Macrocycle‐Based Crystalline Supramolecular Assemblies Built with Intermolecular Charge‐Transfer Interactions
Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research pro...
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| Published in | Angewandte Chemie International Edition Vol. 62; no. 14; pp. e202218142 - n/a |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
27.03.2023
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research progress on the macrocycle‐based crystalline supramolecular assemblies primarily driven by intermolecular CT interactions (a.k.a. macrocycle‐based crystalline CT assemblies, MCCAs for short), which are classified by their donor–acceptor (D‐A) constituent elements, including simplex macrocyclic hosts, heterogeneous macrocyclic hosts, and host–guest D‐A pairs. Particular attention will be focused on their diverse functions and applications, as well as the underlying CT mechanisms from the perspective of crystal engineering. Finally, the remaining challenges and prospects are outlined.
This Minireview highlights the advancements in the field of macrocycle‐based crystalline charge‐transfer assemblies, including their preparation, structures, and diverse supramolecular functions and applications, such as vapochromic behavior and supramolecular tessellations, arising from the CT state. Future perspectives and challenges of this emerging research field are also presented. |
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| AbstractList | Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research progress on the macrocycle-based crystalline supramolecular assemblies primarily driven by intermolecular CT interactions (a.k.a. macrocycle-based crystalline CT assemblies, MCCAs for short), which are classified by their donor-acceptor (D-A) constituent elements, including simplex macrocyclic hosts, heterogeneous macrocyclic hosts, and host-guest D-A pairs. Particular attention will be focused on their diverse functions and applications, as well as the underlying CT mechanisms from the perspective of crystal engineering. Finally, the remaining challenges and prospects are outlined. Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research progress on the macrocycle‐based crystalline supramolecular assemblies primarily driven by intermolecular CT interactions (a.k.a. macrocycle‐based crystalline CT assemblies, MCCAs for short), which are classified by their donor–acceptor (D‐A) constituent elements, including simplex macrocyclic hosts, heterogeneous macrocyclic hosts, and host–guest D‐A pairs. Particular attention will be focused on their diverse functions and applications, as well as the underlying CT mechanisms from the perspective of crystal engineering. Finally, the remaining challenges and prospects are outlined. This Minireview highlights the advancements in the field of macrocycle‐based crystalline charge‐transfer assemblies, including their preparation, structures, and diverse supramolecular functions and applications, such as vapochromic behavior and supramolecular tessellations, arising from the CT state. Future perspectives and challenges of this emerging research field are also presented. Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research progress on the macrocycle-based crystalline supramolecular assemblies primarily driven by intermolecular CT interactions (a.k.a. macrocycle-based crystalline CT assemblies, MCCAs for short), which are classified by their donor-acceptor (D-A) constituent elements, including simplex macrocyclic hosts, heterogeneous macrocyclic hosts, and host-guest D-A pairs. Particular attention will be focused on their diverse functions and applications, as well as the underlying CT mechanisms from the perspective of crystal engineering. Finally, the remaining challenges and prospects are outlined.Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes, and have proved to be of great practical value in the solid state during the past few years. In this Minireview, we summarize the research progress on the macrocycle-based crystalline supramolecular assemblies primarily driven by intermolecular CT interactions (a.k.a. macrocycle-based crystalline CT assemblies, MCCAs for short), which are classified by their donor-acceptor (D-A) constituent elements, including simplex macrocyclic hosts, heterogeneous macrocyclic hosts, and host-guest D-A pairs. Particular attention will be focused on their diverse functions and applications, as well as the underlying CT mechanisms from the perspective of crystal engineering. Finally, the remaining challenges and prospects are outlined. |
| Author | Wu, Gengxin Wu, Jia‐Rui Yang, Ying‐Wei Li, Dongxia |
| Author_xml | – sequence: 1 givenname: Jia‐Rui surname: Wu fullname: Wu, Jia‐Rui organization: Jilin University – sequence: 2 givenname: Gengxin surname: Wu fullname: Wu, Gengxin organization: Jilin University – sequence: 3 givenname: Dongxia surname: Li fullname: Li, Dongxia organization: Jilin University – sequence: 4 givenname: Ying‐Wei orcidid: 0000-0001-8839-8161 surname: Yang fullname: Yang, Ying‐Wei email: ywyang@jlu.edu.cn organization: Jilin University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36651562$$D View this record in MEDLINE/PubMed |
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| Snippet | Synthetic macrocycles have served as principal tools for supramolecular chemistry, have greatly extended the scope of organic charge transfer (CT) complexes,... |
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| SubjectTerms | Assemblies Charge Transfer Host-Guest Systems Macrocycles Molecular Crystals Supramolecular Chemistry |
| Title | Macrocycle‐Based Crystalline Supramolecular Assemblies Built with Intermolecular Charge‐Transfer Interactions |
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