Priority and Prospect of Sulfide‐Based Solid‐Electrolyte Membrane

All‐solid‐state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy‐dense integration and critical intrinsic safety, yet they still require cost‐effective manufacturing and the integration of thin membrane‐based SE separators i...

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Published inAdvanced materials (Weinheim) Vol. 35; no. 50; pp. e2206013 - n/a
Main Authors Liu, Hong, Liang, Yuhao, Wang, Chao, Li, Dabing, Yan, Xiaoqin, Nan, Ce‐Wen, Fan, Li‐Zhen
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.12.2023
Subjects
all‐solid‐state lithium batteries
cell integration
Criteria
Electrolytic cells
Energy storage
Lithium batteries
Manufacturing
Mass production
Materials science
membrane processing
Membranes
Molten salt electrolytes
Separators
Solid electrolytes
Storage systems
sulfide solid electrolyte
Supply chains
all-solid-state lithium batteries
cell integration
membrane processing
sulfide solid electrolyte
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Abstract All‐solid‐state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy‐dense integration and critical intrinsic safety, yet they still require cost‐effective manufacturing and the integration of thin membrane‐based SE separators into large‐format cells to achieve scalable deployment. This review, based on an overview of sulfide SE materials, is expounded on why implementing a thin membrane‐based separator is the priority for mass production of ASSLBs and critical criteria for capturing a high‐quality thin sulfide SE membrane are identified. Moreover, from the aspects of material availability, membrane processing, and cell integration, the major challenges and associated strategies are described to meet these criteria throughout the whole manufacturing chain to provide a realistic assessment of the current status of sulfide SE membranes. Finally, future directions and prospects for scalable and manufacturable sulfide SE membranes for ASSLBs are presented. This review expounds on why implementing a membrane‐based electrolyte is the priority for mass production of all‐solid‐state lithium batteries and identifies critical criteria for capturing a high‐quality thin sulfide electrolyte membrane. The challenges and associated strategies for achieving these criteria in terms of material availability, membrane processing, and cell integration are systematically analyzed and summarized.
AbstractList All‐solid‐state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy‐dense integration and critical intrinsic safety, yet they still require cost‐effective manufacturing and the integration of thin membrane‐based SE separators into large‐format cells to achieve scalable deployment. This review, based on an overview of sulfide SE materials, is expounded on why implementing a thin membrane‐based separator is the priority for mass production of ASSLBs and critical criteria for capturing a high‐quality thin sulfide SE membrane are identified. Moreover, from the aspects of material availability, membrane processing, and cell integration, the major challenges and associated strategies are described to meet these criteria throughout the whole manufacturing chain to provide a realistic assessment of the current status of sulfide SE membranes. Finally, future directions and prospects for scalable and manufacturable sulfide SE membranes for ASSLBs are presented.
All‐solid‐state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy‐dense integration and critical intrinsic safety, yet they still require cost‐effective manufacturing and the integration of thin membrane‐based SE separators into large‐format cells to achieve scalable deployment. This review, based on an overview of sulfide SE materials, is expounded on why implementing a thin membrane‐based separator is the priority for mass production of ASSLBs and critical criteria for capturing a high‐quality thin sulfide SE membrane are identified. Moreover, from the aspects of material availability, membrane processing, and cell integration, the major challenges and associated strategies are described to meet these criteria throughout the whole manufacturing chain to provide a realistic assessment of the current status of sulfide SE membranes. Finally, future directions and prospects for scalable and manufacturable sulfide SE membranes for ASSLBs are presented. This review expounds on why implementing a membrane‐based electrolyte is the priority for mass production of all‐solid‐state lithium batteries and identifies critical criteria for capturing a high‐quality thin sulfide electrolyte membrane. The challenges and associated strategies for achieving these criteria in terms of material availability, membrane processing, and cell integration are systematically analyzed and summarized.
All-solid-state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy-dense integration and critical intrinsic safety, yet they still require cost-effective manufacturing and the integration of thin membrane-based SE separators into large-format cells to achieve scalable deployment. This review, based on an overview of sulfide SE materials, is expounded on why implementing a thin membrane-based separator is the priority for mass production of ASSLBs and critical criteria for capturing a high-quality thin sulfide SE membrane are identified. Moreover, from the aspects of material availability, membrane processing, and cell integration, the major challenges and associated strategies are described to meet these criteria throughout the whole manufacturing chain to provide a realistic assessment of the current status of sulfide SE membranes. Finally, future directions and prospects for scalable and manufacturable sulfide SE membranes for ASSLBs are presented.All-solid-state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy-dense integration and critical intrinsic safety, yet they still require cost-effective manufacturing and the integration of thin membrane-based SE separators into large-format cells to achieve scalable deployment. This review, based on an overview of sulfide SE materials, is expounded on why implementing a thin membrane-based separator is the priority for mass production of ASSLBs and critical criteria for capturing a high-quality thin sulfide SE membrane are identified. Moreover, from the aspects of material availability, membrane processing, and cell integration, the major challenges and associated strategies are described to meet these criteria throughout the whole manufacturing chain to provide a realistic assessment of the current status of sulfide SE membranes. Finally, future directions and prospects for scalable and manufacturable sulfide SE membranes for ASSLBs are presented.
Author Liang, Yuhao
Yan, Xiaoqin
Wang, Chao
Li, Dabing
Fan, Li‐Zhen
Liu, Hong
Nan, Ce‐Wen
Author_xml – sequence: 1
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  surname: Liu
  fullname: Liu, Hong
  organization: University of Science and Technology Beijing
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  givenname: Yuhao
  surname: Liang
  fullname: Liang, Yuhao
  organization: University of Science and Technology Beijing
– sequence: 3
  givenname: Chao
  surname: Wang
  fullname: Wang, Chao
  organization: University of Science and Technology Beijing
– sequence: 4
  givenname: Dabing
  surname: Li
  fullname: Li, Dabing
  organization: University of Science and Technology Beijing
– sequence: 5
  givenname: Xiaoqin
  orcidid: 0000-0002-0717-0710
  surname: Yan
  fullname: Yan, Xiaoqin
  email: xqyan@mater.ustb.edu.cn
  organization: University of Science and Technology Beijing
– sequence: 6
  givenname: Ce‐Wen
  surname: Nan
  fullname: Nan, Ce‐Wen
  organization: Tsinghua University
– sequence: 7
  givenname: Li‐Zhen
  surname: Fan
  fullname: Fan, Li‐Zhen
  email: fanlizhen@ustb.edu.cn
  organization: University of Science and Technology Beijing
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35984755$$D View this record in MEDLINE/PubMed
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Snippet All‐solid‐state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy‐dense integration...
All-solid-state lithium batteries (ASSLBs) employing sulfide solid electrolytes (SEs) promise sustainable energy storage systems with energy-dense integration...
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SubjectTerms all‐solid‐state lithium batteries
cell integration
Criteria
Electrolytic cells
Energy storage
Lithium batteries
Manufacturing
Mass production
Materials science
membrane processing
Membranes
Molten salt electrolytes
Separators
Solid electrolytes
Storage systems
sulfide solid electrolyte
Supply chains
Title Priority and Prospect of Sulfide‐Based Solid‐Electrolyte Membrane
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202206013
https://www.ncbi.nlm.nih.gov/pubmed/35984755
https://www.proquest.com/docview/2901390471
https://www.proquest.com/docview/2704869357
Volume 35
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