Revisiting the Roles of Natural Graphite in Ongoing Lithium‐Ion Batteries

Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate lithiation/de‐lithiation potential, and has been extensively used as the anode of lithium‐ion batteries (LIBs). With the requirements of reduci...

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Published inAdvanced materials (Weinheim) Vol. 34; no. 18; pp. e2106704 - n/a
Main Authors Zhao, Liang, Ding, Baichuan, Qin, Xian‐Ying, Wang, Zhijie, Lv, Wei, He, Yan‐Bing, Yang, Quan‐Hong, Kang, Feiyu
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.05.2022
Subjects
Anodes
Electrochemical analysis
Emissions control
Energy consumption
flake graphite
graphene
Graphite
Lithium-ion batteries
Materials science
microcrystalline graphite
natural graphite‐based anodes
microcrystalline graphite
lithium-ion batteries
flake graphite
graphene
natural graphite-based anodes
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Abstract Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate lithiation/de‐lithiation potential, and has been extensively used as the anode of lithium‐ion batteries (LIBs). With the requirements of reducing CO2 emission to achieve carbon neutral, the market share of NG anode will continue to grow due to its excellent processability and low production energy consumption. NG, which is abundant in China, can be divided into flake graphite (FG) and microcrystalline graphite (MG). In the past 30 years, many researchers have focused on developing modified NG and its derivatives with superior electrochemical performance, promoting their wide applications in LIBs. Here, a comprehensive overview of the origin, roles, and research progress of NG‐based materials in ongoing LIBs is provided, including their structure, properties, electrochemical performance, modification methods, derivatives, composites, and applications, especially the strategies to improve their high‐rate and low‐temperature charging performance. Prospects regarding the development orientation as well as future applications of NG‐based materials are also considered, which will provide significant guidance for the current and future research of high‐energy‐density LIBs. A comprehensive overview of natural graphite‐based materials in ongoing lithium‐ion batteries is presented, covering fundamental mechanisms, detailed applications, and an outlook of natural graphite‐based materials, from not only the aspects of structure and properties, modifications, derivatives, and composites, but also perspectives in terms of natural graphite in hybrid lithium‐ion/lithium‐metal cells and all‐solid‐state lithium batteries.
AbstractList Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate lithiation/de‐lithiation potential, and has been extensively used as the anode of lithium‐ion batteries (LIBs). With the requirements of reducing CO2 emission to achieve carbon neutral, the market share of NG anode will continue to grow due to its excellent processability and low production energy consumption. NG, which is abundant in China, can be divided into flake graphite (FG) and microcrystalline graphite (MG). In the past 30 years, many researchers have focused on developing modified NG and its derivatives with superior electrochemical performance, promoting their wide applications in LIBs. Here, a comprehensive overview of the origin, roles, and research progress of NG‐based materials in ongoing LIBs is provided, including their structure, properties, electrochemical performance, modification methods, derivatives, composites, and applications, especially the strategies to improve their high‐rate and low‐temperature charging performance. Prospects regarding the development orientation as well as future applications of NG‐based materials are also considered, which will provide significant guidance for the current and future research of high‐energy‐density LIBs.
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g –1 and appropriate lithiation/de‐lithiation potential, and has been extensively used as the anode of lithium‐ion batteries (LIBs). With the requirements of reducing CO 2 emission to achieve carbon neutral, the market share of NG anode will continue to grow due to its excellent processability and low production energy consumption. NG, which is abundant in China, can be divided into flake graphite (FG) and microcrystalline graphite (MG). In the past 30 years, many researchers have focused on developing modified NG and its derivatives with superior electrochemical performance, promoting their wide applications in LIBs. Here, a comprehensive overview of the origin, roles, and research progress of NG‐based materials in ongoing LIBs is provided, including their structure, properties, electrochemical performance, modification methods, derivatives, composites, and applications, especially the strategies to improve their high‐rate and low‐temperature charging performance. Prospects regarding the development orientation as well as future applications of NG‐based materials are also considered, which will provide significant guidance for the current and future research of high‐energy‐density LIBs.
