Fabrication of a Liquid Scintillator based on 7-Diethylamino-4-Methylcoumarin for Radiation Detection
Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are easy to manufacture, large in size, and have a short fluorescence decay time. However, they are not suitable for gamma spectroscopy because they are...
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| Published in | Journal of fluorescence Vol. 33; no. 5; pp. 1705 - 1716 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Springer US
01.09.2023
Springer Nature B.V |
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| Abstract | Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are easy to manufacture, large in size, and have a short fluorescence decay time. However, they are not suitable for gamma spectroscopy because they are composed of a low-atomic-number material. In this regard, alternative materials for the secondary solute used in basic organic liquid scintillators have been investigated, and the applicability of alternative materials, the detection characteristics, and neutron/gamma identification tests were all assessed. 7-Diethylamino-4-methylcoumarin (DMC), selected as an alternative material, is a benzopyrone derivative in the form of colorless crystals with high fluorescence, a high quantum yield in the visible region, and excellent light stability. In addition, it has a large Stokes shift, and solubility in a solvent is good. Through an analysis in this study, it was found that the absorption wavelength range of DMC coincides with the emission wavelength range of PPO, which is the primary solute used with DMC. Finally, it was confirmed that the optimal concentration of DMC was 0.08 wt%. As a result of performing gamma and neutron measurement tests using a DMC-based liquid scintillator, it was found to perform well (FOM = 1.42) compared to a commercial liquid scintillator, BC-501A. |
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| AbstractList | Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are easy to manufacture, large in size, and have a short fluorescence decay time. However, they are not suitable for gamma spectroscopy because they are composed of a low-atomic-number material. In this regard, alternative materials for the secondary solute used in basic organic liquid scintillators have been investigated, and the applicability of alternative materials, the detection characteristics, and neutron/gamma identification tests were all assessed. 7-Diethylamino-4-methylcoumarin (DMC), selected as an alternative material, is a benzopyrone derivative in the form of colorless crystals with high fluorescence, a high quantum yield in the visible region, and excellent light stability. In addition, it has a large Stokes shift, and solubility in a solvent is good. Through an analysis in this study, it was found that the absorption wavelength range of DMC coincides with the emission wavelength range of PPO, which is the primary solute used with DMC. Finally, it was confirmed that the optimal concentration of DMC was 0.08 wt%. As a result of performing gamma and neutron measurement tests using a DMC-based liquid scintillator, it was found to perform well (FOM = 1.42) compared to a commercial liquid scintillator, BC-501A. Abstract Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are easy to manufacture, large in size, and have a short fluorescence decay time. However, they are not suitable for gamma spectroscopy because they are composed of a low-atomic-number material. In this regard, alternative materials for the secondary solute used in basic organic liquid scintillators have been investigated, and the applicability of alternative materials, the detection characteristics, and neutron/gamma identification tests were all assessed. 7-Diethylamino-4-methylcoumarin (DMC), selected as an alternative material, is a benzopyrone derivative in the form of colorless crystals with high fluorescence, a high quantum yield in the visible region, and excellent light stability. In addition, it has a large Stokes shift, and solubility in a solvent is good. Through an analysis in this study, it was found that the absorption wavelength range of DMC coincides with the emission wavelength range of PPO, which is the primary solute used with DMC. Finally, it was confirmed that the optimal concentration of DMC was 0.08 wt%. As a result of performing gamma and neutron measurement tests using a DMC-based liquid scintillator, it was found to perform well (FOM = 1.42) compared to a commercial liquid scintillator, BC-501A. |
| Author | Hong, Sang Bum Roh, Changhyun Park, Yong Dae Lee, Chae Hun Min, Su Jung Yoon, Seon Kwang Seo, Bum Kyoung Cheong, Jae Hak |
| Author_xml | – sequence: 1 givenname: Su Jung surname: Min fullname: Min, Su Jung organization: Department of Nuclear Engineering, Kyung Hee University, Decommissioning Technology Research Division, Korea Atomic Energy Research Institute (KAERI) – sequence: 2 givenname: Yong Dae surname: Park fullname: Park, Yong Dae organization: Radiation Research Division, Korea Atomic Energy Research Institute (KAERI) – sequence: 3 givenname: Seon Kwang surname: Yoon fullname: Yoon, Seon Kwang organization: Advanced Fuel Cycle System Research Division, Korea Atomic Energy Research Institute (KAERI), Nuclear Science and Technology, Quantum Energy Chemical Engineering, University of Science and Technology (UST) – sequence: 4 givenname: Chae Hun surname: Lee fullname: Lee, Chae Hun organization: Advanced Fuel Cycle System Research Division, Korea Atomic Energy Research Institute (KAERI) – sequence: 5 givenname: Bum Kyoung surname: Seo fullname: Seo, Bum Kyoung organization: Decommissioning Technology Research Division, Korea Atomic Energy Research Institute (KAERI) – sequence: 6 givenname: Jae Hak surname: Cheong fullname: Cheong, Jae Hak email: jhcheong@khu.ac.kr organization: Department of Nuclear Engineering, Kyung Hee University – sequence: 7 givenname: Changhyun surname: Roh fullname: Roh, Changhyun email: chroh@kaeri.re.kr organization: Decommissioning Technology Research Division, Korea Atomic Energy Research Institute (KAERI), Nuclear Science and Technology, Quantum Energy Chemical Engineering, University of Science and Technology (UST) – sequence: 8 givenname: Sang Bum surname: Hong fullname: Hong, Sang Bum email: sbhong@kaeri.re.kr organization: Decommissioning Technology Research Division, Korea Atomic Energy Research Institute (KAERI) |
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| Keywords | Fabrication Gamma rays Fluorescence Detection Liquid scintillator 7-Diethylamino-4-methylcoumarin |
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| Snippet | Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are easy to... Abstract Organic liquid scintillation detectors are widely used to measure the presence of radiation. With these devices, there are advantages in that they are... |
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| SubjectTerms | Analytical Chemistry Atomic properties Biochemistry Biological and Medical Physics Biomedical and Life Sciences Biomedicine Biophysics Biotechnology Fluorescence Gamma spectroscopy Organic liquids Radiation Scintillation counters |
| Title | Fabrication of a Liquid Scintillator based on 7-Diethylamino-4-Methylcoumarin for Radiation Detection |
| URI | https://link.springer.com/article/10.1007/s10895-023-03162-x https://www.ncbi.nlm.nih.gov/pubmed/36826726 https://www.proquest.com/docview/2870006526/abstract/ https://search.proquest.com/docview/2780070393 |
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