Intensifying Hydrogen Spillover for Boosting Electrocatalytic Hydrogen Evolution Reaction

Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak h...

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Published inChemical record Vol. 23; no. 3; pp. e202200244 - n/a
Main Authors Xu, Hui, Li, Junru, Chu, Xianxu
Format Journal Article
LanguageEnglish
Published United States Wiley Subscription Services, Inc 01.03.2023
Subjects
Adsorption
Catalysis
Catalysts
Electrocatalysis
Electrocatalysts
Electrolysis
Energy barrier
Hydrogen
Hydrogen evolution reaction
Hydrogen evolution reactions
Hydrogen production
Hydrogen spillover
Metal-support
Reaction mechanisms
Electrocatalysis
Hydrogen evolution reaction
Metal-support
Energy barrier
Hydrogen spillover
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Abstract Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak hydrogen adsorption on support. By taking advantageous merits of efficient hydrogen transfer, hydrogen spillover‐based binary catalysts have been widely investigated, which paves a new way for boosting the development of hydrogen production by water electrolysis. In this paper, we summarize the recent progress of this interesting field by focusing on the advanced strategies for intensifying the hydrogen spillover towards HER. In addition, the challenging issues and some perspective insights in the future development of hydrogen spillover‐based electrocatalysts are also systematically discussed. This review has summarized the recent findings achieved in hydrogen spillover‐based electrocatalysts for boosting HER by highlighting the definition of hydrogen spillover and manifesting the modification strategies for designing them to better suit the application demand in the near future.
AbstractList Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak hydrogen adsorption on support. By taking advantageous merits of efficient hydrogen transfer, hydrogen spillover‐based binary catalysts have been widely investigated, which paves a new way for boosting the development of hydrogen production by water electrolysis. In this paper, we summarize the recent progress of this interesting field by focusing on the advanced strategies for intensifying the hydrogen spillover towards HER. In addition, the challenging issues and some perspective insights in the future development of hydrogen spillover‐based electrocatalysts are also systematically discussed.
Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak hydrogen adsorption on support. By taking advantageous merits of efficient hydrogen transfer, hydrogen spillover-based binary catalysts have been widely investigated, which paves a new way for boosting the development of hydrogen production by water electrolysis. In this paper, we summarize the recent progress of this interesting field by focusing on the advanced strategies for intensifying the hydrogen spillover towards HER. In addition, the challenging issues and some perspective insights in the future development of hydrogen spillover-based electrocatalysts are also systematically discussed.Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak hydrogen adsorption on support. By taking advantageous merits of efficient hydrogen transfer, hydrogen spillover-based binary catalysts have been widely investigated, which paves a new way for boosting the development of hydrogen production by water electrolysis. In this paper, we summarize the recent progress of this interesting field by focusing on the advanced strategies for intensifying the hydrogen spillover towards HER. In addition, the challenging issues and some perspective insights in the future development of hydrogen spillover-based electrocatalysts are also systematically discussed.
Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their distinct reaction mechanism and beneficial terms for simultaneously weakening the strong hydrogen adsorption on metal and strengthening the weak hydrogen adsorption on support. By taking advantageous merits of efficient hydrogen transfer, hydrogen spillover‐based binary catalysts have been widely investigated, which paves a new way for boosting the development of hydrogen production by water electrolysis. In this paper, we summarize the recent progress of this interesting field by focusing on the advanced strategies for intensifying the hydrogen spillover towards HER. In addition, the challenging issues and some perspective insights in the future development of hydrogen spillover‐based electrocatalysts are also systematically discussed. This review has summarized the recent findings achieved in hydrogen spillover‐based electrocatalysts for boosting HER by highlighting the definition of hydrogen spillover and manifesting the modification strategies for designing them to better suit the application demand in the near future.
Author Xu, Hui
Chu, Xianxu
Li, Junru
Author_xml – sequence: 1
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  orcidid: 0000-0002-1744-4180
  surname: Xu
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  givenname: Junru
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  fullname: Li, Junru
  organization: Shangqiu Normal University
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  givenname: Xianxu
  surname: Chu
  fullname: Chu, Xianxu
  email: xxchu13633@163.com
  organization: Soochow University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/36482015$$D View this record in MEDLINE/PubMed
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Keywords Electrocatalysis
Hydrogen evolution reaction
Metal-support
Energy barrier
Hydrogen spillover
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Snippet Hydrogen spillover has attracted increasing interests in the field of electrocatalytic hydrogen evolution reaction (HER) in recent years because of their...
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StartPage e202200244
SubjectTerms Adsorption
Catalysis
Catalysts
Electrocatalysis
Electrocatalysts
Electrolysis
Energy barrier
Hydrogen
Hydrogen evolution reaction
Hydrogen evolution reactions
Hydrogen production
Hydrogen spillover
Metal-support
Reaction mechanisms
Title Intensifying Hydrogen Spillover for Boosting Electrocatalytic Hydrogen Evolution Reaction
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Ftcr.202200244
https://www.ncbi.nlm.nih.gov/pubmed/36482015
https://www.proquest.com/docview/2785210889
https://www.proquest.com/docview/2753310954
Volume 23
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