π‐Expanded Carbazoles as Hole‐Selective Self‐Assembled Monolayers for High‐Performance Perovskite Solar Cells
Carbazole‐derived self‐assembled monolayers (SAMs) are promising hole‐selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover,...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 51; pp. e202213560 - n/a |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
WEINHEIM
Wiley
19.12.2022
Wiley Subscription Services, Inc |
| Edition | International ed. in English |
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| Abstract | Carbazole‐derived self‐assembled monolayers (SAMs) are promising hole‐selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole‐derived SAMs, CbzPh and CbzNaph through asymmetric or helical π‐expansion for improved molecular dipole moment and strengthened π‐π interaction. The helical π‐expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its π‐scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability.
A molecular design strategy is introduced for carbazole‐derived self‐assembled monolayers (SAM) to facilitate dense assembly and tune the indium tinoxide (ITO) workfunction. Through asymmetric or helical π‐expansion, CbzPh and CbzNaph are obtained as efficient hole‐selective layers (HSL) for inverted perovskite solar cells (PSC). Larger molecular dipoles in CbzPh and CbzNaph can better tune the ITO workfunction, whereas the stronger π‐π interactions ensure more ordered and denser SAM assembly. |
|---|---|
| AbstractList | Carbazole-derived self-assembled monolayers (SAMs) are promising hole-selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole-derived SAMs, CbzPh and CbzNaph through asymmetric or helical π-expansion for improved molecular dipole moment and strengthened π-π interaction. The helical π-expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its π-scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability.Carbazole-derived self-assembled monolayers (SAMs) are promising hole-selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole-derived SAMs, CbzPh and CbzNaph through asymmetric or helical π-expansion for improved molecular dipole moment and strengthened π-π interaction. The helical π-expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its π-scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability. Carbazole‐derived self‐assembled monolayers (SAMs) are promising hole‐selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole‐derived SAMs, CbzPh and CbzNaph through asymmetric or helical π‐expansion for improved molecular dipole moment and strengthened π‐π interaction. The helical π‐expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its π‐scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability. Carbazole-derived self-assembled monolayers (SAMs) are promising hole-selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole-derived SAMs, CbzPh and CbzNaph through asymmetric or helical pi-expansion for improved molecular dipole moment and strengthened pi-pi interaction. The helical pi-expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its pi-scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability. Carbazole‐derived self‐assembled monolayers (SAMs) are promising hole‐selective materials for inverted perovskite solar cells (PSCs). However, they often possess small dipoles which prohibit them from effectively modulating the workfunction of ITO substrate, limiting the PSC photovoltage. Moreover, their properties can be drastically affected by even subtle structural modifications, undermining the final PSC performance. Here, we designed two carbazole‐derived SAMs, CbzPh and CbzNaph through asymmetric or helical π‐expansion for improved molecular dipole moment and strengthened π‐π interaction. The helical π‐expanded CbzNaph has the largest dipole, forming densely packed and ordered monolayer, facilitated by the highly ordered assembly observed in its π‐scaffold's single crystal. These synergistically modulate the perovskite crystallization atop and tune the ITO workfunction. Consequently, the champion PSC employing CbzNaph showed an excellent 24.1 % efficiency and improved stability. A molecular design strategy is introduced for carbazole‐derived self‐assembled monolayers (SAM) to facilitate dense assembly and tune the indium tinoxide (ITO) workfunction. Through asymmetric or helical π‐expansion, CbzPh and CbzNaph are obtained as efficient hole‐selective layers (HSL) for inverted perovskite solar cells (PSC). Larger molecular dipoles in CbzPh and CbzNaph can better tune the ITO workfunction, whereas the stronger π‐π interactions ensure more ordered and denser SAM assembly. |
| Author | Li, Mingliang Qi, Feng Lin, Francis R. Jen, Alex K.‐Y. Li, Fengzhu Jiang, Wenlin |
| Author_xml | – sequence: 1 givenname: Wenlin orcidid: 0000-0003-2387-1901 surname: Jiang fullname: Jiang, Wenlin organization: City University of Hong Kong – sequence: 2 givenname: Fengzhu surname: Li fullname: Li, Fengzhu organization: City University of Hong Kong – sequence: 3 givenname: Mingliang surname: Li fullname: Li, Mingliang organization: City University of Hong Kong – sequence: 4 givenname: Feng surname: Qi fullname: Qi, Feng organization: City University of Hong Kong – sequence: 5 givenname: Francis R. surname: Lin fullname: Lin, Francis R. organization: City University of Hong Kong – sequence: 6 givenname: Alex K.‐Y. orcidid: 0000-0002-9219-7749 surname: Jen fullname: Jen, Alex K.‐Y. email: alexjen@cityu.edu.hk organization: City University of Hong Kong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36300589$$D View this record in MEDLINE/PubMed |
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| Keywords | PHOSPHONIC-ACIDS Perovskite SPIN-CAST Self-Assembled Monolayer Hole-Selective Layer Carbazole Solar Cells EFFICIENCY SURFACES |
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| PublicationCentury | 2000 |
| PublicationDate | December 19, 2022 |
| PublicationDateYYYYMMDD | 2022-12-19 |
| PublicationDate_xml | – month: 12 year: 2022 text: December 19, 2022 day: 19 |
| PublicationDecade | 2020 |
| PublicationPlace | WEINHEIM |
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| PublicationTitle | Angewandte Chemie International Edition |
| PublicationTitleAbbrev | ANGEW CHEM INT EDIT |
| PublicationTitleAlternate | Angew Chem Int Ed Engl |
| PublicationYear | 2022 |
| Publisher | Wiley Wiley Subscription Services, Inc |
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| Snippet | Carbazole‐derived self‐assembled monolayers (SAMs) are promising hole‐selective materials for inverted perovskite solar cells (PSCs). However, they often... Carbazole-derived self-assembled monolayers (SAMs) are promising hole-selective materials for inverted perovskite solar cells (PSCs). However, they often... |
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| SubjectTerms | Carbazole Carbazoles Chemistry Chemistry, Multidisciplinary Crystallization Dipole moments Hole-Selective Layer Monolayers Perovskite Perovskites Photovoltaic cells Physical Sciences Science & Technology Self-Assembled Monolayer Single crystals Solar Cells Substrates |
| Title | π‐Expanded Carbazoles as Hole‐Selective Self‐Assembled Monolayers for High‐Performance Perovskite Solar Cells |
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