Measurement and interpretation of growth of binary droplets suspended in a water- n-propanol-nitrogen mixture by means of a piston-expansion-tube
We generate a cloud of monodisperse binary droplets in a piston-expansion- tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By Mie light scattering we measure the growth rate of the droplets in the radius range from 0.16 to 3 μm. We investigate the water- n-propanol sy...
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| Published in | International journal of heat and mass transfer Vol. 40; no. 14; pp. 3407 - 3417 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.09.1997
Elsevier |
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| Abstract | We generate a cloud of monodisperse binary droplets in a piston-expansion-
tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By Mie light scattering we measure the growth rate of the droplets in the radius range from 0.16 to 3 μm. We investigate the water-
n-propanol system because the growth behavior of the pure substances is very well known from previous studies. Our model calculations are an extension of a successful unary model to the binary case in which the droplet composition is treated as a variable. The calculation starts at the nucleus, passes through the transition zone about Knudsen number one and extends to the final droplet/vapor equilibrium which is only reached when vapor depletion and heat release are taken into account. The model is in good agreement with the experimental data. |
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| AbstractList | We generate a cloud of monodisperse binary droplets in a piston-expansion-tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By Mie light scattering we measure the growth rate of the droplets in the radius range from 0.16 to 3 mu m. We investigate the water-n-propanol system because the growth behavior of the pure substances is very well known from previous studies. Our model calculations are an extension of a successful unary model to the binary case in which the droplet composition is treated as a variable. The calculation starts at the nucleus, passes through the transition zone about Knudsen number one and extends to the final droplet/vapor equilibrium which is only reached when vapor depletion and heat release are taken into account. The model is in good agreement with the experimental data. We generate a cloud of monodisperse binary droplets in a piston-expansion- tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By Mie light scattering we measure the growth rate of the droplets in the radius range from 0.16 to 3 μm. We investigate the water- n-propanol system because the growth behavior of the pure substances is very well known from previous studies. Our model calculations are an extension of a successful unary model to the binary case in which the droplet composition is treated as a variable. The calculation starts at the nucleus, passes through the transition zone about Knudsen number one and extends to the final droplet/vapor equilibrium which is only reached when vapor depletion and heat release are taken into account. The model is in good agreement with the experimental data. |
| Author | Rodemann, T. Peters, F. |
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| Cites_doi | 10.1016/S0021-8502(05)80032-1 10.1016/0021-8502(88)90225-X 10.1209/0295-5075/29/2/004 10.1016/0017-9310(94)90100-7 10.1002/bbpc.19830871008 10.1063/1.472361 10.1515/zpch-1940-18616 10.1007/BF01002370 10.1063/1.467117 10.1016/0017-9310(93)90112-J 10.1063/1.450111 10.1016/0017-9310(84)90292-8 10.1016/0021-9797(92)90205-Z 10.1016/0021-8502(92)90367-5 10.1063/1.3253094 10.1002/bbpc.19830870411 10.1175/1520-0469(1970)027<1160:KOHGFA>2.0.CO;2 10.1080/02786829308959645 10.1002/aic.690120119 10.1016/S0021-8502(05)80011-4 10.1080/02786828608959089 10.1021/je60014a011 10.1063/1.469823 10.1016/0017-9310(95)00089-R |
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| Keywords | Water Aerosols Monodispersed particle Models Propanol Nitrogen Experimental study Droplet Supersaturated steam |
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| References_xml | – year: 1991 ident: BIB29 publication-title: VDI-Wärmeatlas – volume: 53 start-page: 39 year: 1973 end-page: 56 ident: BIB7 article-title: Verhalten von Dämpfen löslicher Zweistoffgemische bei publication-title: Expansion in Überschalldüsen—Tropfenkoaleszenz in einer Potentialwirbelströmung contributor: fullname: Kaser – year: 1980 ident: BIB32 article-title: Microphysics of Clouds and Precipitation contributor: fullname: Klett – volume: 1 start-page: 3 year: 1972 end-page: 34 ident: BIB27 article-title: Gaseous diffusion coefficients publication-title: Journal of Physical and Chemical Reference Data contributor: fullname: Mason – start-page: 111 year: 1992 end-page: 120 ident: BIB25 article-title: Homogeneous nucleation rates of particle formation from vapor mixtures publication-title: Proceedings of 13th International Conference on Nucleation and Atmospheric Aerosols contributor: fullname: Viisanen – year: 1987 ident: BIB26 article-title: The Properties of Gases 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| Snippet | We generate a cloud of monodisperse binary droplets in a piston-expansion-
tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By... We generate a cloud of monodisperse binary droplets in a piston-expansion-tube by homogeneous nucleation and subsequent growth in a supersaturated vapor. By... |
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| SubjectTerms | Aerosols Alcohols Calculations Chemistry Colloidal state and disperse state Exact sciences and technology General and physical chemistry Light scattering Mathematical models Mixtures Nitrogen Nucleation Tubes (components) Vapors Water |
| Title | Measurement and interpretation of growth of binary droplets suspended in a water- n-propanol-nitrogen mixture by means of a piston-expansion-tube |
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