Understanding the fouling/scaling resistance of superhydrophobic/omniphobic membranes in membrane distillation

Membrane distillation has shown great promises in desalinating various water streams. Significant progresses have been made in the past decades owing to the development of advanced membrane materials, such as superhydrophobic and omniphobic membranes. However, fouling and scaling remains a critical...

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Published inDesalination Vol. 499; p. 114864
Main Authors Liu, Li, Xiao, Zechun, Liu, Yongjie, Li, Xuemei, Yin, Huabing, Volkov, Alexey, He, Tao
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.02.2021
Subjects
Fouling/scaling resistant
Membrane distillation
Omniphobic
Slip
Superhydrophobic
Superhydrophobic
Membrane distillation
Fouling/scaling resistant
Omniphobic
Slip
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Abstract Membrane distillation has shown great promises in desalinating various water streams. Significant progresses have been made in the past decades owing to the development of advanced membrane materials, such as superhydrophobic and omniphobic membranes. However, fouling and scaling remains a critical issue for stable operation. This account summarizes contemporary theories in fouling and scaling formation and their limitations in explaining the fouling resistance of superhydrophobic and omniphobic membranes. A new understanding is proposed based on hydrodynamics where non-slip boundary conditions play a critical role. By distinguishing a pinned and suspended wetting state, it is suggested that a superhydrophobic or omniphobic membrane correlates to a suspended wetting state, consequently a slip surface leading to scaling/fouling resistance. A new framework for analyzing the fouling/scaling behavior of MD membrane is provided to identify the wetting and hydrodynamic character of the membrane. A novel concept of treating the highly saline waste streams is suggested to cover membrane synthesis, module design and process optimization. The present work will be of interest to scientists and engineers searching for solutions to the MD fouling issues. •New understanding of fouling/scaling resistance of superhydrophobic membranes was proposed.•Water-air-solid interface with suspended wetting incurs potential slippage.•Sustaining suspended wetting and slippage is critical for antifouling and antiscaling.•Conventional thermodynamic theories for fouling/scaling are special case of non-slip.
AbstractList Membrane distillation has shown great promises in desalinating various water streams. Significant progresses have been made in the past decades owing to the development of advanced membrane materials, such as superhydrophobic and omniphobic membranes. However, fouling and scaling remains a critical issue for stable operation. This account summarizes contemporary theories in fouling and scaling formation and their limitations in explaining the fouling resistance of superhydrophobic and omniphobic membranes. A new understanding is proposed based on hydrodynamics where non-slip boundary conditions play a critical role. By distinguishing a pinned and suspended wetting state, it is suggested that a superhydrophobic or omniphobic membrane correlates to a suspended wetting state, consequently a slip surface leading to scaling/fouling resistance. A new framework for analyzing the fouling/scaling behavior of MD membrane is provided to identify the wetting and hydrodynamic character of the membrane. A novel concept of treating the highly saline waste streams is suggested to cover membrane synthesis, module design and process optimization. The present work will be of interest to scientists and engineers searching for solutions to the MD fouling issues. •New understanding of fouling/scaling resistance of superhydrophobic membranes was proposed.•Water-air-solid interface with suspended wetting incurs potential slippage.•Sustaining suspended wetting and slippage is critical for antifouling and antiscaling.•Conventional thermodynamic theories for fouling/scaling are special case of non-slip.
ArticleNumber 114864
Author Volkov, Alexey
Yin, Huabing
Liu, Li
He, Tao
Xiao, Zechun
Liu, Yongjie
Li, Xuemei
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  givenname: Li
  surname: Liu
  fullname: Liu, Li
  organization: Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, China
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  fullname: Xiao, Zechun
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  givenname: Tao
  surname: He
  fullname: He, Tao
  email: het@sari.ac.cn
  organization: Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, China
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Membrane distillation
Fouling/scaling resistant
Omniphobic
Slip
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  issue: 1–3
  year: 2005
  ident: 10.1016/j.desal.2020.114864_bb0675
  article-title: Modeling concentration polarization in reverse osmosis processes
  publication-title: Desalination
  doi: 10.1016/j.desal.2005.05.017
– volume: 556
  start-page: 352
  year: 2018
  ident: 10.1016/j.desal.2020.114864_bb0390
  article-title: Comparison of fouling propensity between reverse osmosis, forward osmosis, and membrane distillation
  publication-title: J. Membr. Sci.
  doi: 10.1016/j.memsci.2018.03.065
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Snippet Membrane distillation has shown great promises in desalinating various water streams. Significant progresses have been made in the past decades owing to the...
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elsevier
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StartPage 114864
SubjectTerms Fouling/scaling resistant
Membrane distillation
Omniphobic
Slip
Superhydrophobic
Title Understanding the fouling/scaling resistance of superhydrophobic/omniphobic membranes in membrane distillation
URI https://dx.doi.org/10.1016/j.desal.2020.114864
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