Charge‐Assisted Ionic Hydrogen‐Bonded Organic Frameworks: Designable and Stabilized Multifunctional Materials

Hydrogen‐bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydroge...

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Published inChemistry : a European journal Vol. 30; no. 17; pp. e202303580 - n/a
Main Authors Chen, Xu‐Yong, Cao, Li‐Hui, Bai, Xiang‐Tian, Cao, Xiao‐Jie
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 20.03.2024
Subjects
charge-assisted
Construction
Covalent bonds
designable
Hydrogen
Hydrogen bonding
Hydrogen bonds
hydrogen-bonded organic frameworks
Interpenetrating networks
ionic
Ligands
multifunctional
Multifunctional materials
Proton conduction
stabilized
Structural stability
charge-assisted, ionic, hydrogen-bonded organic frameworks, designable, stabilized, multifunctional
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Abstract Hydrogen‐bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π–π stacking, highly interpenetrated networks, charge‐assisted, ligand‐bond‐assisted, molecular weaving, and covalent cross‐linking. Charge‐assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge‐assisted ionic HOFs, and introduces the different building block construction modes of charge‐assisted ionic HOFs. Highlight the applications of charge‐assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge‐assisted ionic HOFs structures and multifunctional applications. Strategies for the construction of charge‐assisted ionic hydrogen‐bonded organic frameworks (HOFs) as well as recent advances form the focus of this review. The applications of these charge‐assisted ionic hydrogen‐bonded organic frameworks in gas adsorption and separation, proton conduction, and biological applications are highlighted, as well as prospects for future developments in this field.
AbstractList Hydrogen-bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π-π stacking, highly interpenetrated networks, charge-assisted, ligand-bond-assisted, molecular weaving, and covalent cross-linking. Charge-assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge-assisted ionic HOFs, and introduces the different building block construction modes of charge-assisted ionic HOFs. Highlight the applications of charge-assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge-assisted ionic HOFs structures and multifunctional applications.Hydrogen-bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π-π stacking, highly interpenetrated networks, charge-assisted, ligand-bond-assisted, molecular weaving, and covalent cross-linking. Charge-assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge-assisted ionic HOFs, and introduces the different building block construction modes of charge-assisted ionic HOFs. Highlight the applications of charge-assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge-assisted ionic HOFs structures and multifunctional applications.
Hydrogen‐bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π–π stacking, highly interpenetrated networks, charge‐assisted, ligand‐bond‐assisted, molecular weaving, and covalent cross‐linking. Charge‐assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge‐assisted ionic HOFs, and introduces the different building block construction modes of charge‐assisted ionic HOFs. Highlight the applications of charge‐assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge‐assisted ionic HOFs structures and multifunctional applications.
Hydrogen-bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π-π stacking, highly interpenetrated networks, charge-assisted, ligand-bond-assisted, molecular weaving, and covalent cross-linking. Charge-assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge-assisted ionic HOFs, introduces the different building block construction modes of charge-assisted ionic HOFs. Highlight the applications of charge-assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge-assisted ionic HOFs structures and multifunctional applications.
Hydrogen‐bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high crystallinity, mild reaction conditions, good solution processability, and reproducibility. Coupled with the reversibility and flexibility of hydrogen bonds, HOFs can be assembled into a wide diversity of crystalline structures. Since the bonding energy of hydrogen bonds is lower than that of ligand and covalent bonds, the framework of HOFs is prone to collapse after desolventisation and the stability is not high, which limits the development and application of HOFs. In recent years, numerous stable and functional HOFs have been developed by π–π stacking, highly interpenetrated networks, charge‐assisted, ligand‐bond‐assisted, molecular weaving, and covalent cross‐linking. Charge‐assisted ionic HOFs introduce electrostatic attraction into HOFs to improve stability while enriching structural diversity and functionality. In this paper, we review the development, the principles of rational design and assembly of charge‐assisted ionic HOFs, and introduces the different building block construction modes of charge‐assisted ionic HOFs. Highlight the applications of charge‐assisted ionic HOFs in gas adsorption and separation, proton conduction, biological applications, etc., and prospects for the diverse design of charge‐assisted ionic HOFs structures and multifunctional applications. Strategies for the construction of charge‐assisted ionic hydrogen‐bonded organic frameworks (HOFs) as well as recent advances form the focus of this review. The applications of these charge‐assisted ionic hydrogen‐bonded organic frameworks in gas adsorption and separation, proton conduction, and biological applications are highlighted, as well as prospects for future developments in this field.
Author Bai, Xiang‐Tian
Cao, Li‐Hui
Chen, Xu‐Yong
Cao, Xiao‐Jie
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  surname: Chen
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  surname: Cao
  fullname: Cao, Li‐Hui
  email: caolihui@sust.edu.cn
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  fullname: Bai, Xiang‐Tian
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  surname: Cao
  fullname: Cao, Xiao‐Jie
  organization: Shaanxi University of Science and Technology
BackLink https://www.ncbi.nlm.nih.gov/pubmed/38179818$$D View this record in MEDLINE/PubMed
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2023; 23
2023; 29
2015; 44
2020; 49
2016; 353
2011; 21
2014; 9
2001; 13
2012; 336
2023; 10
2021; 7
2015; 15
2021; 6
2007; 129
2018; 140
2023; 11
2013; 42
2023; 19
2017; 23
1996; 52
2016; 52
2019; 141
2016; 55
2022; 144
2021; 13
2021; 12
2023
2022; 61
2017; 12
2010; 132
2013; 135
1988; 110
2016; 138
2013; 495
2022; 55
2009; 38
2007; 46
2019; 131
2018; 57
1994; 6
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Yang J. (e_1_2_8_96_1) 2020; 399
e_1_2_8_13_1
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Zhou Q. (e_1_2_8_180_1) 2023
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Snippet Hydrogen‐bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high...
Hydrogen-bonded organic frameworks (HOFs) are a class of crystalline framework materials assembled by hydrogen bonds. HOFs have the advantages of high...
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SubjectTerms charge-assisted
Construction
Covalent bonds
designable
Hydrogen
Hydrogen bonding
Hydrogen bonds
hydrogen-bonded organic frameworks
Interpenetrating networks
ionic
Ligands
multifunctional
Multifunctional materials
Proton conduction
stabilized
Structural stability
Title Charge‐Assisted Ionic Hydrogen‐Bonded Organic Frameworks: Designable and Stabilized Multifunctional Materials
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fchem.202303580
https://www.ncbi.nlm.nih.gov/pubmed/38179818
https://www.proquest.com/docview/2984996389
https://www.proquest.com/docview/2915987631
Volume 30
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