From Lead Iodide to a Radical Form Lead‐Iodide Superlattice: High Conductance Gain and Broader Band for Photoconductive Response
Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superl...
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| Published in | Angewandte Chemie International Edition Vol. 58; no. 9; pp. 2692 - 2695 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
25.02.2019
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| Edition | International ed. in English |
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| Online Access | Get full text |
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| Abstract | Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI2 (EtDAB=tetraethylbenzidine), with radical and non‐radical forms. The non‐radical form has a non‐ionic structure that differs from the common ionic structures for inorganic–organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis‐IR), than pure PbI2 and the non‐radical form of the superlattice.
Lead the way: The first lead‐iodide superlattice constructed from non‐ionic organic molecules and PbI2 through van der Waals interactions is a new type of inorganic–organic hybrid and has a radical and a non‐radical form. The radical form has an almost five orders of magnitude greater conductivity and broader band photoconductive response than that of the non‐radical form or pure PbI2. |
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| AbstractList | Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI2 (EtDAB=tetraethylbenzidine), with radical and non‐radical forms. The non‐radical form has a non‐ionic structure that differs from the common ionic structures for inorganic–organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis‐IR), than pure PbI2 and the non‐radical form of the superlattice. Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI (EtDAB=tetraethylbenzidine), with radical and non-radical forms. The non-radical form has a non-ionic structure that differs from the common ionic structures for inorganic-organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis-IR), than pure PbI and the non-radical form of the superlattice. Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI 2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI 2 (EtDAB=tetraethylbenzidine), with radical and non‐radical forms. The non‐radical form has a non‐ionic structure that differs from the common ionic structures for inorganic–organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis‐IR), than pure PbI 2 and the non‐radical form of the superlattice. Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI2 (EtDAB=tetraethylbenzidine), with radical and non‐radical forms. The non‐radical form has a non‐ionic structure that differs from the common ionic structures for inorganic–organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis‐IR), than pure PbI2 and the non‐radical form of the superlattice. Lead the way: The first lead‐iodide superlattice constructed from non‐ionic organic molecules and PbI2 through van der Waals interactions is a new type of inorganic–organic hybrid and has a radical and a non‐radical form. The radical form has an almost five orders of magnitude greater conductivity and broader band photoconductive response than that of the non‐radical form or pure PbI2. Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI2 (EtDAB=tetraethylbenzidine), with radical and non-radical forms. The non-radical form has a non-ionic structure that differs from the common ionic structures for inorganic-organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis-IR), than pure PbI2 and the non-radical form of the superlattice.Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of tetraethylbenzidine (EtDAB) into interlamination of the established 2D PbI2 semiconductor through a mild solution method yielded the first lead iodide superlattice, EtDAB⋅4PbI2 (EtDAB=tetraethylbenzidine), with radical and non-radical forms. The non-radical form has a non-ionic structure that differs from the common ionic structures for inorganic-organic hybrid lead halides. The radical form shows five orders of magnitude greater conductance and broader photoconductive response range (UV/Vis → UV/Vis-IR), than pure PbI2 and the non-radical form of the superlattice. |
| Author | Wang, Guan‐E Zhang, Ning‐Ning Wang, Ming‐Sheng Xu, Gang Yao, Ming‐Shui Guo, Guo‐Cong |
| Author_xml | – sequence: 1 givenname: Guan‐E surname: Wang fullname: Wang, Guan‐E organization: Chinese Academy of Sciences – sequence: 2 givenname: Gang surname: Xu fullname: Xu, Gang organization: Chinese Academy of Sciences – sequence: 3 givenname: Ning‐Ning surname: Zhang fullname: Zhang, Ning‐Ning organization: Chinese Academy of Sciences – sequence: 4 givenname: Ming‐Shui surname: Yao fullname: Yao, Ming‐Shui organization: Chinese Academy of Sciences – sequence: 5 givenname: Ming‐Sheng orcidid: 0000-0002-2400-719X surname: Wang fullname: Wang, Ming‐Sheng email: mswang@fjirsm.ac.cn organization: Chinese Academy of Sciences – sequence: 6 givenname: Guo‐Cong surname: Guo fullname: Guo, Guo‐Cong organization: Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30614186$$D View this record in MEDLINE/PubMed |
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| Copyright | 2019 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Keywords | inorganic-organic hybrids lead halides radicals semiconductors superlattices |
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| Snippet | Superlattice materials offer new opportunities to modify optical and electrical properties of recently emerging 2D materials. The insertion of... |
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| SubjectTerms | Conductance Electrical properties Halides inorganic–organic hybrids Iodides lead halides Optical properties radicals Resistance semiconductors Superlattices |
| Title | From Lead Iodide to a Radical Form Lead‐Iodide Superlattice: High Conductance Gain and Broader Band for Photoconductive Response |
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