Pressure‐Tuned Multicolor Emission of 2D Lead Halide Perovskites with Ultrahigh Color Purity
The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide‐range and ultrapure photoluminescence emissions in a family of h...
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| Published in | Angewandte Chemie International Edition Vol. 62; no. 12; pp. e202218675 - n/a |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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13.03.2023
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| Edition | International ed. in English |
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| Abstract | The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide‐range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA]2PbBr4−4xI4x (MeOPEA=4‐methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C−H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide‐range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra‐wide color gamut and high color purity which are highly useful for pressure sensing.
Wide‐range and ultrapure emissions are achieved in 2D lead halide perovskites (LHPs) by combined chemical pressure from halogen doping/substitution and physical pressure from hydrostatic compression. This work demonstrates precise emission tuning and effective color regulation of 2D LHPs by pressure engineering, which would open a new pathway for developing ultrapure emitters and highly sensitive pressure sensors. |
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| AbstractList | The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide‐range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA] 2 PbBr 4−4 x I 4 x (MeOPEA=4‐methoxyphenethylammonium; x =0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C−H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide‐range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra‐wide color gamut and high color purity which are highly useful for pressure sensing. The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide‐range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA]2PbBr4−4xI4x (MeOPEA=4‐methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C−H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide‐range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra‐wide color gamut and high color purity which are highly useful for pressure sensing. The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide-range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA]2 PbBr4-4x I4x (MeOPEA=4-methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C-H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide-range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra-wide color gamut and high color purity which are highly useful for pressure sensing.The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide-range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA]2 PbBr4-4x I4x (MeOPEA=4-methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C-H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide-range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra-wide color gamut and high color purity which are highly useful for pressure sensing. The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide‐range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA]2PbBr4−4xI4x (MeOPEA=4‐methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C−H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide‐range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra‐wide color gamut and high color purity which are highly useful for pressure sensing. Wide‐range and ultrapure emissions are achieved in 2D lead halide perovskites (LHPs) by combined chemical pressure from halogen doping/substitution and physical pressure from hydrostatic compression. This work demonstrates precise emission tuning and effective color regulation of 2D LHPs by pressure engineering, which would open a new pathway for developing ultrapure emitters and highly sensitive pressure sensors. The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through internal molecular engineering and external stimuli. Herein, we report the wide-range and ultrapure photoluminescence emissions in a family of homologous 2D LHPs, [MeOPEA] PbBr I (MeOPEA=4-methoxyphenethylammonium; x=0, 0.2, 0.425, 0.575, 1) enabled through internal chemical pressure and external hydrostatic pressure. The chemical pressure, induced by the C-H⋅⋅⋅π interactions and halogen doping/substitution strengthens the structural rigidity to give sustained narrow emissions, and regulates the emission energy, respectively. Further manipulation of physical pressure leads to wide-range emission tuning from 412 to 647 nm in a continuous and reversible manner. This work could open up new pathways for developing 2D LHP emitters with ultra-wide color gamut and high color purity which are highly useful for pressure sensing. |
| Author | Li, Zhi‐Gang Fan, Jia‐Hui Yao, Zhao‐Quan Qin, Yan Wu, Xiang Li, Wei Bu, Xian‐He Li, Xiang Song, Haipeng Gao, Fei‐Fei |
| Author_xml | – sequence: 1 givenname: Fei‐Fei orcidid: 0000-0002-6900-817X surname: Gao fullname: Gao, Fei‐Fei organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry – sequence: 2 givenname: Haipeng surname: Song fullname: Song, Haipeng organization: China University of Geosciences (Wuhan) – sequence: 3 givenname: Zhi‐Gang surname: Li fullname: Li, Zhi‐Gang organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry – sequence: 4 givenname: Yan orcidid: 0000-0002-6187-601X surname: Qin fullname: Qin, Yan email: qinyan@ncu.edu.cn organization: Nanchang University – sequence: 5 givenname: Xiang surname: Li fullname: Li, Xiang organization: Universität Münster – sequence: 6 givenname: Zhao‐Quan surname: Yao fullname: Yao, Zhao‐Quan organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry – sequence: 7 givenname: Jia‐Hui surname: Fan fullname: Fan, Jia‐Hui organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry – sequence: 8 givenname: Xiang surname: Wu fullname: Wu, Xiang organization: China University of Geosciences (Wuhan) – sequence: 9 givenname: Wei orcidid: 0000-0002-5277-6850 surname: Li fullname: Li, Wei email: wl276@nankai.edu.cn organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry – sequence: 10 givenname: Xian‐He orcidid: 0000-0002-2646-7974 surname: Bu fullname: Bu, Xian‐He email: buxh@nankai.edu.cn organization: Nankai University & TKL of Metal and Molecule Based Material Chemistry |
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| Keywords | Color Purity Pressure Engineering Lead Halide Perovskites Multicolor Emission |
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| Snippet | The chemical diversity and structural flexibility of lead halide perovskites (LHPs) offer tremendous opportunities to tune their optical properties through... |
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| SubjectTerms | Color Color Purity Emission Emissions Emitters External pressure External stimuli Hydrostatic pressure Lead compounds Lead Halide Perovskites Metal halides Multicolor Emission Optical properties Perovskites Photoluminescence Photons Pressure Pressure Engineering Purity Rigidity |
| Title | Pressure‐Tuned Multicolor Emission of 2D Lead Halide Perovskites with Ultrahigh Color Purity |
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