Surface activated polyethylene separator promoting Li+ ion transport in gel polymer electrolytes and cycling stability of Li-metal anode
[Display omitted] •A surface activated polyethylene separator was used to support gel polymer electrolyte.•Li+ ion transport ability was improved in gel polymer electrolyte.•Effective lithium dendrite suppression and extended cycle lifespan were demonstrated. This paper proposes a strategy to fabric...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 368; pp. 321 - 330 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.07.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•A surface activated polyethylene separator was used to support gel polymer electrolyte.•Li+ ion transport ability was improved in gel polymer electrolyte.•Effective lithium dendrite suppression and extended cycle lifespan were demonstrated.
This paper proposes a strategy to fabricate surface activated polyethylene (PE)-supported gel polymer electrolyte (GPE) with high ion transport ability, excellent electrolyte retention and mechanical properties to stabilize lithium (Li)-metal anodes. The inert outer and inner pore surface activation of polyethylene is demonstrated by coating an ultrathin zirconium oxide nanocrystal (ZrO2)/polyhedral oligomeric silsesquioxane (POSS) composite layer through a simple layer by layer (LBL) assembly method prior to the in situ polymerization. It is found that the activation layer may improve the Li+ ion transference number and induce the formation of GPE with a gradient structure by the interaction with the initiator system, giving rise to higher ion transport ability of final GPE. On the other hand, the GPE using the activated PE separator as support improves the Li/electrolyte interfacial stability during storage and repeated lithium plating/stripping cycling. A stable voltage profile with cycling for more than 800 h in a Li/Li symmetric cell was obtained by using surface activated PE-supported GPE. When it is assembled into the cells with metallic lithium anodes and lithium cobalt oxide (LiCoO2) cathodes, the cells show excellent rate capability and cycling performance, as well as effective dendrite inhibition. |
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| AbstractList | This paper proposes a strategy to fabricate surface activated polyethylene (PE)-supported gel polymer electrolyte (GPE) with high ion transport ability, excellent electrolyte retention and mechanical properties to stabilize lithium (Li)-metal anodes. The inert outer and inner pore surface activation of polyethylene is demonstrated by coating an ultrathin zirconium oxide nanocrystal (ZrO2)/polyhedral oligomeric silsesquioxane (POSS) composite layer through a simple layer by layer (LBL) assembly method prior to the in situ polymerization. It is found that the activation layer may improve the Li+ ion transference number and induce the formation of GPE with a gradient structure by the interaction with the initiator system, giving rise to higher ion transport ability of final GPE. On the other hand, the GPE using the activated PE separator as support improves the Li/electrolyte interfacial stability during storage and repeated lithium plating/stripping cycling. A stable voltage profile with cycling for more than 800 h in a Li/Li symmetric cell was obtained by using surface activated PE-supported GPE. When it is assembled into the cells with metallic lithium anodes and lithium cobalt oxide (LiCoO2) cathodes, the cells show excellent rate capability and cycling performance, as well as effective dendrite inhibition. [Display omitted] •A surface activated polyethylene separator was used to support gel polymer electrolyte.•Li+ ion transport ability was improved in gel polymer electrolyte.•Effective lithium dendrite suppression and extended cycle lifespan were demonstrated. This paper proposes a strategy to fabricate surface activated polyethylene (PE)-supported gel polymer electrolyte (GPE) with high ion transport ability, excellent electrolyte retention and mechanical properties to stabilize lithium (Li)-metal anodes. The inert outer and inner pore surface activation of polyethylene is demonstrated by coating an ultrathin zirconium oxide nanocrystal (ZrO2)/polyhedral oligomeric silsesquioxane (POSS) composite layer through a simple layer by layer (LBL) assembly method prior to the in situ polymerization. It is found that the activation layer may improve the Li+ ion transference number and induce the formation of GPE with a gradient structure by the interaction with the initiator system, giving rise to higher ion transport ability of final GPE. On the other hand, the GPE using the activated PE separator as support improves the Li/electrolyte interfacial stability during storage and repeated lithium plating/stripping cycling. A stable voltage profile with cycling for more than 800 h in a Li/Li symmetric cell was obtained by using surface activated PE-supported GPE. When it is assembled into the cells with metallic lithium anodes and lithium cobalt oxide (LiCoO2) cathodes, the cells show excellent rate capability and cycling performance, as well as effective dendrite inhibition. |
| Author | Zhu, Jiefang Shi, Liyi Edström, Kristina Zhao, Yin Mindemark, Jonas Qiu, Zhengfu Yuan, Shuai Wang, Zhuyi |
| Author_xml | – sequence: 1 givenname: Zhengfu surname: Qiu fullname: Qiu, Zhengfu organization: School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China – sequence: 2 givenname: Liyi surname: Shi fullname: Shi, Liyi organization: Research Centre of Nanoscience and Nanotechnology, Shanghai University, Shanghai 200444, China – sequence: 3 givenname: Zhuyi orcidid: 0000-0002-6326-8106 surname: Wang fullname: Wang, Zhuyi email: bamboo2009@shu.edu.cn organization: Research Centre of Nanoscience and Nanotechnology, Shanghai University, Shanghai 200444, China – sequence: 4 givenname: Jonas surname: Mindemark fullname: Mindemark, Jonas organization: Department of Chemistry-Ångström Laboratory, Uppsala University, SE-751 21 Uppsala, Sweden – sequence: 5 givenname: Jiefang orcidid: 0000-0002-6531-185X surname: Zhu fullname: Zhu, Jiefang organization: Department of Chemistry-Ångström Laboratory, Uppsala University, SE-751 21 Uppsala, Sweden – sequence: 6 givenname: Kristina surname: Edström fullname: Edström, Kristina organization: Department of Chemistry-Ångström Laboratory, Uppsala University, SE-751 21 Uppsala, Sweden – sequence: 7 givenname: Yin orcidid: 0000-0001-6718-2994 surname: Zhao fullname: Zhao, Yin organization: Research Centre of Nanoscience and Nanotechnology, Shanghai University, Shanghai 200444, China – sequence: 8 givenname: Shuai surname: Yuan fullname: Yuan, Shuai email: s.yuan@shu.edu.cn organization: Research Centre of Nanoscience and Nanotechnology, Shanghai University, Shanghai 200444, China |
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•A surface activated polyethylene separator was used to support gel polymer electrolyte.•Li+ ion transport ability was improved in gel... This paper proposes a strategy to fabricate surface activated polyethylene (PE)-supported gel polymer electrolyte (GPE) with high ion transport ability,... |
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| StartPage | 321 |
| SubjectTerms | Gel polymer electrolyte Li-metal anode Polyethylene support Surface activation |
| Title | Surface activated polyethylene separator promoting Li+ ion transport in gel polymer electrolytes and cycling stability of Li-metal anode |
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