Microscopic Observation of π Spin Polarization by d Localized Spin in λ Type BETS Based Organic Superconductors

In this study, 77Se NMR measurements were carried out to detect the π spin polarization of the organic BETS (BETS = Bis(ethylenedithio)tetraselenafulvalene) molecule of the field induced superconductor, λ-(BETS)2Fe1−xGaxCl4, which shows a superconducting transition at relatively low magnetic field c...

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Published inCrystals (Basel) Vol. 10; no. 11; p. 1055
Main Authors Hiraki, Ko-ichi, Takahashi, Toshihiro, Akiba, Hiroshi, Nishio, Yutaka, Zhou, Biao
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 01.11.2020
Subjects
(BETS)2Fe1−xGaxCl4
Dependence
Electrolytes
Exchanging
FISC
Heat
Low temperature
Magnetic fields
NMR
Nuclear magnetic resonance
Organic superconductors
Polarization (spin alignment)
Single crystals
π-d interaction
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Abstract In this study, 77Se NMR measurements were carried out to detect the π spin polarization of the organic BETS (BETS = Bis(ethylenedithio)tetraselenafulvalene) molecule of the field induced superconductor, λ-(BETS)2Fe1−xGaxCl4, which shows a superconducting transition at relatively low magnetic field compared to the non-doped λ-(BETS)2FeCl4. From the analysis of the NMR spectrum at low temperature, it was clarified that the exchange interaction between π and 3d spins in the Ga doping system is smaller than that in the Fe salt. It is also clarified that the conduction π spins feel the “averaged” exchange field from the localized 3d spins at the dilute Fe sites.
AbstractList In this study, 77Se NMR measurements were carried out to detect the π spin polarization of the organic BETS (BETS = Bis(ethylenedithio)tetraselenafulvalene) molecule of the field induced superconductor, λ-(BETS)2Fe1−xGaxCl4, which shows a superconducting transition at relatively low magnetic field compared to the non-doped λ-(BETS)2FeCl4. From the analysis of the NMR spectrum at low temperature, it was clarified that the exchange interaction between π and 3d spins in the Ga doping system is smaller than that in the Fe salt. It is also clarified that the conduction π spins feel the “averaged” exchange field from the localized 3d spins at the dilute Fe sites.
Author Nishio, Yutaka
Takahashi, Toshihiro
Akiba, Hiroshi
Hiraki, Ko-ichi
Zhou, Biao
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  surname: Zhou
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Snippet In this study, 77Se NMR measurements were carried out to detect the π spin polarization of the organic BETS (BETS = Bis(ethylenedithio)tetraselenafulvalene)...
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StartPage 1055
SubjectTerms (BETS)2Fe1−xGaxCl4
Dependence
Electrolytes
Exchanging
FISC
Heat
Low temperature
Magnetic fields
NMR
Nuclear magnetic resonance
Organic superconductors
Polarization (spin alignment)
Single crystals
π-d interaction
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Title Microscopic Observation of π Spin Polarization by d Localized Spin in λ Type BETS Based Organic Superconductors
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