Highly Efficient Flexible Perovskite Solar Cells through Pentylammonium Acetate Modification with Certified Efficiency of 23.35

Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their m...

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Published inAdvanced materials (Weinheim) Vol. 35; no. 3; pp. e2206387 - n/a
Main Authors Gao, Danpeng, Li, Bo, Li, Zhen, Wu, Xin, Zhang, Shoufeng, Zhao, Dan, Jiang, Xiaofen, Zhang, Chunlei, Wang, Yan, Li, Zhenjiang, Li, Nan, Xiao, Shuang, Choy, Wallace C. H., Jen, Alex K.‐Y., Yang, Shangfeng, Zhu, Zonglong
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.01.2023
Subjects
Bends
Circuits
Energy conversion efficiency
flexible solar cells
high efficiency
interface modification
Materials science
mechanical stability
Perovskites
Photovoltaic cells
Solar cells
perovskites
high efficiency
flexible solar cells
interface modification
mechanical stability
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Abstract Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA+ and Ac− have strong chemical binding with both acceptor and donor defects of surface‐terminating ends on perovskite films. The PenAAc‐modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm2, certified: 23.35%) with a high open‐circuit voltage (VOC) of 1.17 V. Large‐area devices (1.0 cm2) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends. Highly efficient and stable flexible inverted perovskite solar cells are developed through modifying the interface between perovskite and hole transport layer via pentylammonium acetate molecule, which achieve a record power conversion efficiency of 23.68% (0.08 cm2, certified: 23.35%) and excellent mechanical stability.
AbstractList Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA and Ac have strong chemical binding with both acceptor and donor defects of surface-terminating ends on perovskite films. The PenAAc-modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm , certified: 23.35%) with a high open-circuit voltage (V ) of 1.17 V. Large-area devices (1.0 cm ) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends.
Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA+ and Ac- have strong chemical binding with both acceptor and donor defects of surface-terminating ends on perovskite films. The PenAAc-modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm2 , certified: 23.35%) with a high open-circuit voltage (VOC ) of 1.17 V. Large-area devices (1.0 cm2 ) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends.Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA+ and Ac- have strong chemical binding with both acceptor and donor defects of surface-terminating ends on perovskite films. The PenAAc-modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm2 , certified: 23.35%) with a high open-circuit voltage (VOC ) of 1.17 V. Large-area devices (1.0 cm2 ) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends.
Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA + and Ac − have strong chemical binding with both acceptor and donor defects of surface‐terminating ends on perovskite films. The PenAAc‐modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm 2 , certified: 23.35%) with a high open‐circuit voltage ( V OC ) of 1.17 V. Large‐area devices (1.0 cm 2 ) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends.
Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA+ and Ac− have strong chemical binding with both acceptor and donor defects of surface‐terminating ends on perovskite films. The PenAAc‐modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm2, certified: 23.35%) with a high open‐circuit voltage (VOC) of 1.17 V. Large‐area devices (1.0 cm2) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends. Highly efficient and stable flexible inverted perovskite solar cells are developed through modifying the interface between perovskite and hole transport layer via pentylammonium acetate molecule, which achieve a record power conversion efficiency of 23.68% (0.08 cm2, certified: 23.35%) and excellent mechanical stability.
Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion efficiency (PCE) of up to 25.7%. However, the record PCE of flexible PSCs (≈22.4%) still lags far behind their rigid counterparts and their mechanical stabilities are also not satisfactory. Herein, through modifying the interface between perovskite and hole transport layer via pentylammonium acetate (PenAAc) molecule a highly efficient and stable flexible inverted PSC is reported. Through synthetic manipulation of anion and cation, it is shown that the PenA+ and Ac− have strong chemical binding with both acceptor and donor defects of surface‐terminating ends on perovskite films. The PenAAc‐modified flexible PSCs achieve a record PCE of 23.68% (0.08 cm2, certified: 23.35%) with a high open‐circuit voltage (VOC) of 1.17 V. Large‐area devices (1.0 cm2) also realized an exceptional PCE of 21.52%. Moreover, the fabricated devices show excellent stability under mechanical bending, with PCE remaining above 91% of the original PCE even after 5000 bends.
Author Li, Zhen
Yang, Shangfeng
Xiao, Shuang
Li, Nan
Zhang, Chunlei
Li, Zhenjiang
Wu, Xin
Zhao, Dan
Gao, Danpeng
Zhang, Shoufeng
Jen, Alex K.‐Y.
Wang, Yan
Li, Bo
Zhu, Zonglong
Choy, Wallace C. H.
Jiang, Xiaofen
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  organization: City University of Hong Kong
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  fullname: Li, Zhen
  organization: City University of Hong Kong
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  organization: City University of Hong Kong
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  organization: City University of Hong Kong
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  fullname: Zhao, Dan
  organization: City University of Hong Kong
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  organization: University of Science and Technology of China
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  surname: Zhang
  fullname: Zhang, Chunlei
  organization: City University of Hong Kong
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  fullname: Wang, Yan
  organization: City University of Hong Kong
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  organization: City University of Hong Kong
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  fullname: Li, Nan
  organization: The Chinese University of Hong Kong
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  fullname: Xiao, Shuang
  organization: Shenzhen Technology University
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  givenname: Wallace C. H.
  surname: Choy
  fullname: Choy, Wallace C. H.
  organization: University of Hong Kong
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  surname: Jen
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  givenname: Zonglong
  orcidid: 0000-0002-8285-9665
  surname: Zhu
  fullname: Zhu, Zonglong
  email: zonglzhu@cityu.edu.hk
  organization: City University of Hong Kong
BackLink https://www.ncbi.nlm.nih.gov/pubmed/36349808$$D View this record in MEDLINE/PubMed
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Snippet Among the emerging photovoltaic technologies, rigid perovskite solar cells (PSCs) have made tremendous development owing to their exceptional power conversion...
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SubjectTerms Bends
Circuits
Energy conversion efficiency
flexible solar cells
high efficiency
interface modification
Materials science
mechanical stability
Perovskites
Photovoltaic cells
Solar cells
Title Highly Efficient Flexible Perovskite Solar Cells through Pentylammonium Acetate Modification with Certified Efficiency of 23.35
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