Boundary‐Rich Carbon‐Based Electrocatalysts with Manganese(II)‐Coordinated Active Environment for Selective Synthesis of Hydrogen Peroxide

• Published in: Angewandte Chemie International Edition Vol. 63; no. 13; pp. e202317660 - n/a
• Main Authors: Dong, Ling‐Yu, Wang, Jing‐Song, Li, Tian‐Yi, Wu, Tao, Hu, Xu, Wu, Yu‐Tai, Zhu, Min‐Yi, Hao, Guang‐Ping, Lu, An‐Hui
• Format: Journal Article
• Language: English
• Published: Germany Wiley Subscription Services, Inc 22.03.2024
• Edition: International ed. in English
• Subjects: Adsorption; Benzamide; Benzonitrile; Carbon; Cascade chemical reactions; Catalysts; Charge transfer; Electrocatalysts; Electron spin; Electronic properties; Electronic structure; electrosynthesis; Enrichment; Hydrogen peroxide; Hydroxyl groups; Manganese; nonprecious catalysts; Oxygen enrichment; porous carbons; Synthesis; tandem reaction; tandem reaction; nonprecious catalysts; electrosynthesis; porous carbons; hydrogen peroxide

Coordinated manganese (Mn) electrocatalysts owing to their electronic structure flexibility, non‐toxic and earth abundant features are promising for electrocatalytic reactions. However, achieving selective hydrogen peroxide (H2O2) production through two electron oxygen reduction (2e‐ORR) is a challe...