Aggregation and breakup of colloidal particle aggregates in shear flow: A combined Monte Carlo - Stokesian dynamics approach

A method for the simulation of aggregation and breakup processes in colloidal particle suspensions is presented. The method combines a Monte Carlo algorithm to determine, on the basis of probabilistic considerations, the sequence of aggregation and breakup events, and a Discrete Element Method, buil...

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Published inPowder technology Vol. 388; pp. 357 - 370
Main Authors Frungieri, Graziano, Vanni, Marco
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 01.08.2021
Elsevier BV
Subjects
Agglomeration
Aggregates
Aggregation
Algorithms
Breakup
Colloidal suspensions
Colloiding
Discrete element method
Monte Carlo
Monte Carlo simulation
Shear flow
Shear stress
Shearing
Solid suspensions
technology
Aggregation
Colloidal suspensions
Breakup
Discrete element method
Monte Carlo
Shear flow
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Abstract A method for the simulation of aggregation and breakup processes in colloidal particle suspensions is presented. The method combines a Monte Carlo algorithm to determine, on the basis of probabilistic considerations, the sequence of aggregation and breakup events, and a Discrete Element Method, built in the framework of Stokesian dynamics and contact mechanics, to accurately reproduce them. Liquid-solid suspensions subject to a uniform shear stress are investigated. The model is seen to be able to reproduce the typical dynamic steady state which is observed in colloidal suspensions under severe shearing, in which the effects of aggregation and breakup balance each other. The structural properties of the aggregates and the dynamics of the aggregation and breakup phenomena are characterized in detail. Both fragmentation and erosion are seen to contribute to the breakup process, which is characterized by an exponent similar to the one reported in the literature for compact clusters. [Display omitted] •A method to study shear aggregation and breakup in colloidal suspensions is reported.•A Monte Carlo algorithm is used to sample an expected sequence of particle events.•A discrete element method reproduces in detail aggregation and breakup events.•An equilibrium between aggregation and breakup of colloidal clusters is reached.•Size and shape distribution of the aggregates are characterized in detail.
AbstractList A method for the simulation of aggregation and breakup processes in colloidal particle suspensions is presented. The method combines a Monte Carlo algorithm to determine, on the basis of probabilistic considerations, the sequence of aggregation and breakup events, and a Discrete Element Method, built in the framework of Stokesian dynamics and contact mechanics, to accurately reproduce them. Liquid-solid suspensions subject to a uniform shear stress are investigated. The model is seen to be able to reproduce the typical dynamic steady state which is observed in colloidal suspensions under severe shearing, in which the effects of aggregation and breakup balance each other. The structural properties of the aggregates and the dynamics of the aggregation and breakup phenomena are characterized in detail. Both fragmentation and erosion are seen to contribute to the breakup process, which is characterized by an exponent similar to the one reported in the literature for compact clusters. [Display omitted] •A method to study shear aggregation and breakup in colloidal suspensions is reported.•A Monte Carlo algorithm is used to sample an expected sequence of particle events.•A discrete element method reproduces in detail aggregation and breakup events.•An equilibrium between aggregation and breakup of colloidal clusters is reached.•Size and shape distribution of the aggregates are characterized in detail.
A method for the simulation of aggregation and breakup processes in colloidal particle suspensions is presented. The method combines a Monte Carlo algorithm to determine, on the basis of probabilistic considerations, the sequence of aggregation and breakup events, and a Discrete Element Method, built in the framework of Stokesian dynamics and contact mechanics, to accurately reproduce them. Liquid-solid suspensions subject to a uniform shear stress are investigated. The model is seen to be able to reproduce the typical dynamic steady state which is observed in colloidal suspensions under severe shearing, in which the effects of aggregation and breakup balance each other. The structural properties of the aggregates and the dynamics of the aggregation and breakup phenomena are characterized in detail. Both fragmentation and erosion are seen to contribute to the breakup process, which is characterized by an exponent similar to the one reported in the literature for compact clusters.
Author Frungieri, Graziano
Vanni, Marco
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  fullname: Frungieri, Graziano
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  givenname: Marco
  surname: Vanni
  fullname: Vanni, Marco
  email: marco.vanni@polito.it
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Keywords Aggregation
Colloidal suspensions
Breakup
Discrete element method
Monte Carlo
Shear flow
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Snippet A method for the simulation of aggregation and breakup processes in colloidal particle suspensions is presented. The method combines a Monte Carlo algorithm to...
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elsevier
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StartPage 357
SubjectTerms Agglomeration
Aggregates
Aggregation
Algorithms
Breakup
Colloidal suspensions
Colloiding
Discrete element method
Monte Carlo
Monte Carlo simulation
Shear flow
Shear stress
Shearing
Solid suspensions
technology
Title Aggregation and breakup of colloidal particle aggregates in shear flow: A combined Monte Carlo - Stokesian dynamics approach
URI https://dx.doi.org/10.1016/j.powtec.2021.04.076
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https://www.proquest.com/docview/2551913721
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