Effects of praseodymium doping on thermoelectric transport properties of CaMnO3 compound system
The rare earth Pr doped Ca1-xPrxMnO3 （x=0, 0.06, 0.08, 0.1, 0.12, and 0.14） compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited sin-gle phase composition within the experimental doping rang...
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| Published in | Journal of rare earths Vol. 31; no. 9; pp. 885 - 890 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.09.2013
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1002-0721 2509-4963 |
| DOI | 10.1016/S1002-0721(12)60374-3 |
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| Abstract | The rare earth Pr doped Ca1-xPrxMnO3 （x=0, 0.06, 0.08, 0.1, 0.12, and 0.14） compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited sin-gle phase composition within the experimental doping range, with condensed bulk microstructure and small porosities. The electrical resistivity was remarkably reduced for doped samples, on account of the enhanced carrier concentration;the absolute value of See-beck coefficient was deteriorated mainly due to enhanced electron carrier concentration. The electrical performances of the doped samples reflected by resistivity and Seebeck coefficient fluctuations were optimistically tuned, with an optimized power factor value of 0.342 mW/（m·K2） at 873 K for x=0.08 sample, which was very much higher comparing with that of the un-doped sample. The lattice thermal conduction was really confined, leading to distinctly repressed total thermal conductivity. The thermoelectric per-formance was noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound was favorably optimized with the maximum value 0.16 at 873 K. |
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| AbstractList | The rare earth Pr doped Ca1-xPrxMnO3 （x=0, 0.06, 0.08, 0.1, 0.12, and 0.14） compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited sin-gle phase composition within the experimental doping range, with condensed bulk microstructure and small porosities. The electrical resistivity was remarkably reduced for doped samples, on account of the enhanced carrier concentration;the absolute value of See-beck coefficient was deteriorated mainly due to enhanced electron carrier concentration. The electrical performances of the doped samples reflected by resistivity and Seebeck coefficient fluctuations were optimistically tuned, with an optimized power factor value of 0.342 mW/（m·K2） at 873 K for x=0.08 sample, which was very much higher comparing with that of the un-doped sample. The lattice thermal conduction was really confined, leading to distinctly repressed total thermal conductivity. The thermoelectric per-formance was noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound was favorably optimized with the maximum value 0.16 at 873 K. The rare earth Pr doped Ca1-xPrxMnO3 (x=0, 0.06, 0.08, 0.1, 0.12, and 0.14) compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited single phase composition within the experimental doping range, with condensed bulk microstructure and small porosities. The electrical resistivity was remarkably reduced for doped samples, on account of the enhanced carrier concentration; the absolute value of Seebeck coefficient was deteriorated mainly due to enhanced electron carrier concentration. The electrical performances of the doped samples reflected by resistivity and Seebeck coefficient fluctuations were optimistically tuned, with an optimized power factor value of 0.342 mW/(m.K2) at 873 K for x=0.08 sample, which was very much higher comparing with that of the un-doped sample. The lattice thermal conduction was really confined, leading to distinctly repressed total thermal conductivity. The thermoelectric performance was noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound was favorably optimized with the maximum value 0.16 at 873 K. The rare earth Pr doped Ca1−xPrxMnO3 (x=0, 0.06, 0.08, 0.1, 0.12, and 0.14) compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited single phase composition within the experimental doping range, with condensed bulk microstructure and small porosities. The electrical resistivity was remarkably reduced for doped samples, on account of the enhanced carrier concentration; the absolute value of Seebeck coefficient was deteriorated mainly due to enhanced electron carrier concentration. The electrical performances of the doped samples reflected by resistivity and Seebeck coefficient fluctuations were optimistically tuned, with an optimized power factor value of 0.342 mW/(m·K2) at 873 K for x=0.08 sample, which was very much higher comparing with that of the un-doped sample. The lattice thermal conduction was really confined, leading to distinctly repressed total thermal conductivity. The thermoelectric performance was noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound was favorably optimized with the maximum value 0.16 at 873 K. Pr doped Ca1−xPrxMnO3 (x=0, 0.06, 0.08, 0.1, 0.12, and 0.14) compound bulk samples are prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The thermoelectric performance is noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound is favorably optimized with the maximum value 0.16 at 873 K |