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate lithiation/de‐lithiation potential, and has been extensively used as the anode of lithium‐ion batteries (LIBs). With the requirements of reducing CO2 emission to achieve carbon neutral, the market share of NG anode will continue to grow due to its excellent processability and low production energy consumption. NG, which is abundant in China, can be divided into flake graphite (FG) and microcrystalline graphite (MG). In the past 30 years, many researchers have focused on developing modified NG and its derivatives with superior electrochemical performance, promoting their wide applications in LIBs. Here, a comprehensive overview of the origin, roles, and research progress of NG‐based materials in ongoing LIBs is provided, including their structure, properties, electrochemical performance, modification methods, derivatives, composites, and applications, especially the strategies to improve their high‐rate and low‐temperature charging performance. Prospects regarding the development orientation as well as future applications of NG‐based materials are also considered, which will provide significant guidance for the current and future research of high‐energy‐density LIBs. A comprehensive overview of natural graphite‐based materials in ongoing lithium‐ion batteries is presented, covering fundamental mechanisms, detailed applications, and an outlook of natural graphite‐based materials, from not only the aspects of structure and properties, modifications, derivatives, and composites, but also perspectives in terms of natural graphite in hybrid lithium‐ion/lithium‐metal cells and all‐solid‐state lithium batteries.
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g and appropriate lithiation/de-lithiation potential, and has been extensively used as the anode of lithium-ion batteries (LIBs). With the requirements of reducing CO emission to achieve carbon neutral, the market share of NG anode will continue to grow due to its excellent processability and low production energy consumption. NG, which is abundant in China, can be divided into flake graphite (FG) and microcrystalline graphite (MG). In the past 30 years, many researchers have focused on developing modified NG and its derivatives with superior electrochemical performance, promoting their wide applications in LIBs. Here, a comprehensive overview of the origin, roles, and research progress of NG-based materials in ongoing LIBs is provided, including their structure, properties, electrochemical performance, modification methods, derivatives, composites, and applications, especially the strategies to improve their high-rate and low-temperature charging performance. Prospects regarding the development orientation as well as future applications of NG-based materials are also considered, which will provide significant guidance for the current and future research of high-energy-density LIBs.
Author Yang, Quan‐Hong
He, Yan‐Bing
Zhao, Liang
Qin, Xian‐Ying
Wang, Zhijie
Lv, Wei
Ding, Baichuan
Kang, Feiyu
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  surname: Zhao
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  organization: Tsinghua University
– sequence: 2
  givenname: Baichuan
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  fullname: Ding, Baichuan
  organization: Tsinghua University
– sequence: 3
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  surname: Qin
  fullname: Qin, Xian‐Ying
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– sequence: 4
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  fullname: Wang, Zhijie
  organization: Tsinghua University
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  givenname: Wei
  surname: Lv
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  organization: Tsinghua University
– sequence: 6
  givenname: Yan‐Bing
  surname: He
  fullname: He, Yan‐Bing
  organization: Tsinghua University
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  organization: Tianjin University
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  givenname: Feiyu
  orcidid: 0000-0002-3704-4379
  surname: Kang
  fullname: Kang, Feiyu
  email: fykang@mail.tsinghua.edu.cn
  organization: Tsinghua University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35032965$$D View this record in MEDLINE/PubMed
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flake graphite
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Snippet Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate...
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g and appropriate...
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g –1 and appropriate...
Graphite, commonly including artificial graphite and natural graphite (NG), possesses a relatively high theoretical capacity of 372 mA h g–1 and appropriate...
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StartPage e2106704
SubjectTerms Anodes
Electrochemical analysis
Emissions control
Energy consumption
flake graphite
graphene
Graphite
Lithium-ion batteries
Materials science
microcrystalline graphite
natural graphite‐based anodes
Title Revisiting the Roles of Natural Graphite in Ongoing Lithium‐Ion Batteries
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202106704
https://www.ncbi.nlm.nih.gov/pubmed/35032965
https://www.proquest.com/docview/2659611137
https://search.proquest.com/docview/2620079744
Volume 34
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