Spatially-controlled complex molecules and their applications
The understanding of molecular structure and function is at the very heart of the chemical and molecular sciences. Experiments that allow for the creation of structurally pure samples and the investigation of their molecular dynamics and chemical function have developed tremendeously over the last f...
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| Published in | International reviews in physical chemistry Vol. 34; no. 4; pp. 557 - 590 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Abingdon
Taylor & Francis
02.10.2015
Taylor & Francis Ltd |
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| Online Access | Get full text |
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| Abstract | The understanding of molecular structure and function is at the very heart of the chemical and molecular sciences. Experiments that allow for the creation of structurally pure samples and the investigation of their molecular dynamics and chemical function have developed tremendeously over the last few decades, although 'there's plenty of room at the bottom' for better control as well as further applications. Here, we describe the use of inhomogeneous electric fields for the manipulation of neutral molecules in the gas-phase, i.e. for the separation of complex molecules according to size, structural isomer, and quantum state. For these complex molecules, all quantum states are strong-field seeking, requiring dynamic fields for their confinement. Current applications of these controlled samples are summarised and interesting future applications discussed. |
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| AbstractList | The understanding of molecular structure and function is at the very heart of the chemical and molecular sciences. Experiments that allow for the creation of structurally pure samples and the investigation of their molecular dynamics and chemical function have developed tremendeously over the last few decades, although 'there's plenty of room at the bottom' for better control as well as further applications. Here, we describe the use of inhomogeneous electric fields for the manipulation of neutral molecules in the gas-phase, i.e. for the separation of complex molecules according to size, structural isomer, and quantum state. For these complex molecules, all quantum states are strong-field seeking, requiring dynamic fields for their confinement. Current applications of these controlled samples are summarised and interesting future applications discussed. |
| Author | Horke, Daniel A. Chang, Yuan-Pin Trippel, Sebastian Küpper, Jochen |
| Author_xml | – sequence: 1 givenname: Yuan-Pin surname: Chang fullname: Chang, Yuan-Pin organization: Center for Free-Electron Laser Science, DESY – sequence: 2 givenname: Daniel A. surname: Horke fullname: Horke, Daniel A. organization: Center for Free-Electron Laser Science, DESY – sequence: 3 givenname: Sebastian surname: Trippel fullname: Trippel, Sebastian organization: Center for Free-Electron Laser Science, DESY – sequence: 4 givenname: Jochen orcidid: 0000-0003-4395-9345 surname: Küpper fullname: Küpper, Jochen email: jochen.kuepper@cfel.de organization: The Hamburg Center for Ultrafast Imaging, Universität Hamburg |
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| SubjectTerms | alignment and orientation chirality Confinement conformer selection controlled molecules Dynamics Electric fields enantiomer separation Inhomogeneous electric fields Isomers Molecular dynamics Molecular structure Molecules Physical chemistry Quantum physics quantum-state selection reaction dynamics and kinetics Separation structure-function relationship |
| Title | Spatially-controlled complex molecules and their applications |
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