An Unsteady Heterogeneous Mass Transfer Model for Gas Absorption Enhanced by Dispersed Third Phase Droplets
A model for one-dimensional unsteady heterogeneous mass transfer was developed based on Danck- werts＇ surface renewal theory in order to describe the mass transfer enhancement of absorption process for a slightly soluble gas in a gas-liquid-liquid system. The model accounts for the mass transfer res...
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| Published in | Chinese journal of chemical engineering Vol. 17; no. 4; pp. 602 - 607 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
2009
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| Abstract | A model for one-dimensional unsteady heterogeneous mass transfer was developed based on Danck- werts＇ surface renewal theory in order to describe the mass transfer enhancement of absorption process for a slightly soluble gas in a gas-liquid-liquid system. The model accounts for the mass transfer resistance within the dispersed phase and the effect of emulsion viscosity on mass transfer. An analytical solution for enhancement factor was obtained by Laplace domain transformation. The absorption rates of carbon dioxide in the dodecane-in-water and castor oil-in-water systems were measured in a thermostatic reactor, and the enhancement factors were calculated at different volume fractions of dispersed phase and stirrer speeds. The model predictions agree well with the experimental data. |
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| AbstractList | A model for one-dimensional unsteady heterogeneous mass transfer was developed based on Danck- werts＇ surface renewal theory in order to describe the mass transfer enhancement of absorption process for a slightly soluble gas in a gas-liquid-liquid system. The model accounts for the mass transfer resistance within the dispersed phase and the effect of emulsion viscosity on mass transfer. An analytical solution for enhancement factor was obtained by Laplace domain transformation. The absorption rates of carbon dioxide in the dodecane-in-water and castor oil-in-water systems were measured in a thermostatic reactor, and the enhancement factors were calculated at different volume fractions of dispersed phase and stirrer speeds. The model predictions agree well with the experimental data. A model for one-dimensional unsteady heterogeneous mass transfer was developed based on Danckwerts' surface renewal theory in order to describe the mass transfer enhancement of absorption process for a slightly soluble gas in a gas-liquid-liquid system. The model accounts for the mass transfer resistance within the dispersed phase and the effect of emulsion viscosity on mass transfer. An analytical solution for enhancement factor was obtained by Laplace domain transformation. The absorption rates of carbon dioxide in the dodecane-in-water and castor oil-in-water systems were measured in a thermostatic reactor, and the enhancement factors were calculated at different volume fractions of dispersed phase and stirrer speeds. The model predictions agree well with the experimental data. |
| Author | 沈树华 马友光 卢素敏 朱春英 |
| AuthorAffiliation | School of Chemical Engineering and Technology, State Key Laboratory of Chemical Engineering, Tianjin University, Tianjin 300072, China |
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| CitedBy_id | crossref_primary_10_1016_j_cjche_2017_01_010 crossref_primary_10_1021_acs_jced_3c00750 crossref_primary_10_1016_S1004_9541_13_60550_9 crossref_primary_10_1016_j_cep_2021_108547 crossref_primary_10_1016_j_applthermaleng_2016_02_030 crossref_primary_10_1016_j_cjche_2021_07_028 |
| Cites_doi | 10.1016/S0255-2701(02)00067-3 10.1002/aic.690010222 10.1016/0009-2509(80)80090-X 10.1016/0009-2509(94)00441-S 10.1016/S0009-2509(98)00251-6 10.1016/0009-2509(90)87089-B 10.1016/S0009-2509(97)00249-2 10.1016/S0009-2509(98)00104-3 10.1002/aic.690401005 10.1016/0009-2509(86)87066-X 10.1016/0009-2509(93)80237-K 10.1002/aic.690070420 10.1016/0300-9467(79)80104-5 10.1016/0009-2509(90)87003-B 10.1016/j.cej.2006.03.029 10.1016/0009-2509(95)00133-P 10.1002/bit.260350605 10.1021/je60052a018 10.1016/j.ces.2005.07.035 10.1016/S0009-2509(99)00491-1 |
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| SubjectTerms | absorption Carbon dioxide Chemical engineering Dispersion Droplets enhancement factor gas-liquid-liquid Mass transfer Mathematical models Natural gas Unsteady 中水系统 传质模型 吸收过程 增强因子 强化传质 拉普拉斯 表面重建 阻力模型 |
| Title | An Unsteady Heterogeneous Mass Transfer Model for Gas Absorption Enhanced by Dispersed Third Phase Droplets |
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