity Control and Pollutants Removal

The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore‐nanospace post‐engineering strategy to optimize the hydrophilicity, wate...

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Published inAngewandte Chemie International Edition Vol. 61; no. 4; pp. e202112097 - n/a
Main Authors Zhu, Neng‐Xiu, Wei, Zhang‐Wen, Chen, Cheng‐Xia, Xiong, Xiao‐Hong, Xiong, Yang‐Yang, Zeng, Zheng, Wang, Wei, Jiang, Ji‐Jun, Fan, Ya‐Nan, Su, Cheng‐Yong
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 21.01.2022
EditionInternational ed. in English
Subjects
Adsorbed water
Adsorption
Air Pollution, Indoor
Air quality
Contaminants
Control stability
Dehumidification
Gels
Health risks
high water-stable MOFs
Humidity
Humidity control
Hydrophilicity
Hydrophobicity
Indoor air pollution
indoor air purification
Indoor air quality
Indoor environments
indoor humidity control
Metal-organic frameworks
Metal-Organic Frameworks - chemistry
MOF pore-nanospace engineering
Moisture control
Molecular Structure
Nanoparticles - chemistry
Optimization
Particle Size
Pollutant removal
Pollutants
Pollution control
Recyclability
Regeneration
Relative humidity
Silica
Silicon dioxide
Surface Properties
Water - chemistry
Water Pollutants, Chemical - chemistry
Water Pollutants, Chemical - isolation & purification
Water purification
water-adsorption based applications
Work capacity
Zeolites
indoor air purification
MOF pore-nanospace engineering
high water-stable MOFs
indoor humidity control
water-adsorption based applications
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Abstract The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore‐nanospace post‐engineering strategy to optimize the hydrophilicity, water‐uptake capacity and air‐purifying ability of metal‐organic frameworks (MOFs) with long‐term stability, offering an ideal candidate with autonomous multi‐functionality of moisture control and pollutants sequestration. Through variant tuning of organic‐linkers carrying hydrophobic and hydrophilic groups in the pore‐nanospaces of prototypical UiO‐67, a moderately hydrophilic MOF (UiO‐67‐4Me‐NH2‐38 %) with high thermal, hydrolytic and acid‐base stability is screened out, featuring S‐shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %–65 % RH) and adverse health effects minimization (40–60 % RH). Its exceptional attributes of water‐uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application. A moderately hydrophilic MOF of UiO‐67‐4Me‐NH2‐38 % with high thermal, hydrolytic and acid‐base stability has been obtained by a pore‐nanospace post‐engineering strategy, which shows ideal S‐shaped water‐sorption isotherm, high water‐uptake working capacity and efficiency in the ASHRAE recommended humidity range, and prior capture ability of harmful organic and inorganic vapors, providing a promising candidate for autonomous indoor humidity control and air purification.
AbstractList The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica-gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore-nanospace post-engineering strategy to optimize the hydrophilicity, water-uptake capacity and air-purifying ability of metal-organic frameworks (MOFs) with long-term stability, offering an ideal candidate with autonomous multi-functionality of moisture control and pollutants sequestration. Through variant tuning of organic-linkers carrying hydrophobic and hydrophilic groups in the pore-nanospaces of prototypical UiO-67, a moderately hydrophilic MOF (UiO-67-4Me-NH -38 %) with high thermal, hydrolytic and acid-base stability is screened out, featuring S-shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %-65 % RH) and adverse health effects minimization (40-60 % RH). Its exceptional attributes of water-uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application.
