Anthraquinone Covalent Organic Framework Hollow Tubes as Binder Microadditives in Li−S Batteries
The exploration of new application forms of covalent organic frameworks (COFs) in Li−S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low‐density ad...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 3; pp. e202113315 - n/a |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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17.01.2022
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| Edition | International ed. in English |
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| Abstract | The exploration of new application forms of covalent organic frameworks (COFs) in Li−S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low‐density advantage to obtain lightweight, portable, or high‐energy‐density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone‐COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode.
Covalent organic frameworks could have implications as microadditives of binders (≈1 wt % in cathode) and a series of anthraquinone‐COF based hollow tubes have been prepared as model microadditives to obtain a high‐performance binder in Li−S batteries. |
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| AbstractList | The exploration of new application forms of covalent organic frameworks (COFs) in Li−S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low‐density advantage to obtain lightweight, portable, or high‐energy‐density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone‐COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode. The exploration of new application forms of covalent organic frameworks (COFs) in Li-S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low-density advantage to obtain lightweight, portable, or high-energy-density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone-COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode. The exploration of new application forms of covalent organic frameworks (COFs) in Li-S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low-density advantage to obtain lightweight, portable, or high-energy-density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone-COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode.The exploration of new application forms of covalent organic frameworks (COFs) in Li-S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low-density advantage to obtain lightweight, portable, or high-energy-density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone-COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode. The exploration of new application forms of covalent organic frameworks (COFs) in Li−S batteries that can overcome drawbacks like low conductivity or high loading when typically applied as sulfur host materials (mostly ≈20 to ≈40 wt % loading in cathode) is desirable to maximize their low‐density advantage to obtain lightweight, portable, or high‐energy‐density devices. Here, we establish that COFs could have implications as microadditives of binders (≈1 wt % in cathode), and a series of anthraquinone‐COF based hollow tubes have been prepared as model microadditives. The microadditives can strengthen the basic properties of the binder and spontaneously immobilize and catalytically convert lithium polysulfides, as proved by density functional calculations, thus showing almost doubly enhanced reversible capacity compared with that of the bare electrode. Covalent organic frameworks could have implications as microadditives of binders (≈1 wt % in cathode) and a series of anthraquinone‐COF based hollow tubes have been prepared as model microadditives to obtain a high‐performance binder in Li−S batteries. |
| Author | Zhou, Jie Chen, Yifa Liu, Ming Lan, Ya‐Qian Li, Qi Dong, Long‐Zhang Guo, Can Gao, Guang‐Kuo Li, Shun‐Li Tian, Xi |
| Author_xml | – sequence: 1 givenname: Can surname: Guo fullname: Guo, Can organization: South China Normal University – sequence: 2 givenname: Ming surname: Liu fullname: Liu, Ming organization: Nanjing Normal University – sequence: 3 givenname: Guang‐Kuo surname: Gao fullname: Gao, Guang‐Kuo organization: South China Normal University – sequence: 4 givenname: Xi surname: Tian fullname: Tian, Xi organization: Nanjing Normal University – sequence: 5 givenname: Jie surname: Zhou fullname: Zhou, Jie organization: South China Normal University – sequence: 6 givenname: Long‐Zhang surname: Dong fullname: Dong, Long‐Zhang organization: Nanjing Normal University – sequence: 7 givenname: Qi surname: Li fullname: Li, Qi organization: Nanjing Normal University – sequence: 8 givenname: Yifa surname: Chen fullname: Chen, Yifa email: chyf927821@163.com organization: Nanjing Normal University – sequence: 9 givenname: Shun‐Li surname: Li fullname: Li, Shun‐Li organization: Nanjing Normal University – sequence: 10 givenname: Ya‐Qian orcidid: 0000-0002-2140-7980 surname: Lan fullname: Lan, Ya‐Qian email: yqlan@njnu.edu.cn, yqlan@m.scnu.edu.cn organization: South China Normal University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34716649$$D View this record in MEDLINE/PubMed |
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| Keywords | microadditives anthraquinone covalent organic frameworks Li−S batteries batteries |
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| Snippet | The exploration of new application forms of covalent organic frameworks (COFs) in Li−S batteries that can overcome drawbacks like low conductivity or high... The exploration of new application forms of covalent organic frameworks (COFs) in Li-S batteries that can overcome drawbacks like low conductivity or high... |
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| SubjectTerms | Anthraquinone Anthraquinones Basic converters batteries Binders Cathodes covalent organic frameworks Density Lithium Li−S batteries Low conductivity microadditives Portable equipment Sulfur Tubes |
| Title | Anthraquinone Covalent Organic Framework Hollow Tubes as Binder Microadditives in Li−S Batteries |
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