Engineering efficient hole transport layer Ferrihydrite-MXene on BiVO4 photoanodes for photoelectrochemical water splitting: Work function and conductivity regulated
Although great interest is focused on development of semiconductor photoanodes for efficient photoelectrochemical (PEC) water splitting, the pressing bottleneck to address the intrinsic charge transport for enhancement of PEC performance still remains to be resolved. Herein, hole transport layer (Fh...
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| Published in | Applied catalysis. B, Environmental Vol. 315; p. 121606 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
15.10.2022
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| Subjects | |
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| Abstract | Although great interest is focused on development of semiconductor photoanodes for efficient photoelectrochemical (PEC) water splitting, the pressing bottleneck to address the intrinsic charge transport for enhancement of PEC performance still remains to be resolved. Herein, hole transport layer (Fh-MXene) constructed by doping of MXene (Ti3C2) in Ferrihydrite (Fh) is loaded on BiVO4 photoanode. This novel BiVO4@Fh-MXene photoanode achieves high current density of 4.55 mA cm−2 at 1.23 V versus reversible hydrogen electrode (vs. RHE), exhibiting excellent photostability. From electrochemical analysis and density functional theory calculations, high PEC performance is ascribed to incorporation of Fh-MXene as hole transport layer, enhancing conductivity and water oxidation reaction. Notably, MXene can improve band alignment of BiVO4/Fh-MXene interface by tuning work function, which strengthens the built-in electric field for more efficient hole extraction. This work provides a simple method to design photoanodes with efficient charge transport layers for feasible PEC water splitting application.
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•Novel hole transfer layer Fh-MXene loaded on BiVO4 photoanode for PEC water splitting.•MXene tune work function of Fh for strengthening the built-in electric field.•Fh-MXene with high conductivity promote the intrinsic charge transport of photoanode.•Exposure of metal sites and hydrophilic functional groups improve water oxidation.•BiVO4@Fh-MXene photoanode exhibit five times enhanced PEC performance than BiVO4. |
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| AbstractList | Although great interest is focused on development of semiconductor photoanodes for efficient photoelectrochemical (PEC) water splitting, the pressing bottleneck to address the intrinsic charge transport for enhancement of PEC performance still remains to be resolved. Herein, hole transport layer (Fh-MXene) constructed by doping of MXene (Ti3C2) in Ferrihydrite (Fh) is loaded on BiVO4 photoanode. This novel BiVO4@Fh-MXene photoanode achieves high current density of 4.55 mA cm−2 at 1.23 V versus reversible hydrogen electrode (vs. RHE), exhibiting excellent photostability. From electrochemical analysis and density functional theory calculations, high PEC performance is ascribed to incorporation of Fh-MXene as hole transport layer, enhancing conductivity and water oxidation reaction. Notably, MXene can improve band alignment of BiVO4/Fh-MXene interface by tuning work function, which strengthens the built-in electric field for more efficient hole extraction. This work provides a simple method to design photoanodes with efficient charge transport layers for feasible PEC water splitting application.
[Display omitted]
•Novel hole transfer layer Fh-MXene loaded on BiVO4 photoanode for PEC water splitting.•MXene tune work function of Fh for strengthening the built-in electric field.•Fh-MXene with high conductivity promote the intrinsic charge transport of photoanode.•Exposure of metal sites and hydrophilic functional groups improve water oxidation.•BiVO4@Fh-MXene photoanode exhibit five times enhanced PEC performance than BiVO4. |
| ArticleNumber | 121606 |
| Author | Wang, Jinnan Corvini, Philippe François-Xavier Bai, Weihao Zhou, Ye Peng, Gang Li, Aimin |
| Author_xml | – sequence: 1 givenname: Weihao surname: Bai fullname: Bai, Weihao organization: State Key Laboratory of Pollution Control and Resource Reuse & School of the Environment Nanjing University, Nanjing 210023, China – sequence: 2 givenname: Ye surname: Zhou fullname: Zhou, Ye organization: State Key Laboratory of Pollution Control and Resource Reuse & School of the Environment Nanjing University, Nanjing 210023, China – sequence: 3 givenname: Gang surname: Peng fullname: Peng, Gang organization: State Key Laboratory of Pollution Control and Resource Reuse & School of the Environment Nanjing University, Nanjing 210023, China – sequence: 4 givenname: Jinnan surname: Wang fullname: Wang, Jinnan email: wjnnju@163.com organization: State Key Laboratory of Pollution Control and Resource Reuse & School of the Environment Nanjing University, Nanjing 210023, China – sequence: 5 givenname: Aimin surname: Li fullname: Li, Aimin organization: State Key Laboratory of Pollution Control and Resource Reuse & School of the Environment Nanjing University, Nanjing 210023, China – sequence: 6 givenname: Philippe François-Xavier surname: Corvini fullname: Corvini, Philippe François-Xavier organization: School of Life Sciences, University of Applied Sciences and Arts Northwestern Switzerland, Basel 4132, Switzerland |
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| Keywords | Work function and conductivity regulated Hole transport layer BiVO4 photoanodes Ferrihydrite-MXene Photoelectrochemical water splitting |
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| StartPage | 121606 |
| SubjectTerms | BiVO4 photoanodes Ferrihydrite-MXene Hole transport layer Photoelectrochemical water splitting Work function and conductivity regulated |
| Title | Engineering efficient hole transport layer Ferrihydrite-MXene on BiVO4 photoanodes for photoelectrochemical water splitting: Work function and conductivity regulated |
| URI | https://dx.doi.org/10.1016/j.apcatb.2022.121606 |
| Volume | 315 |
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