Modulation of destructive quantum interference by bridge groups in truxene-based single-molecule junctions

Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order...

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Published inChemical communications (Cambridge, England) Vol. 57; no. 5; pp. 667 - 67
Main Authors Wang, Lin, Zhao, Zhihao, Shinde, Digambar B, Lai, Zhiping, Wang, Dong
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 21.01.2021
Subjects
Carbonyls
electron transfer
Electron transport
energy
Interference
Measurement techniques
nitrogen
Resistance
Transport properties
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Abstract Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order of magnitude compared with non-substituted analogues. It can be ascribed that the anti-resonance feature produced by destructive quantum interference (DQI) is alleviated and pushed away from the Fermi energy. These findings provide an effective chemical strategy for manipulating the DQI behavior in single molecular devices. Nitrogen and carbonyl bridge substituents embedded in truxene derivatives enhance the single-molecule conductance prominently by alleviating the destructive quantum interference effect and pushing away the anti-resonance dip from the Fermi energy.
AbstractList Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order of magnitude compared with non-substituted analogues. It can be ascribed that the anti-resonance feature produced by destructive quantum interference (DQI) is alleviated and pushed away from the Fermi energy. These findings provide an effective chemical strategy for manipulating the DQI behavior in single molecular devices.
Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order of magnitude compared with non-substituted analogues. It can be ascribed that the anti-resonance feature produced by destructive quantum interference (DQI) is alleviated and pushed away from the Fermi energy. These findings provide an effective chemical strategy for manipulating the DQI behavior in single molecular devices.Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order of magnitude compared with non-substituted analogues. It can be ascribed that the anti-resonance feature produced by destructive quantum interference (DQI) is alleviated and pushed away from the Fermi energy. These findings provide an effective chemical strategy for manipulating the DQI behavior in single molecular devices.
Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical study. Molecules with nitrogen and carbonyl substituents at the bridge sites exhibit higher single-molecule conductances by almost one order of magnitude compared with non-substituted analogues. It can be ascribed that the anti-resonance feature produced by destructive quantum interference (DQI) is alleviated and pushed away from the Fermi energy. These findings provide an effective chemical strategy for manipulating the DQI behavior in single molecular devices. Nitrogen and carbonyl bridge substituents embedded in truxene derivatives enhance the single-molecule conductance prominently by alleviating the destructive quantum interference effect and pushing away the anti-resonance dip from the Fermi energy.
Author Wang, Lin
Lai, Zhiping
Wang, Dong
Zhao, Zhihao
Shinde, Digambar B
AuthorAffiliation King Abdullah University of Science and Technology (KAUST)
Institute of Chemistry
China University of Geosciences
Chinese Academy of Sciences (CAS)
School of Materials Science and Technology
Division of Physical Science and Engineering
CAS Key Laboratory of Molecular Nanostructure and Nanotechnology and Beijing National Laboratory for Molecular Sciences
Advanced Membranes and Porous Materials Center
University of Chinese Academy of Sciences
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– name: CAS Key Laboratory of Molecular Nanostructure and Nanotechnology and Beijing National Laboratory for Molecular Sciences
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Snippet Electron transport properties of polycyclic truxene derivatives have been investigated by the single molecule conductance measurement technique and theoretical...
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SubjectTerms Carbonyls
electron transfer
Electron transport
energy
Interference
Measurement techniques
nitrogen
Resistance
Transport properties
Title Modulation of destructive quantum interference by bridge groups in truxene-based single-molecule junctions
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Volume 57
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