| Author | 张飞鹏 牛保成 张坤书 张忻 路清梅 张久兴 |
| AuthorAffiliation | Institute of Physics, Henan University of Urban Construction, Pingdingshan 467036, China Key Laboratory of Advanced Functional Materials, Chinese Ministry of Education, College of Materials Science and Engineering, Beijing University of Technology, Beijing 100124, China |
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| CitedBy_id | crossref_primary_10_1007_s10854_017_6982_7 crossref_primary_10_1111_jace_14898 crossref_primary_10_1080_01411594_2021_1995606 crossref_primary_10_1007_s10853_023_09034_w crossref_primary_10_1103_PhysRevB_96_064105 crossref_primary_10_1016_j_jmmm_2023_170750 crossref_primary_10_1016_j_jallcom_2019_07_188 crossref_primary_10_1016_S1002_0721_14_60498_1 crossref_primary_10_1016_j_matlet_2015_10_081 crossref_primary_10_1088_2053_1591_aaa802 crossref_primary_10_1016_j_jallcom_2024_175809 crossref_primary_10_1016_j_ijhydene_2015_09_017 crossref_primary_10_1016_j_jallcom_2020_154466 crossref_primary_10_3390_ma11101807 crossref_primary_10_1007_s11664_019_07386_1 crossref_primary_10_1016_j_jre_2018_06_011 crossref_primary_10_1590_1980_5373_mr_2020_0169 crossref_primary_10_1016_j_cej_2020_127364 |
| Cites_doi | 10.1016/j.ssc.2012.06.027 10.1016/j.jallcom.2011.01.032 10.1063/1.3475719 10.1016/j.materresbull.2010.01.023 10.1016/j.jeurceramsoc.2011.10.007 10.1126/science.1156446 10.1016/j.jallcom.2012.01.093 10.1016/j.tsf.2012.02.022 10.1016/j.solidstatesciences.2007.10.022 10.1063/1.3003065 10.1038/asiamat.2010.138 10.1016/S1002-0721(10)60504-2 10.1016/j.jallcom.2010.09.102 10.1016/S1002-0721(12)60072-6 10.1007/s00339-010-6081-6 10.1063/1.2920210 10.1016/j.physb.2012.01.083 |
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| Keywords | CaMnO3 compound thermoelectric properties Pr doping rare earths |
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| Notes | 11-2788/TF ZHANG Feipeng , NIU Baocheng , ZHANG Kunshu , ZHANG Xin , LU Qingmei, ZHANG Jiuxing （1. Institute of Physics, Henan University of Urban Construction, Pingdingshan 467036, China; 2. Key Laboratory of Advanced Functional Materials, Chinese Ministry of Education, College of Materials Science and Engineering, Beijing University of Technology, Beijing 100124, China） CaMnO3 compound; Pr doping; thermoelectric properties; rare earths The rare earth Pr doped Ca1-xPrxMnO3 （x=0, 0.06, 0.08, 0.1, 0.12, and 0.14） compound bulk samples were prepared to study the effect of Pr doping on thermoelectric transport properties of CaMnO3 compound system. The doped samples exhibited sin-gle phase composition within the experimental doping range, with condensed bulk microstructure and small porosities. The electrical resistivity was remarkably reduced for doped samples, on account of the enhanced carrier concentration;the absolute value of See-beck coefficient was deteriorated mainly due to enhanced electron carrier concentration. The electrical performances of the doped samples reflected by resistivity and Seebeck coefficient fluctuations were optimistically tuned, with an optimized power factor value of 0.342 mW/（m·K2） at 873 K for x=0.08 sample, which was very much higher comparing with that of the un-doped sample. The lattice thermal conduction was really confined, leading to distinctly repressed total thermal conductivity. The thermoelectric per-formance was noticeably improved by Pr doping and the dimensionless figure of merit ZT for the Ca0.92Pr0.08MnO3 compound was favorably optimized with the maximum value 0.16 at 873 K. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| Snippet | The rare earth Pr doped Ca1-xPrxMnO3 （x=0, 0.06, 0.08, 0.1, 0.12, and 0.14） compound bulk samples were prepared to study the effect of Pr doping on... The rare earth Pr doped Ca1−xPrxMnO3 (x=0, 0.06, 0.08, 0.1, 0.12, and 0.14) compound bulk samples were prepared to study the effect of Pr doping on... The rare earth Pr doped Ca1-xPrxMnO3 (x=0, 0.06, 0.08, 0.1, 0.12, and 0.14) compound bulk samples were prepared to study the effect of Pr doping on... |
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| SubjectTerms | Bulk sampling CaMnO3 compound Carrier density Coefficients Doping Electrical resistivity Pr doping Rare earth metals rare earths Seebeck系数 thermoelectric properties Thermoelectricity Transport properties 复合系统 学习效果 微观结构 样品准备 电输运性质 载流子浓度 镨掺杂 |
| Title | Effects of praseodymium doping on thermoelectric transport properties of CaMnO3 compound system |
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