Research Advances in Amorphous‐Crystalline Heterostructures Toward Efficient Electrochemical Applications

Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous‐crystalline heterostructur...

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Published inSmall (Weinheim an der Bergstrasse, Germany) Vol. 19; no. 10; pp. e2206081 - n/a
Main Authors Jin, Yachao, Zhang, Mengxian, Song, Li, Zhang, Mingdao
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.03.2023
Subjects
amorphous‐crystalline heterostructures
Clean energy
Electrocatalysts
Electrochemical analysis
Energy conversion
energy conversion and storage
Energy storage
heterointerfaces
Heterostructures
Hydrogen evolution reactions
Lithium sulfur batteries
Lithium-ion batteries
Nanotechnology
Oxygen evolution reactions
synergistic effect
energy conversion and storage
heterointerfaces
amorphous-crystalline heterostructures
synergistic effect
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Abstract Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous‐crystalline heterostructures have lately surged since they combine the superior advantages of amorphous‐ and crystalline‐phase structures, showing unusual atomic arrangements in heterointerfaces. Nonetheless, there has been much less efforts in systematic analysis and summary of the amorphous‐crystalline heterostructures to examine their complicated interfacial interactions and elusory active sites. The critical structure‐activity correlation and electrocatalytic mechanism remain rather elusive. In this review, the recent advances of amorphous‐crystalline heterostructures in electrochemical energy conversion and storage fields are amply discussed and presented, along with remarks on the challenges and perspectives. Initially, the fundamental characteristics of amorphous‐crystalline heterostructures are introduced to provide scientific viewpoints for structural understanding. Subsequently, the superiorities and current achievements of amorphous‐crystalline heterostructures as highly efficient electrocatalysts/electrodes for hydrogen evolution reaction, oxygen evolution reaction, supercapacitor, lithium‐ion battery, and lithium‐sulfur battery applications are elaborated. At the end of this review, future outlooks and opportunities on amorphous‐crystalline heterostructures are also put forward to promote their further development and application in the field of clean energy. The emerging amorphous‐crystalline heterostructures with distinctive atomic arrangement at the heterointerfaces are promising candidates for next‐generation high‐performance electrocatalysts/electrodes. This review discusses for the first time these ever‐increasing novel multifunctional nanomaterials toward various electrochemical applications, aiming to offer cross‐sectional insights into the structure‐property relationships and provide guidance for the rational design of amorphous‐crystalline heterostructures with desired performance.
AbstractList Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous‐crystalline heterostructures have lately surged since they combine the superior advantages of amorphous‐ and crystalline‐phase structures, showing unusual atomic arrangements in heterointerfaces. Nonetheless, there has been much less efforts in systematic analysis and summary of the amorphous‐crystalline heterostructures to examine their complicated interfacial interactions and elusory active sites. The critical structure‐activity correlation and electrocatalytic mechanism remain rather elusive. In this review, the recent advances of amorphous‐crystalline heterostructures in electrochemical energy conversion and storage fields are amply discussed and presented, along with remarks on the challenges and perspectives. Initially, the fundamental characteristics of amorphous‐crystalline heterostructures are introduced to provide scientific viewpoints for structural understanding. Subsequently, the superiorities and current achievements of amorphous‐crystalline heterostructures as highly efficient electrocatalysts/electrodes for hydrogen evolution reaction, oxygen evolution reaction, supercapacitor, lithium‐ion battery, and lithium‐sulfur battery applications are elaborated. At the end of this review, future outlooks and opportunities on amorphous‐crystalline heterostructures are also put forward to promote their further development and application in the field of clean energy.
Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous‐crystalline heterostructures have lately surged since they combine the superior advantages of amorphous‐ and crystalline‐phase structures, showing unusual atomic arrangements in heterointerfaces. Nonetheless, there has been much less efforts in systematic analysis and summary of the amorphous‐crystalline heterostructures to examine their complicated interfacial interactions and elusory active sites. The critical structure‐activity correlation and electrocatalytic mechanism remain rather elusive. In this review, the recent advances of amorphous‐crystalline heterostructures in electrochemical energy conversion and storage fields are amply discussed and presented, along with remarks on the challenges and perspectives. Initially, the fundamental characteristics of amorphous‐crystalline heterostructures are introduced to provide scientific viewpoints for structural understanding. Subsequently, the superiorities and current achievements of amorphous‐crystalline heterostructures as highly efficient electrocatalysts/electrodes for hydrogen evolution reaction, oxygen evolution reaction, supercapacitor, lithium‐ion battery, and lithium‐sulfur battery applications are elaborated. At the end of this review, future outlooks and opportunities on amorphous‐crystalline heterostructures are also put forward to promote their further development and application in the field of clean energy. The emerging amorphous‐crystalline heterostructures with distinctive atomic arrangement at the heterointerfaces are promising candidates for next‐generation high‐performance electrocatalysts/electrodes. This review discusses for the first time these ever‐increasing novel multifunctional nanomaterials toward various electrochemical applications, aiming to offer cross‐sectional insights into the structure‐property relationships and provide guidance for the rational design of amorphous‐crystalline heterostructures with desired performance.
Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous-crystalline heterostructures have lately surged since they combine the superior advantages of amorphous- and crystalline-phase structures, showing unusual atomic arrangements in heterointerfaces. Nonetheless, there has been much less efforts in systematic analysis and summary of the amorphous-crystalline heterostructures to examine their complicated interfacial interactions and elusory active sites. The critical structure-activity correlation and electrocatalytic mechanism remain rather elusive. In this review, the recent advances of amorphous-crystalline heterostructures in electrochemical energy conversion and storage fields are amply discussed and presented, along with remarks on the challenges and perspectives. Initially, the fundamental characteristics of amorphous-crystalline heterostructures are introduced to provide scientific viewpoints for structural understanding. Subsequently, the superiorities and current achievements of amorphous-crystalline heterostructures as highly efficient electrocatalysts/electrodes for hydrogen evolution reaction, oxygen evolution reaction, supercapacitor, lithium-ion battery, and lithium-sulfur battery applications are elaborated. At the end of this review, future outlooks and opportunities on amorphous-crystalline heterostructures are also put forward to promote their further development and application in the field of clean energy.Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the electrochemical performance for various applications. In this context related research of the newly proposed amorphous-crystalline heterostructures have lately surged since they combine the superior advantages of amorphous- and crystalline-phase structures, showing unusual atomic arrangements in heterointerfaces. Nonetheless, there has been much less efforts in systematic analysis and summary of the amorphous-crystalline heterostructures to examine their complicated interfacial interactions and elusory active sites. The critical structure-activity correlation and electrocatalytic mechanism remain rather elusive. In this review, the recent advances of amorphous-crystalline heterostructures in electrochemical energy conversion and storage fields are amply discussed and presented, along with remarks on the challenges and perspectives. Initially, the fundamental characteristics of amorphous-crystalline heterostructures are introduced to provide scientific viewpoints for structural understanding. Subsequently, the superiorities and current achievements of amorphous-crystalline heterostructures as highly efficient electrocatalysts/electrodes for hydrogen evolution reaction, oxygen evolution reaction, supercapacitor, lithium-ion battery, and lithium-sulfur battery applications are elaborated. At the end of this review, future outlooks and opportunities on amorphous-crystalline heterostructures are also put forward to promote their further development and application in the field of clean energy.
Author Jin, Yachao
Song, Li
Zhang, Mingdao
Zhang, Mengxian
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  surname: Jin
  fullname: Jin, Yachao
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  organization: Nanjing University of Information Science & Technology
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  surname: Zhang
  fullname: Zhang, Mengxian
  organization: Nanjing University of Information Science & Technology
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  fullname: Song, Li
  organization: Nanjing University of Information Science & Technology
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  givenname: Mingdao
  surname: Zhang
  fullname: Zhang, Mingdao
  email: zhangmd@nuist.edu.cn
  organization: Nanjing University of Information Science & Technology
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Thu Apr 03 07:02:40 EDT 2025
Tue Jul 01 02:54:22 EDT 2025
Thu Apr 24 23:10:06 EDT 2025
Wed Jan 22 16:23:13 EST 2025
IsPeerReviewed true
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Issue 10
Keywords energy conversion and storage
heterointerfaces
amorphous-crystalline heterostructures
synergistic effect
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Snippet Interface engineering of heterostructures has proven a promising strategy to effectively modulate their physicochemical properties and further improve the...
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SubjectTerms amorphous‐crystalline heterostructures
Clean energy
Electrocatalysts
Electrochemical analysis
Energy conversion
energy conversion and storage
Energy storage
heterointerfaces
Heterostructures
Hydrogen evolution reactions
Lithium sulfur batteries
Lithium-ion batteries
Nanotechnology
Oxygen evolution reactions
synergistic effect
Title Research Advances in Amorphous‐Crystalline Heterostructures Toward Efficient Electrochemical Applications
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fsmll.202206081
https://www.ncbi.nlm.nih.gov/pubmed/36526597
https://www.proquest.com/docview/2785181457
https://www.proquest.com/docview/2755575034
Volume 19
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