The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica-gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore-nanospace post-engineering strategy to optimize the hydrophilicity, water-uptake capacity and air-purifying ability of metal-organic frameworks (MOFs) with long-term stability, offering an ideal candidate with autonomous multi-functionality of moisture control and pollutants sequestration. Through variant tuning of organic-linkers carrying hydrophobic and hydrophilic groups in the pore-nanospaces of prototypical UiO-67, a moderately hydrophilic MOF (UiO-67-4Me-NH2 -38 %) with high thermal, hydrolytic and acid-base stability is screened out, featuring S-shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %-65 % RH) and adverse health effects minimization (40-60 % RH). Its exceptional attributes of water-uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application.The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica-gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore-nanospace post-engineering strategy to optimize the hydrophilicity, water-uptake capacity and air-purifying ability of metal-organic frameworks (MOFs) with long-term stability, offering an ideal candidate with autonomous multi-functionality of moisture control and pollutants sequestration. Through variant tuning of organic-linkers carrying hydrophobic and hydrophilic groups in the pore-nanospaces of prototypical UiO-67, a moderately hydrophilic MOF (UiO-67-4Me-NH2 -38 %) with high thermal, hydrolytic and acid-base stability is screened out, featuring S-shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %-65 % RH) and adverse health effects minimization (40-60 % RH). Its exceptional attributes of water-uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application.
The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore‐nanospace post‐engineering strategy to optimize the hydrophilicity, water‐uptake capacity and air‐purifying ability of metal‐organic frameworks (MOFs) with long‐term stability, offering an ideal candidate with autonomous multi‐functionality of moisture control and pollutants sequestration. Through variant tuning of organic‐linkers carrying hydrophobic and hydrophilic groups in the pore‐nanospaces of prototypical UiO‐67, a moderately hydrophilic MOF (UiO‐67‐4Me‐NH2‐38 %) with high thermal, hydrolytic and acid‐base stability is screened out, featuring S‐shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %–65 % RH) and adverse health effects minimization (40–60 % RH). Its exceptional attributes of water‐uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application.
The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore‐nanospace post‐engineering strategy to optimize the hydrophilicity, water‐uptake capacity and air‐purifying ability of metal‐organic frameworks (MOFs) with long‐term stability, offering an ideal candidate with autonomous multi‐functionality of moisture control and pollutants sequestration. Through variant tuning of organic‐linkers carrying hydrophobic and hydrophilic groups in the pore‐nanospaces of prototypical UiO‐67, a moderately hydrophilic MOF (UiO‐67‐4Me‐NH2‐38 %) with high thermal, hydrolytic and acid‐base stability is screened out, featuring S‐shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %–65 % RH) and adverse health effects minimization (40–60 % RH). Its exceptional attributes of water‐uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application. A moderately hydrophilic MOF of UiO‐67‐4Me‐NH2‐38 % with high thermal, hydrolytic and acid‐base stability has been obtained by a pore‐nanospace post‐engineering strategy, which shows ideal S‐shaped water‐sorption isotherm, high water‐uptake working capacity and efficiency in the ASHRAE recommended humidity range, and prior capture ability of harmful organic and inorganic vapors, providing a promising candidate for autonomous indoor humidity control and air purification.
The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air dehumidification and harmful gases capture. Herein, we develop a pore‐nanospace post‐engineering strategy to optimize the hydrophilicity, water‐uptake capacity and air‐purifying ability of metal‐organic frameworks (MOFs) with long‐term stability, offering an ideal candidate with autonomous multi‐functionality of moisture control and pollutants sequestration. Through variant tuning of organic‐linkers carrying hydrophobic and hydrophilic groups in the pore‐nanospaces of prototypical UiO‐67, a moderately hydrophilic MOF (UiO‐67‐4Me‐NH 2 ‐38 %) with high thermal, hydrolytic and acid‐base stability is screened out, featuring S‐shaped water sorption isotherms exactly located in the recommended comfortable and healthy ranges of relative humidity for indoor ventilation (45 %–65 % RH) and adverse health effects minimization (40–60 % RH). Its exceptional attributes of water‐uptake working capacity/efficiency, contaminants removal, recyclability and regeneration promise a great potential in confined indoor environment application.
