Solvent influence on the nonlinear optical properties of molecular systems in the presence of degenerate and non-degenerate four-wave mixing
The nonlinear optical properties are studied theoretically of a molecular system immersed in a thermal bath and interacting with a four-wave mixing signal. A methodology based on cumulant expansions to obtain the average in the Fourier components associated with the coherences and populations, calcu...
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Published in | Journal of modern optics Vol. 59; no. 1; pp. 71 - 82 |
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Main Authors | , |
Format | Journal Article |
Language | English |
Published |
Abingdon
Taylor & Francis Group
10.01.2012
Taylor & Francis Ltd |
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Abstract | The nonlinear optical properties are studied theoretically of a molecular system immersed in a thermal bath and interacting with a four-wave mixing signal. A methodology based on cumulant expansions to obtain the average in the Fourier components associated with the coherences and populations, calculated by the optical stochastic Bloch equations, is employed. The system properties are analyzed as a function of the frequency detuning of the high-intensity pump beam and parameterized by the frequency detuning of the probe beam, both with respect to the Bohr frequency of the system. The longitudinal and transversal relaxation times and the bath effects, modeled as white noise, are also included as parameters in the calculation. Different cases, with degenerate and non-degenerate optical frequencies are examined and compared, resulting in differences related to the maximum in the population pulsation effects. |
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AbstractList | The nonlinear optical properties are studied theoretically of a molecular system immersed in a thermal bath and interacting with a four-wave mixing signal. A methodology based on cumulant expansions to obtain the average in the Fourier components associated with the coherences and populations, calculated by the optical stochastic Bloch equations, is employed. The system properties are analyzed as a function of the frequency detuning of the high-intensity pump beam and parameterized by the frequency detuning of the probe beam, both with respect to the Bohr frequency of the system. The longitudinal and transversal relaxation times and the bath effects, modeled as white noise, are also included as parameters in the calculation. Different cases, with degenerate and non-degenerate optical frequencies are examined and compared, resulting in differences related to the maximum in the population pulsation effects. The nonlinear optical properties are studied theoretically of a molecular system immersed in a thermal bath and interacting with a four-wave mixing signal. A methodology based on cumulant expansions to obtain the average in the Fourier components associated with the coherences and populations, calculated by the optical stochastic Bloch equations, is employed. The system properties are analyzed as a function of the frequency detuning of the high-intensity pump beam and parameterized by the frequency detuning of the probe beam, both with respect to the Bohr frequency of the system. The longitudinal and transversal relaxation times and the bath effects, modeled as white noise, are also included as parameters in the calculation. Different cases, with degenerate and non-degenerate optical frequencies are examined and compared, resulting in differences related to the maximum in the population pulsation effects. [PUBLICATION ABSTRACT] |
Author | Paz, J.L. Mendoza-García, A. |
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Cites_doi | 10.1103/PhysRevA.32.1526 10.1088/0953-4075/28/19/021 10.1016/j.jms.2005.04.002 10.1103/PhysRevA.47.4185 10.1103/PhysRevLett.101.056802 10.1039/cs9831200453 10.1103/PhysRevLett.104.046803 10.1016/j.jqsrt.2010.08.008 10.1007/978-3-662-02452-2 10.1364/AOP.3.000001 10.1103/PhysRevA.38.4657 10.1016/j.jqsrt.2009.08.002 10.1103/PhysRevA.53.543 10.1006/jtbi.1993.1049 10.1016/S0375-9601(00)00082-7 10.1063/1.1808226 10.1063/1.448444 10.1021/jp810852c 10.1016/0375-9601(95)00081-D 10.1021/nl901101g 10.1142/S021797920905434X 10.1016/S0375-9601(96)00923-1 |
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SubjectTerms | Beams (radiation) Electric noise Four-wave mixing Frequencies Mathematical models nonlinear optical properties Nonlinearity Optical properties optical stochastic Bloch equation Populations Pulsation Relaxation time Solvents white noise |
Title | Solvent influence on the nonlinear optical properties of molecular systems in the presence of degenerate and non-degenerate four-wave mixing |
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