Effect of contaminants on mass transfer coefficients in bubble column and airlift contactors
In this work, the effects of surface-active contaminants on mass transfer coefficients k L a and k L were studied in two different bubble contactors. The oxygen transfer coefficient, k L , was obtained from the volumetric oxygen transfer coefficient, k L a, since the specific interfacial area, a, co...
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Published in | Chemical engineering science Vol. 58; no. 8; pp. 1431 - 1440 |
---|---|
Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
Oxford
Elsevier Ltd
01.04.2003
Elsevier |
Subjects | |
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Abstract | In this work, the effects of surface-active contaminants on mass transfer coefficients
k
L
a and
k
L
were studied in two different bubble contactors. The oxygen transfer coefficient,
k
L
, was obtained from the volumetric oxygen transfer coefficient,
k
L
a, since the specific interfacial area,
a, could be determined from the fractional gas holdup,
ε, and the average bubble diameter,
d
32. Water at different heights and antifoam solutions of 0.5–
100
ppm
were used as working media, under varying gas sparging conditions, in small-scale bubble column and rectangular airlift contactors of 6.7 and
0.85×10
−3
m
3
capacity, respectively. Both the antifoam concentration and the bubble residence time were shown to control
k
L
a and
k
L
values over a span of almost 400%. A theoretical interpretation is proposed based on modelling the kinetics of single bubble contamination, followed by sudden surface transition from mobile to rigid condition, in accordance with the stagnant cap model. Model results match experimental
k
L
data within ±30%. |
---|---|
AbstractList | In this work, the effects of surface-active contaminants on mass transfer coefficients
k
L
a and
k
L
were studied in two different bubble contactors. The oxygen transfer coefficient,
k
L
, was obtained from the volumetric oxygen transfer coefficient,
k
L
a, since the specific interfacial area,
a, could be determined from the fractional gas holdup,
ε, and the average bubble diameter,
d
32. Water at different heights and antifoam solutions of 0.5–
100
ppm
were used as working media, under varying gas sparging conditions, in small-scale bubble column and rectangular airlift contactors of 6.7 and
0.85×10
−3
m
3
capacity, respectively. Both the antifoam concentration and the bubble residence time were shown to control
k
L
a and
k
L
values over a span of almost 400%. A theoretical interpretation is proposed based on modelling the kinetics of single bubble contamination, followed by sudden surface transition from mobile to rigid condition, in accordance with the stagnant cap model. Model results match experimental
k
L
data within ±30%. In this work, the effects of surface-active contaminants on mass transfer coefficients k(subL)a and k(subL) were studied in two different bubble contactors. The oxygen transfer coefficient, k(subL), was obtained from the volumetric oxygen transfer coefficient, k(subL)a, since the specific interfacial area, a, could be determined from the fractional gas holdup, epsilon, and the average bubble diameter, d(sub32). Water at different heights and antifoam solutions of 0.5-100 ppm were used as working media, under varying gas sparging conditions, in small-scale bubble column and rectangular airlift contactors of 6.7 and 0.85 x 10(super-3) m(super3) capacity, respectively. Both the antifoam concentration and the bubble residence time were shown to control k(subL)a and k(subL) values over a span of almost 400%. A theoretical interpretation is proposed based on modelling the kinetics of single bubble contamination, followed by sudden surface transition from mobile to rigid condition, in accordance with the stagnant cap model. Model results match experimental k(subL) data within + or - 30%. |
Author | Orvalho, S.C.P Reis, A Alves, S.S Vasconcelos, J.M.T Rodrigues, J.M.L Mendes, R.L |
Author_xml | – sequence: 1 givenname: J.M.T surname: Vasconcelos fullname: Vasconcelos, J.M.T organization: Centro de Eng. Biologica e Quimica, Department of Chemical Engineering, Instituto Superior Técnico, Lisboa 1049-001, Portugal – sequence: 2 givenname: J.M.L surname: Rodrigues fullname: Rodrigues, J.M.L organization: Centro de Eng. Biologica e Quimica, Department of Chemical Engineering, Instituto Superior Técnico, Lisboa 1049-001, Portugal – sequence: 3 givenname: S.C.P surname: Orvalho fullname: Orvalho, S.C.P organization: Centro de Eng. Biologica e Quimica, Department of Chemical Engineering, Instituto Superior Técnico, Lisboa 1049-001, Portugal – sequence: 4 givenname: S.S surname: Alves fullname: Alves, S.S email: salves@alfa.ist.utl.pt organization: Centro de Eng. Biologica e Quimica, Department of Chemical Engineering, Instituto Superior Técnico, Lisboa 1049-001, Portugal – sequence: 5 givenname: R.L surname: Mendes fullname: Mendes, R.L organization: Dep. Energias Renováveis, Instituto Nacional de Engenharia e Tecnologia Industrial, Edificio G, Lisboa 1649-038, Portugal – sequence: 6 givenname: A surname: Reis fullname: Reis, A organization: Dep. Energias Renováveis, Instituto Nacional de Engenharia e Tecnologia Industrial, Edificio G, Lisboa 1649-038, Portugal |
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Keywords | Bubble Surfactant Mass transfer Interface Airlift Bubble column Gas liquid Airlift reactor Mass transfer coefficient Theoretical study Oxygen transfer Volumetric mass transfer coefficient Experimental study Modeling |
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k
L
a and
k
L
were studied in two different bubble contactors. The... In this work, the effects of surface-active contaminants on mass transfer coefficients k(subL)a and k(subL) were studied in two different bubble contactors.... |
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SubjectTerms | Airlift Applied sciences Bubble Bubble column Chemical engineering Exact sciences and technology Interface Mass transfer Reactors Surfactant |
Title | Effect of contaminants on mass transfer coefficients in bubble column and airlift contactors |
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