Co, Fe codoped holey carbon nanosheets as bifunctional oxygen electrocatalysts for rechargeable Zn-air batteries
Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm...
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| Published in | Chemical communications (Cambridge, England) Vol. 57; no. 16; pp. 249 - 252 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
25.02.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm
−2
for the OER, outperforming commercial Pt/C and IrO
2
, respectively. Furthermore, as the air-cathode for rechargeable Zn-air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm
−2
and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion.
CoFe@HNSs exhibited bifunctional oxygen electrocatalytic activity, and exhibit a high-power density of 131.3 mW cm
−2
and long-term stability over 140 h. |
|---|---|
| AbstractList | Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm−2 for the OER, outperforming commercial Pt/C and IrO2, respectively. Furthermore, as the air-cathode for rechargeable Zn–air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm−2 and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm −2 for the OER, outperforming commercial Pt/C and IrO 2 , respectively. Furthermore, as the air-cathode for rechargeable Zn–air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm −2 and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm-2 for the OER, outperforming commercial Pt/C and IrO2, respectively. Furthermore, as the air-cathode for rechargeable Zn-air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm-2 and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion.Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm-2 for the OER, outperforming commercial Pt/C and IrO2, respectively. Furthermore, as the air-cathode for rechargeable Zn-air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm-2 and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm⁻² for the OER, outperforming commercial Pt/C and IrO₂, respectively. Furthermore, as the air-cathode for rechargeable Zn–air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm⁻² and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm −2 for the OER, outperforming commercial Pt/C and IrO 2 , respectively. Furthermore, as the air-cathode for rechargeable Zn-air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm −2 and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. CoFe@HNSs exhibited bifunctional oxygen electrocatalytic activity, and exhibit a high-power density of 131.3 mW cm −2 and long-term stability over 140 h. Unique Co, Fe codoped holey carbon nanosheets with high surface area and abundant bimetal single atoms (CoFe@HNSs) exhibited remarkable bifunctional oxygen electrocatalytic activity (0.704 V) with very positive half-wave potential (0.897 V) for the ORR and small potential (1.601 V) to drive 10 mA cm for the OER, outperforming commercial Pt/C and IrO , respectively. Furthermore, as the air-cathode for rechargeable Zn-air batteries, the CoFe@HNS based device exhibits a high-power density of 131.3 mW cm and long-term stability over 140 h, indicating the attractive potential of CoFe@HNSs applied in energy storage and conversion. |
| Author | Zhang, Xueting Ma, Fei-Xiang Tan, Yuanbo Qin, Ke Zhu, Zhenye Zhang, Jiaheng |
| AuthorAffiliation | Shenzhen Key Laboratory of Flexible Printed Electronics Technology, School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen) Department of Mechanical Engineering, City University of Hong Kong Kowloon School of Materials Science and Engineering, Harbin Institute of Technology Shenzhen |
| AuthorAffiliation_xml | – name: Shenzhen Key Laboratory of Flexible Printed Electronics Technology, School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen) – name: School of Materials Science and Engineering, Harbin Institute of Technology Shenzhen – name: Department of Mechanical Engineering, City University of Hong Kong Kowloon |
| Author_xml | – sequence: 1 givenname: Xueting surname: Zhang fullname: Zhang, Xueting – sequence: 2 givenname: Zhenye surname: Zhu fullname: Zhu, Zhenye – sequence: 3 givenname: Yuanbo surname: Tan fullname: Tan, Yuanbo – sequence: 4 givenname: Ke surname: Qin fullname: Qin, Ke – sequence: 5 givenname: Fei-Xiang surname: Ma fullname: Ma, Fei-Xiang – sequence: 6 givenname: Jiaheng surname: Zhang fullname: Zhang, Jiaheng |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33507178$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Bimetals Carbon Cobalt Electrocatalysts energy Energy storage Iron Metal air batteries Nanosheets oxygen Rechargeable batteries surface area Zinc-oxygen batteries |
| Title | Co, Fe codoped holey carbon nanosheets as bifunctional oxygen electrocatalysts for rechargeable Zn-air batteries |
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