Efficient and Color‐Tunable Dual‐Mode Afterglow from Large‐Area and Flexible Polymer‐Based Transparent Films for Anti‐Counterfeiting and Information Encryption

It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual‐mo...

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Published inAngewandte Chemie International Edition Vol. 61; no. 23; pp. e202201820 - n/a
Main Authors Yang, Yifan, Liang, Yaohui, Zheng, Yitao, Li, Jian‐An, Wu, Shiying, Zhang, Huaqing, Huang, Tepeng, Luo, Suilian, Liu, Cong, Shi, Guang, Sun, Fengqiang, Chi, Zhenguo, Xu, Bingjia
Format Journal Article
LanguageEnglish
Published WEINHEIM Wiley 07.06.2022
Wiley Subscription Services, Inc
EditionInternational ed. in English
Subjects
Afterglow
Anti-Counterfeiting
Chemistry
Chemistry, Multidisciplinary
Color
Counterfeiting
Doped Polymer Films
Phosphorescence
Physical Sciences
Polymer films
Polymers
Polyvinyl alcohol
Science & Technology
Thermally Activated Delayed Fluorescence
Doped Polymer Films
Afterglow
Phosphorescence
ROOM-TEMPERATURE PHOSPHORESCENCE
Thermally Activated Delayed Fluorescence
Anti-Counterfeiting
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Abstract It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual‐mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA‐doped PVA film exhibits intense blue afterglow with Φafterglow and τafterglow up to 19.8 % and 1.81 s, respectively, representing state‐of‐the‐art dual‐mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large‐area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature‐sensitive security ink for anti‐counterfeiting and information encryption. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films simultaneously produce persistent thermally activated delayed fluorescence and ultralong organic phosphorescence, and their afterglow colors can be linearly tuned by temperature. Besides, the IbCzA‐doped PVA film presents state‐of‐the‐art dual‐mode organic afterglow performance.
AbstractList It remains a great challenge to develop polymer-based materials with efficient and color-tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual-mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA-doped PVA film exhibits intense blue afterglow with Φafterglow and τafterglow up to 19.8 % and 1.81 s, respectively, representing state-of-the-art dual-mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large-area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature-sensitive security ink for anti-counterfeiting and information encryption.It remains a great challenge to develop polymer-based materials with efficient and color-tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual-mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA-doped PVA film exhibits intense blue afterglow with Φafterglow and τafterglow up to 19.8 % and 1.81 s, respectively, representing state-of-the-art dual-mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large-area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature-sensitive security ink for anti-counterfeiting and information encryption.
It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual‐mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA‐doped PVA film exhibits intense blue afterglow with Φ afterglow and τ afterglow up to 19.8 % and 1.81 s, respectively, representing state‐of‐the‐art dual‐mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large‐area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature‐sensitive security ink for anti‐counterfeiting and information encryption.
It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual‐mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA‐doped PVA film exhibits intense blue afterglow with Φafterglow and τafterglow up to 19.8 % and 1.81 s, respectively, representing state‐of‐the‐art dual‐mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large‐area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature‐sensitive security ink for anti‐counterfeiting and information encryption.
It remains a great challenge to develop polymer-based materials with efficient and color-tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual-mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA-doped PVA film exhibits intense blue afterglow with Φ and τ up to 19.8 % and 1.81 s, respectively, representing state-of-the-art dual-mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large-area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature-sensitive security ink for anti-counterfeiting and information encryption.
It remains a great challenge to develop polymer-based materials with efficient and color-tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual-mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA-doped PVA film exhibits intense blue afterglow with phi(afterglow) and tau(afterglow) up to 19.8 % and 1.81 s, respectively, representing state-of-the-art dual-mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large-area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature-sensitive security ink for anti-counterfeiting and information encryption.
