Effect of adsorbed water on wetting properties of borosilicate glass, quartz, and sapphire
Contact angles of a variety of hydrophobic liquids were measured on clean surfaces of borosilicate glass, quartz, and sapphire at 20°C with the RH at 0.6% and 95%. The adsorption of water molecules at 0.6% RH resulted in the formation of only a fraction of a monolayer; yet it converted each high-ene...
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| Published in | Journal of colloid and interface science Vol. 29; no. 3; pp. 413 - 423 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
01.01.1969
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| Online Access | Get full text |
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| Abstract | Contact angles of a variety of hydrophobic liquids were measured on clean surfaces of borosilicate glass, quartz, and sapphire at 20°C with the RH at 0.6% and 95%. The adsorption of water molecules at 0.6% RH resulted in the formation of only a fraction of a monolayer; yet it converted each high-energy solid surface to one having a low critical surface tension of wetting,
γ
c
. The increased amount of water adsorbed at 95% RH to form a film comprising little more than a condensed monolayer further lowered
γ
c
to a value somewhat above that of bulk water. At each relative humidity investigated the value of
γ
c
was the same for each of these three solids; hence
γ
c
was dependent upon the surface concentration of adsorbed water but was independent of the chemical nature of the solid substrate. The somewhat different values of
γ
c
obtained on using several different homologous series of hydrophobic liquids are explained in terms of differences in the contribution from nondispersion interfacial forces acting between the water film and the contacting organic liquid molecules. These results reveal clearly the important influence of only a monolayer of adsorbed water upon the spreading, adhesion, and contact angles of organic liquids resting upon high-energy, hydrophilic, solid surfaces. |
|---|---|
| AbstractList | Contact angles of a variety of hydrophobic liquids were measured on clean surfaces of borosilicate glass, quartz, and sapphire at 20°C with the RH at 0.6% and 95%. The adsorption of water molecules at 0.6% RH resulted in the formation of only a fraction of a monolayer; yet it converted each high-energy solid surface to one having a low critical surface tension of wetting,
γ
c
. The increased amount of water adsorbed at 95% RH to form a film comprising little more than a condensed monolayer further lowered
γ
c
to a value somewhat above that of bulk water. At each relative humidity investigated the value of
γ
c
was the same for each of these three solids; hence
γ
c
was dependent upon the surface concentration of adsorbed water but was independent of the chemical nature of the solid substrate. The somewhat different values of
γ
c
obtained on using several different homologous series of hydrophobic liquids are explained in terms of differences in the contribution from nondispersion interfacial forces acting between the water film and the contacting organic liquid molecules. These results reveal clearly the important influence of only a monolayer of adsorbed water upon the spreading, adhesion, and contact angles of organic liquids resting upon high-energy, hydrophilic, solid surfaces. |
| Author | Bernett, Marianne K Zisman, W.A |
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| Cites_doi | 10.1016/0095-8522(58)90010-2 10.1111/j.1151-2916.1962.tb11096.x 10.1021/j100862a038 10.1002/pen.760070104 10.1021/j100864a020 10.1021/ja01433a001 10.1016/0095-8522(50)90044-4 10.1039/jr9620002206 10.1021/j100884a511 10.1111/j.1151-2916.1967.tb15166.x 10.1038/2051005b0 10.1016/0095-8522(65)90006-1 10.1021/j100881a006 10.1021/j100871a064 10.1021/j100814a032 10.1021/ba-1964-0043.ch001 10.1016/0021-9797(67)90272-X 10.1016/0042-207X(60)90112-3 |
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| Snippet | Contact angles of a variety of hydrophobic liquids were measured on clean surfaces of borosilicate glass, quartz, and sapphire at 20°C with the RH at 0.6% and... |
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| Title | Effect of adsorbed water on wetting properties of borosilicate glass, quartz, and sapphire |
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