Unsymmetrically Chlorinated Non‐Fused Electron Acceptor Leads to High‐Efficiency and Stable Organic Solar Cells
Searching the cost‐effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non‐fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the N...
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| Published in | Angewandte Chemie International Edition Vol. 62; no. 5; pp. e202214931 - n/a |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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WEINHEIM
Wiley
26.01.2023
Wiley Subscription Services, Inc |
| Edition | International ed. in English |
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| Abstract | Searching the cost‐effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non‐fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the NFREA derived OSCs. These OSCs exhibit the superior operational stabilities under one sun equivalent illumination without ultraviolet (UV) filtration. It is revealed that the modulation of halogen substituents on aromatic side chains, as the new structural tool to tune the intermolecular interaction and optoelectronic properties of acceptors, not only promotes the interlocked tic‐tac‐toe frame of three‐dimensional stacks in solid, but also improves charge dynamics of acceptors to enable high‐performance and stable OSCs.
Two non‐fused ring electron acceptors (NFREAs) have been developed. The halogen substituents on the aromatic side chains, as the new structure design tools, not only facilitate the construction of 3D stacks in solid, but also optimize the optoelectronic properties of the NFREAs, leading to organic solar cells with 16.2 % efficiency and excellent operational stability. |
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| AbstractList | Searching the cost-effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non-fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the NFREA derived OSCs. These OSCs exhibit the superior operational stabilities under one sun equivalent illumination without ultraviolet (UV) filtration. It is revealed that the modulation of halogen substituents on aromatic side chains, as the new structural tool to tune the intermolecular interaction and optoelectronic properties of acceptors, not only promotes the interlocked tic-tac-toe frame of three-dimensional stacks in solid, but also improves charge dynamics of acceptors to enable high-performance and stable OSCs.Searching the cost-effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non-fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the NFREA derived OSCs. These OSCs exhibit the superior operational stabilities under one sun equivalent illumination without ultraviolet (UV) filtration. It is revealed that the modulation of halogen substituents on aromatic side chains, as the new structural tool to tune the intermolecular interaction and optoelectronic properties of acceptors, not only promotes the interlocked tic-tac-toe frame of three-dimensional stacks in solid, but also improves charge dynamics of acceptors to enable high-performance and stable OSCs. Searching the cost‐effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non‐fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the NFREA derived OSCs. These OSCs exhibit the superior operational stabilities under one sun equivalent illumination without ultraviolet (UV) filtration. It is revealed that the modulation of halogen substituents on aromatic side chains, as the new structural tool to tune the intermolecular interaction and optoelectronic properties of acceptors, not only promotes the interlocked tic‐tac‐toe frame of three‐dimensional stacks in solid, but also improves charge dynamics of acceptors to enable high‐performance and stable OSCs. Searching the cost‐effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled. Herein, we have succeeded in developing two non‐fused ring electron acceptors (NFREAs), leading to the highest efficiency of 16.2 % for the NFREA derived OSCs. These OSCs exhibit the superior operational stabilities under one sun equivalent illumination without ultraviolet (UV) filtration. It is revealed that the modulation of halogen substituents on aromatic side chains, as the new structural tool to tune the intermolecular interaction and optoelectronic properties of acceptors, not only promotes the interlocked tic‐tac‐toe frame of three‐dimensional stacks in solid, but also improves charge dynamics of acceptors to enable high‐performance and stable OSCs. Two non‐fused ring electron acceptors (NFREAs) have been developed. The halogen substituents on the aromatic side chains, as the new structure design tools, not only facilitate the construction of 3D stacks in solid, but also optimize the optoelectronic properties of the NFREAs, leading to organic solar cells with 16.2 % efficiency and excellent operational stability. |
| Author | Ma, De‐Li Zhang, Qian‐Qian Li, Chang‐Zhi |
| Author_xml | – sequence: 1 givenname: De‐Li orcidid: 0000-0002-7399-3766 surname: Ma fullname: Ma, De‐Li organization: Zhejiang University – sequence: 2 givenname: Qian‐Qian surname: Zhang fullname: Zhang, Qian‐Qian organization: Zhejiang University – sequence: 3 givenname: Chang‐Zhi orcidid: 0000-0003-1968-2032 surname: Li fullname: Li, Chang‐Zhi email: czli@zju.edu.cn organization: Zhejiang University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36433656$$D View this record in MEDLINE/PubMed |
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| Keywords | 3D Network EXCITON VOLTAGE IMPACT Chlorination Non-Fused-Ring Acceptor Single Crystal DELOCALIZATION Organic Solar Cells ENABLES |
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| Snippet | Searching the cost‐effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled.... Searching the cost-effective organic semiconductors is strongly needed in order to facilitate the practice of organic solar cells (OSCs), yet to be fulfilled.... |
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| SubjectTerms | 3D Network Chemistry Chemistry, Multidisciplinary Chlorination Non-Fused-Ring Acceptor Optoelectronics Organic semiconductors Organic Solar Cells Photovoltaic cells Physical Sciences Science & Technology Single Crystal Solar cells |
| Title | Unsymmetrically Chlorinated Non‐Fused Electron Acceptor Leads to High‐Efficiency and Stable Organic Solar Cells |
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