It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films can produce unique dual‐mode afterglow, which is composed of persistent thermally activated delayed fluorescence and ultralong organic phosphorescence. Besides, the IbCzA‐doped PVA film exhibits intense blue afterglow with Φafterglow and τafterglow up to 19.8 % and 1.81 s, respectively, representing state‐of‐the‐art dual‐mode organic afterglow performance. Moreover, our reported film has high flexibility, excellent transparency, and large‐area producibility; and the afterglow color of the film can be linearly tuned by temperature. Inspired by these distinctive properties, the PVA doped with IbCzA was employed as temperature‐sensitive security ink for anti‐counterfeiting and information encryption. Two indolocarbazole derivatives IaCzA and IbCzA have been synthesized and doped into poly(vinyl alcohol) (PVA) matrices. It is found that the resulting films simultaneously produce persistent thermally activated delayed fluorescence and ultralong organic phosphorescence, and their afterglow colors can be linearly tuned by temperature. Besides, the IbCzA‐doped PVA film presents state‐of‐the‐art dual‐mode organic afterglow performance.
ArticleNumber 202201820
Author Shi, Guang
Liang, Yaohui
Wu, Shiying
Li, Jian‐An
Chi, Zhenguo
Sun, Fengqiang
Liu, Cong
Xu, Bingjia
Zheng, Yitao
Yang, Yifan
Zhang, Huaqing
Luo, Suilian
Huang, Tepeng
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  fullname: Liang, Yaohui
  organization: South China Normal University
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  givenname: Yitao
  surname: Zheng
  fullname: Zheng, Yitao
  organization: South China Normal University
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  givenname: Jian‐An
  surname: Li
  fullname: Li, Jian‐An
  organization: South China Normal University
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  givenname: Shiying
  surname: Wu
  fullname: Wu, Shiying
  organization: South China Normal University
– sequence: 6
  givenname: Huaqing
  surname: Zhang
  fullname: Zhang, Huaqing
  organization: South China Normal University
– sequence: 7
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  surname: Huang
  fullname: Huang, Tepeng
  organization: South China Normal University
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  fullname: Luo, Suilian
  organization: South China Normal University
– sequence: 9
  givenname: Cong
  surname: Liu
  fullname: Liu, Cong
  organization: South China Normal University
– sequence: 10
  givenname: Guang
  surname: Shi
  fullname: Shi, Guang
  email: shiguang@scnu.edu.cn
  organization: South China Normal University
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  surname: Sun
  fullname: Sun, Fengqiang
  organization: South China Normal University
– sequence: 12
  givenname: Zhenguo
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  fullname: Chi, Zhenguo
  email: chizhg@mail.sysu.edu.cn
  organization: Sun Yat-sen University
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  givenname: Bingjia
  orcidid: 0000-0001-6580-3240
  surname: Xu
  fullname: Xu, Bingjia
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  organization: South China Normal University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35315193$$D View this record in MEDLINE/PubMed
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Keywords Doped Polymer Films
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Thermally Activated Delayed Fluorescence
Anti-Counterfeiting
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Snippet It remains a great challenge to develop polymer‐based materials with efficient and color‐tunable organic afterglow. Two indolocarbazole derivatives IaCzA and...
It remains a great challenge to develop polymer-based materials with efficient and color-tunable organic afterglow. Two indolocarbazole derivatives IaCzA and...
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StartPage e202201820
SubjectTerms Afterglow
Anti-Counterfeiting
Chemistry
Chemistry, Multidisciplinary
Color
Counterfeiting
Doped Polymer Films
Phosphorescence
Physical Sciences
Polymer films
Polymers
Polyvinyl alcohol
Science & Technology
Thermally Activated Delayed Fluorescence
Title Efficient and Color‐Tunable Dual‐Mode Afterglow from Large‐Area and Flexible Polymer‐Based Transparent Films for Anti‐Counterfeiting and Information Encryption
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.202201820
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https://www.ncbi.nlm.nih.gov/pubmed/35315193
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