Intrinsic Activity Identification of Noble Metal Single‐Sites for Electrocatalytic Chlorine Evolution

• Published in: Angewandte Chemie International Edition Vol. 64; no. 2; pp. e202414202 - n/a
• Main Authors: Quan, Li, Zhao, Xin, Yang, Li‐Ming, You, Bo, Xia, Bao Yu
• Format: Journal Article
• Language: English
• Published: Germany Wiley Subscription Services, Inc 10.01.2025
• Edition: International ed. in English
• Subjects: Activity descriptor; Atomic structure; Chlorine; Chlorine evolution; Density functional theory; Electrocatalysis; Electrochemistry; Electron paramagnetic resonance; Electron spin resonance; Metals; Nitrogen; Noble metals; Raman spectroscopy; Ruthenium; Single atom catalyst; Spectroscopy; Electrocatalysis; Single atom catalyst; Activity descriptor; Chlorine evolution

Single‐atom catalysts with maximal atom‐utilization have emerged as promising alternatives for chlorine evolution reaction (CER) toward valuable Cl2 production. However, understanding their intrinsic CER activity has so far been plagued due to the lack of well‐defined atomic structure controlling. H...