Author Chen, Cheng‐Xia
Fan, Ya‐Nan
Wang, Wei
Wei, Zhang‐Wen
Jiang, Ji‐Jun
Xiong, Xiao‐Hong
Zhu, Neng‐Xiu
Zeng, Zheng
Xiong, Yang‐Yang
Su, Cheng‐Yong
Author_xml – sequence: 1
  givenname: Neng‐Xiu
  surname: Zhu
  fullname: Zhu, Neng‐Xiu
  organization: Sun Yat-Sen University
– sequence: 2
  givenname: Zhang‐Wen
  surname: Wei
  fullname: Wei, Zhang‐Wen
  organization: Sun Yat-Sen University
– sequence: 3
  givenname: Cheng‐Xia
  surname: Chen
  fullname: Chen, Cheng‐Xia
  organization: Sun Yat-Sen University
– sequence: 4
  givenname: Xiao‐Hong
  surname: Xiong
  fullname: Xiong, Xiao‐Hong
  organization: Sun Yat-Sen University
– sequence: 5
  givenname: Yang‐Yang
  surname: Xiong
  fullname: Xiong, Yang‐Yang
  organization: Sun Yat-Sen University
– sequence: 6
  givenname: Zheng
  surname: Zeng
  fullname: Zeng, Zheng
  organization: Sun Yat-Sen University
– sequence: 7
  givenname: Wei
  surname: Wang
  fullname: Wang, Wei
  organization: Sun Yat-Sen University
– sequence: 8
  givenname: Ji‐Jun
  surname: Jiang
  fullname: Jiang, Ji‐Jun
  organization: Sun Yat-Sen University
– sequence: 9
  givenname: Ya‐Nan
  surname: Fan
  fullname: Fan, Ya‐Nan
  organization: Sun Yat-Sen University
– sequence: 10
  givenname: Cheng‐Yong
  orcidid: 0000-0003-3604-7858
  surname: Su
  fullname: Su, Cheng‐Yong
  email: cesscy@mail.sysu.edu.cn
  organization: Lanzhou University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/34779556$$D View this record in MEDLINE/PubMed
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Keywords indoor air purification
MOF pore-nanospace engineering
high water-stable MOFs
indoor humidity control
water-adsorption based applications
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2019; 10
2017; 46
2020 2020; 59 132
2019; 19
2008; 105
2020; 12
2017; 356
2018; 47
2017; 406
2020; 7
2020; 6
2018; 3
2021; 31
2012; 210
2018; 4
2021; 233
2018; 339
2018; 30
2016; 45
2017; 404
2019; 7
2018; 185
2018; 140
2015; 3
2019; 31
2021; 105
2011; 40
2020; 423
2013; 341
2009; 131
2021; 143
2019; 141
2014; 114
2019 2019; 58 131
2011; 133
2017; 139
2014; 43
2016 2016; 55 128
2021; 12
2012; 112
1986; 65
2004; 14
2019; 48
2017; 56
2020; 26
2018
2016; 138
2020; 235
2008; 130
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SSID ssj0028806
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Snippet The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica‐gels are widely used for air...
The indoor air quality is of prime importance for human daily life and health, for which the adsorbents like zeolites and silica-gels are widely used for air...
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Index Database
Enrichment Source
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StartPage e202112097
SubjectTerms Adsorbed water
Adsorption
Air Pollution, Indoor
Air quality
Contaminants
Control stability
Dehumidification
Gels
Health risks
high water-stable MOFs
Humidity
Humidity control
Hydrophilicity
Hydrophobicity
Indoor air pollution
indoor air purification
Indoor air quality
Indoor environments
indoor humidity control
Metal-organic frameworks
Metal-Organic Frameworks - chemistry
MOF pore-nanospace engineering
Moisture control
Molecular Structure
Nanoparticles - chemistry
Optimization
Particle Size
Pollutant removal
Pollutants
Pollution control
Recyclability
Regeneration
Relative humidity
Silica
Silicon dioxide
Surface Properties
Water - chemistry
Water Pollutants, Chemical - chemistry
Water Pollutants, Chemical - isolation & purification
Water purification
water-adsorption based applications
Work capacity
Zeolites
Title High Water Adsorption MOFs with Optimized Pore‐Nanospaces for Autonomous Indoor Humidity Control and Pollutants Removal
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.202112097
https://www.ncbi.nlm.nih.gov/pubmed/34779556
https://www.proquest.com/docview/2619616278
https://www.proquest.com/docview/2597819606
Volume 61
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