Effect of the necking phenomenon on the optical properties of soot particles
Fractal-like aggregates are commonly modeled as assemblies of spheres positioned in point contact only. The necking phenomenon is usually neglected. Such an approach has some advantages, e.g. faster light scattering simulation programs can be used, however, it may result in many additional errors an...
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| Published in | Journal of quantitative spectroscopy & radiative transfer Vol. 141; pp. 40 - 48 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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01.07.2014
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| Abstract | Fractal-like aggregates are commonly modeled as assemblies of spheres positioned in point contact only. The necking phenomenon is usually neglected. Such an approach has some advantages, e.g. faster light scattering simulation programs can be used, however, it may result in many additional errors and inaccuracies. In our study we try to approximate them and select the most suitable connection model. In our work we focus on the impact of the necking phenomenon on the optical properties of two and five monodisperse soot particles. The results show that small connections can be neglected. Different connection types (the cylindrical, the linear and the quadratic connector) can be used interchangeably, therefore, we recommend the most basic one (i.e. the cylindrical connector). Additionally, when particles are not positioned in point contact (they tend to overlap) this phenomenon should not be omitted due to its impact on the resulting scattering cross sections.
•We examine the impact of connectors on the optical properties of soot particles.•Small connections between primary particles can be neglected.•Different connection types can be used interchangeably. |
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| AbstractList | Fractal-like aggregates are commonly modeled as assemblies of spheres positioned in point contact only. The necking phenomenon is usually neglected. Such an approach has some advantages, e.g. faster light scattering simulation programs can be used, however, it may result in many additional errors and inaccuracies. In our study we try to approximate them and select the most suitable connection model. In our work we focus on the impact of the necking phenomenon on the optical properties of two and five monodisperse soot particles. The results show that small connections can be neglected. Different connection types (the cylindrical, the linear and the quadratic connector) can be used interchangeably, therefore, we recommend the most basic one (i.e. the cylindrical connector). Additionally, when particles are not positioned in point contact (they tend to overlap) this phenomenon should not be omitted due to its impact on the resulting scattering cross sections.
•We examine the impact of connectors on the optical properties of soot particles.•Small connections between primary particles can be neglected.•Different connection types can be used interchangeably. Fractal-like aggregates are commonly modeled as assemblies of spheres positioned in point contact only. The necking phenomenon is usually neglected. Such an approach has some advantages, e.g. faster light scattering simulation programs can be used, however, it may result in many additional errors and inaccuracies. In our study we try to approximate them and select the most suitable connection model. In our work we focus on the impact of the necking phenomenon on the optical properties of two and five monodisperse soot particles. The results show that small connections can be neglected. Different connection types (the cylindrical, the linear and the quadratic connector) can be used interchangeably, therefore, we recommend the most basic one (i.e. the cylindrical connector). Additionally, when particles are not positioned in point contact (they tend to overlap) this phenomenon should not be omitted due to its impact on the resulting scattering cross sections. |
| Author | Skorupski, Krzysztof Mroczka, Janusz |
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| Cites_doi | 10.1016/j.measurement.2013.04.040 10.1103/PhysRevE.82.036703 10.1006/jcis.1997.5046 10.1016/S0021-8502(99)00026-9 10.1364/JOSAA.11.001491 10.1080/02786820117868 10.1007/s00340-011-4781-z 10.1016/j.jqsrt.2007.01.034 10.1016/j.physa.2014.02.072 10.1016/0022-4073(94)90142-2 10.1016/S0022-4073(99)00047-3 10.1016/j.jqsrt.2012.12.014 10.1007/s11051-004-2161-x 10.1016/j.jqsrt.2011.02.019 10.1080/02786820500421521 10.1016/S0010-2180(96)00170-8 10.1103/PhysRevLett.52.1433 10.5194/acp-8-6469-2008 10.1098/rspa.1989.0042 10.1029/2005GL024461 10.1006/jcis.2000.7027 10.1016/S0021-8502(00)00097-5 |
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| SubjectTerms | Approximation Carbon black Connectors Fractal aggregates Joints Light scattering Necking Optical properties Point contact Scattering cross sections Soot |
| Title | Effect of the necking phenomenon on the optical properties of soot particles |
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