Heterostructures Regulating Lithium Polysulfides for Advanced Lithium‐Sulfur Batteries

Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium‐sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single‐component materials in regulating lithium po...

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Published inAdvanced materials (Weinheim) Vol. 35; no. 47; pp. e2303520 - n/a
Main Authors Wang, Tao, He, Jiarui, Zhu, Zhi, Cheng, Xin‐Bing, Zhu, Jian, Lu, Bingan, Wu, Yuping
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.11.2023
Subjects
adsorption
catalysis
heterostructure
Heterostructures
Interlayers
Lithium sulfur batteries
lithium‐sulfur battery
Materials science
Polysulfides
Reaction kinetics
shuttling effect
catalysis
adsorption
lithium-sulfur battery
shuttling effect
heterostructure
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Abstract Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium‐sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single‐component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium‐sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailedly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium‐sulfur batteries is systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium‐sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium‐sulfur batteries. Heterostructures could regulate lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium‐sulfur batteries. This review systematically and detailedly analyzes the principle and the application of heterostructures as sulfur host, interlayer, and separator modifier to promote the performance of lithium‐sulfur batteries.
AbstractList Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium‐sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single‐component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium‐sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailedly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium‐sulfur batteries is systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium‐sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium‐sulfur batteries. Heterostructures could regulate lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium‐sulfur batteries. This review systematically and detailedly analyzes the principle and the application of heterostructures as sulfur host, interlayer, and separator modifier to promote the performance of lithium‐sulfur batteries.
Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium‐sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single‐component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium‐sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailedly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium‐sulfur batteries is systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium‐sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium‐sulfur batteries.
Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium-sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single-component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium-sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium-sulfur batteries are systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium-sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium sulfur batteries. This article is protected by copyright. All rights reserved.
Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium-sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single-component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium-sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailedly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium-sulfur batteries is systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium-sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium-sulfur batteries.Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium-sulfur batteries. Heterostructures, due to unique properties, have congenital advantages that are difficult to be achieved by single-component materials in regulating lithium polysulfides by efficient catalysis and strong adsorption to solve the problems of poor reaction kinetics and serious shuttling effect of lithium-sulfur batteries. In this review, the principles of heterostructures expediting lithium polysulfides conversion and anchoring lithium polysulfides are detailedly analyzed, and the application of heterostructures as sulfur host, interlayer, and separator modifier to improve the performance of lithium-sulfur batteries is systematically reviewed. Finally, the problems that need to be solved in the future study and application of heterostructures in lithium-sulfur batteries are prospected. This review will provide a valuable reference for the development of heterostructures in advanced lithium-sulfur batteries.
Author Lu, Bingan
Zhu, Zhi
Cheng, Xin‐Bing
Zhu, Jian
Wang, Tao
He, Jiarui
Wu, Yuping
Author_xml – sequence: 1
  givenname: Tao
  orcidid: 0000-0003-0454-7081
  surname: Wang
  fullname: Wang, Tao
  organization: Southeast University
– sequence: 2
  givenname: Jiarui
  orcidid: 0000-0003-4665-2306
  surname: He
  fullname: He, Jiarui
  organization: Southeast University
– sequence: 3
  givenname: Zhi
  surname: Zhu
  fullname: Zhu, Zhi
  organization: Southeast University
– sequence: 4
  givenname: Xin‐Bing
  orcidid: 0000-0001-7567-1210
  surname: Cheng
  fullname: Cheng, Xin‐Bing
  organization: Southeast University
– sequence: 5
  givenname: Jian
  orcidid: 0000-0001-9852-1645
  surname: Zhu
  fullname: Zhu, Jian
  organization: Hunan University
– sequence: 6
  givenname: Bingan
  orcidid: 0000-0002-0075-5898
  surname: Lu
  fullname: Lu, Bingan
  organization: Hunan University
– sequence: 7
  givenname: Yuping
  orcidid: 0000-0002-0833-1205
  surname: Wu
  fullname: Wu, Yuping
  email: wuyp@fudan.edu.cn
  organization: Southeast University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/37254027$$D View this record in MEDLINE/PubMed
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shuttling effect
heterostructure
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Snippet Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium‐sulfur batteries. Heterostructures,...
Sluggish reaction kinetics and severe shuttling effect of lithium polysulfides seriously hinder the development of lithium-sulfur batteries. Heterostructures,...
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SubjectTerms adsorption
catalysis
heterostructure
Heterostructures
Interlayers
Lithium sulfur batteries
lithium‐sulfur battery
Materials science
Polysulfides
Reaction kinetics
shuttling effect
Title Heterostructures Regulating Lithium Polysulfides for Advanced Lithium‐Sulfur Batteries
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202303520
https://www.ncbi.nlm.nih.gov/pubmed/37254027
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Volume 35
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