Green light-driven acetone gas sensor based on electrospinned CdS nanospheres/Co3O4 nanofibers hybrid for the detection of exhaled diabetes biomarker
[Display omitted] Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co3O4) nanof...
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| Published in | Journal of colloid and interface science Vol. 606; no. Pt 1; pp. 261 - 271 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.01.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co3O4) nanofibers/cadmium sulfide (CdS) nanospheres hybrid was synthesized by an electrospinning method combined with a hydrothermal method to detect acetone gas. By adjusting loading amount of CdS, the sensing performance of CdS/Co3O4 sensor for acetone at room temperature (25 °C) was greatly ameliorated. In particular, the response of CdS/Co3O4 to 50 ppm acetone gas increased by 25% under 520 nm green light, meanwhile, the response/recovery time was shortened to 5 s/4 s. This is attributed to the heterojunction formed between CdS and Co3O4 as well as the influence of light excitation on the carrier concentration of the surfaces. Meanwhile, the unique high-porosity fiber structure and the catalytic action of cobalt ions also play an essential role in improving the performance. Furthermore, practical diabetic breath was experimentally simulated and proved the potential of the sensor in the future application of disease-assisted diagnosis. |
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| AbstractList | Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co₃O₄) nanofibers/cadmium sulfide (CdS) nanospheres hybrid was synthesized by an electrospinning method combined with a hydrothermal method to detect acetone gas. By adjusting loading amount of CdS, the sensing performance of CdS/Co₃O₄ sensor for acetone at room temperature (25 °C) was greatly ameliorated. In particular, the response of CdS/Co₃O₄ to 50 ppm acetone gas increased by 25% under 520 nm green light, meanwhile, the response/recovery time was shortened to 5 s/4 s. This is attributed to the heterojunction formed between CdS and Co₃O₄ as well as the influence of light excitation on the carrier concentration of the surfaces. Meanwhile, the unique high-porosity fiber structure and the catalytic action of cobalt ions also play an essential role in improving the performance. Furthermore, practical diabetic breath was experimentally simulated and proved the potential of the sensor in the future application of disease-assisted diagnosis. Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co3O4) nanofibers/cadmium sulfide (CdS) nanospheres hybrid was synthesized by an electrospinning method combined with a hydrothermal method to detect acetone gas. By adjusting loading amount of CdS, the sensing performance of CdS/Co3O4 sensor for acetone at room temperature (25 °C) was greatly ameliorated. In particular, the response of CdS/Co3O4 to 50 ppm acetone gas increased by 25% under 520 nm green light, meanwhile, the response/recovery time was shortened to 5 s/4 s. This is attributed to the heterojunction formed between CdS and Co3O4 as well as the influence of light excitation on the carrier concentration of the surfaces. Meanwhile, the unique high-porosity fiber structure and the catalytic action of cobalt ions also play an essential role in improving the performance. Furthermore, practical diabetic breath was experimentally simulated and proved the potential of the sensor in the future application of disease-assisted diagnosis.Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co3O4) nanofibers/cadmium sulfide (CdS) nanospheres hybrid was synthesized by an electrospinning method combined with a hydrothermal method to detect acetone gas. By adjusting loading amount of CdS, the sensing performance of CdS/Co3O4 sensor for acetone at room temperature (25 °C) was greatly ameliorated. In particular, the response of CdS/Co3O4 to 50 ppm acetone gas increased by 25% under 520 nm green light, meanwhile, the response/recovery time was shortened to 5 s/4 s. This is attributed to the heterojunction formed between CdS and Co3O4 as well as the influence of light excitation on the carrier concentration of the surfaces. Meanwhile, the unique high-porosity fiber structure and the catalytic action of cobalt ions also play an essential role in improving the performance. Furthermore, practical diabetic breath was experimentally simulated and proved the potential of the sensor in the future application of disease-assisted diagnosis. [Display omitted] Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis of heterojunctions with special structures can effectively improve sensor performance. Herein, a cobalt oxide (Co3O4) nanofibers/cadmium sulfide (CdS) nanospheres hybrid was synthesized by an electrospinning method combined with a hydrothermal method to detect acetone gas. By adjusting loading amount of CdS, the sensing performance of CdS/Co3O4 sensor for acetone at room temperature (25 °C) was greatly ameliorated. In particular, the response of CdS/Co3O4 to 50 ppm acetone gas increased by 25% under 520 nm green light, meanwhile, the response/recovery time was shortened to 5 s/4 s. This is attributed to the heterojunction formed between CdS and Co3O4 as well as the influence of light excitation on the carrier concentration of the surfaces. Meanwhile, the unique high-porosity fiber structure and the catalytic action of cobalt ions also play an essential role in improving the performance. Furthermore, practical diabetic breath was experimentally simulated and proved the potential of the sensor in the future application of disease-assisted diagnosis. |
| Author | Zhang, Jianhua Li, Tingting Zhang, Dongzhi Guo, Jingyu Yu, Liandong |
| Author_xml | – sequence: 1 givenname: Jingyu surname: Guo fullname: Guo, Jingyu – sequence: 2 givenname: Dongzhi surname: Zhang fullname: Zhang, Dongzhi email: dzzhang@upc.edu.cn – sequence: 3 givenname: Tingting surname: Li fullname: Li, Tingting – sequence: 4 givenname: Jianhua surname: Zhang fullname: Zhang, Jianhua – sequence: 5 givenname: Liandong surname: Yu fullname: Yu, Liandong email: liandongyu@upc.edu.cn |
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| Keywords | Electrospinning CdS/Co3O4 nanocomposites Biomarker detection Acetone sensor Photo-excitation |
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Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable... Morphological and structural characteristics of semiconductors have a significant impact on their gas sensing characteristics. Reasonable design and synthesis... |
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| SubjectTerms | acetone Acetone sensor ambient temperature Biomarker detection biomarkers cadmium sulfide CdS/Co3O4 nanocomposites cobalt cobalt oxide diabetes Electrospinning green light hot water treatment nanofibers nanospheres Photo-excitation |
| Title | Green light-driven acetone gas sensor based on electrospinned CdS nanospheres/Co3O4 nanofibers hybrid for the detection of exhaled diabetes biomarker |
| URI | https://dx.doi.org/10.1016/j.jcis.2021.08.022 https://www.proquest.com/docview/2561490436 https://www.proquest.com/docview/2636753850 |
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