Effects of airborne contaminant exposure on the physical properties and filtration performance of activated, impregnated carbon
The effects of airborne contaminant exposure in humid air on the physical properties and filtration capabilities of a copper/zinc/molybdenum impregnated carbon were investigated. The impregnated carbon was exposed individually to CO2, NH3 and NO2 in humid air, then evaluated for changes in metal spe...
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Published in | Carbon (New York) Vol. 48; no. 9; pp. 2634 - 2643 |
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Main Authors | , |
Format | Journal Article |
Language | English |
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01.08.2010
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Abstract | The effects of airborne contaminant exposure in humid air on the physical properties and filtration capabilities of a copper/zinc/molybdenum impregnated carbon were investigated. The impregnated carbon was exposed individually to CO2, NH3 and NO2 in humid air, then evaluated for changes in metal speciation, metal distribution, porosity and water-uptake. The exposed impregnated carbon was further evaluated for changes in its ability to remove SO2 and cyclohexane from air streams. Exposure to CO2 did not impact the physical properties of the impregnated carbon, with changes in filtration performance were not evident. NH3 exposure resulted in the formation of metal amine complexes, which led to a migration of impregnants from within the pores of the carbon granule to the external surface. NH3 exposure increased SO2 filtration while decreasing cyclohexane filtration. The decrease in cyclohexane filtration was attributed to an increase in water uptake and a decrease in porosity. NO2 exposure significantly decreased the porosity of the carbon substrate while increasing the amount of surface oxygen. The increased surface oxygen greatly increased water uptake. NO2 exposure greatly reduced the SO2 breakthrough time and the ability of the material to remove cyclohexane. |
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AbstractList | The effects of airborne contaminant exposure in humid air on the physical properties and filtration capabilities of a copper/zinc/molybdenum impregnated carbon were investigated. The impregnated carbon was exposed individually to CO2, NH3 and NO2 in humid air, then evaluated for changes in metal speciation, metal distribution, porosity and water-uptake. The exposed impregnated carbon was further evaluated for changes in its ability to remove SO2 and cyclohexane from air streams. Exposure to CO2 did not impact the physical properties of the impregnated carbon, with changes in filtration performance were not evident. NH3 exposure resulted in the formation of metal amine complexes, which led to a migration of impregnants from within the pores of the carbon granule to the external surface. NH3 exposure increased SO2 filtration while decreasing cyclohexane filtration. The decrease in cyclohexane filtration was attributed to an increase in water uptake and a decrease in porosity. NO2 exposure significantly decreased the porosity of the carbon substrate while increasing the amount of surface oxygen. The increased surface oxygen greatly increased water uptake. NO2 exposure greatly reduced the SO2 breakthrough time and the ability of the material to remove cyclohexane. The effects of airborne contaminant exposure in humid air on the physical properties and filtration capabilities of a copper/zinc/molybdenum impregnated carbon were investigated. The impregnated carbon was exposed individually to CO sub(2), NH sub(3) and NO sub(2) in humid air, then evaluated for changes in metal speciation, metal distribution, porosity and water-uptake. The exposed impregnated carbon was further evaluated for changes in its ability to remove SO sub(2) and cyclohexane from air streams. Exposure to CO sub(2) did not impact the physical properties of the impregnated carbon, with changes in filtration performance were not evident. NH sub(3) exposure resulted in the formation of metal amine complexes, which led to a migration of impregnants from within the pores of the carbon granule to the external surface. NH sub(3) exposure increased SO sub(2) filtration while decreasing cyclohexane filtration. The decrease in cyclohexane filtration was attributed to an increase in water uptake and a decrease in porosity. NO sub(2) exposure significantly decreased the porosity of the carbon substrate while increasing the amount of surface oxygen. The increased surface oxygen greatly increased water uptake. NO sub(2) exposure greatly reduced the SO sub(2) breakthrough time and the ability of the material to remove cyclohexane. |
Author | Rossin, Joseph A. Maxwell, Amy H. |
Author_xml | – sequence: 1 givenname: Amy H. surname: Maxwell fullname: Maxwell, Amy H. organization: US Army ECBC, Aberdeen Proving Ground, MD 21010-5423, USA – sequence: 2 givenname: Joseph A. surname: Rossin fullname: Rossin, Joseph A. email: jarossin@guildassociates.com organization: Guild Associate, 5750 Shier-Rings Road, Dublin, OH 4301, USA |
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CitedBy_id | crossref_primary_10_1016_j_diamond_2020_108179 crossref_primary_10_1021_acs_iecr_6b02041 crossref_primary_10_1016_j_cej_2012_02_087 crossref_primary_10_1002_ange_201502155 crossref_primary_10_1021_ie200809r crossref_primary_10_1002_anie_201502155 |
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Keywords | Water Nitrogen oxide Oxygen Amines Filtration Porous materials Migration Metal complex Air Carbon Molybdenum Physical properties Substrates Zinc Ammonia Pore Transition elements Activated carbon Cyclohexane Distribution Porosity Copper Contaminant |
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StartPage | 2634 |
SubjectTerms | Adsorbents Carbon Chemistry Colloidal state and disperse state Contaminants Cross-disciplinary physics: materials science; rheology Cyclohexane Exact sciences and technology Filtration Fullerenes and related materials; diamonds, graphite General and physical chemistry Materials science Nitrogen dioxide Physical properties Physics Porosity Porous materials Specific materials Surface physical chemistry Zinc |
Title | Effects of airborne contaminant exposure on the physical properties and filtration performance of activated, impregnated carbon |
URI | https://dx.doi.org/10.1016/j.carbon.2010.03.069 https://search.proquest.com/docview/753754047 |
Volume | 48 |
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