Inhibition of 5083 aluminium alloy and galvanised steel by lanthanide salts
Lanthanide salts are being considered as an environmentally friendly alternative to the classic systems based on chromates. The inhibitor behaviour of CeCl 3 has been studied for both AA5083 alloy and galvanised steel in aerated NaCl solutions. For AA5083, cerium appears as dispersed islands whilst...
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| Published in | Corrosion science Vol. 43; no. 1; pp. 157 - 170 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
2001
Elsevier Science |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lanthanide salts are being considered as an environmentally friendly alternative to the classic systems based on chromates. The inhibitor behaviour of CeCl
3 has been studied for both AA5083 alloy and galvanised steel in aerated NaCl solutions. For AA5083, cerium appears as dispersed islands whilst in the galvanised steel samples, it is stochastically dispersed onto the metallic surface, forming a film. These differences can be interpreted in terms of the distribution of cathodic areas for each material. In the case of AA5083, Al
6–(Mn,Fe,Cr) acts as permanent cathodic site whilst permanent cathodic sites do not exist in the galvanised steel. |
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| AbstractList | The use of rare earths has been proposed as non-contaminating alternatives to chromates for the process of anticorrosion treatments on metals. This paper presents the study of the inhibitor effect of CeCl(sub3) against the corrosion in seawater of galvanised steel and an aluminium-magnesium alloy (AA5083). Prior to testing, the microstructural characterisation of the two types of specimen was carried out by means of optical microscopy, scanning electron microscopy (SEM) and energy dispersive spectroscopy (EDS). The study of AA5083 revealed three intermetallic compounds distributed unevenly on the aluminium matrix, mainly composed of Al(sub6)-(Mn, Fe, Cr), Al-Mg and Al-(Si, Mg). After immersion in NaCl, a process of local corrosion was observed in the surrounding area of the Al(sub6)-(Mn, Fe, Cr) precipitates. The galvanised steel samples presented a voluminous layer of white corrosion products on the surface. Polarization curves for both metals showed a predominantly cathodic reaction. The corresponding curves for the two samples in NaCl solution with different amounts of CeCl(sub3) showed a decrease in the corrosion potential of the system. It was concluded that corrosion of AA5083 is inhibited by the precipitation of cerium compounds on the Al(sub6)-(Mn, Fe, Cr) intermetallics that act as permanent cathodes. For the galvanised steel, the formation of a continuous cerium-rich film was observed. (Abstract quotes from original text) Lanthanide salts are being considered as an environmentally friendly alternative to the classic systems based on chromates. The inhibitor behaviour of CeCl 3 has been studied for both AA5083 alloy and galvanised steel in aerated NaCl solutions. For AA5083, cerium appears as dispersed islands whilst in the galvanised steel samples, it is stochastically dispersed onto the metallic surface, forming a film. These differences can be interpreted in terms of the distribution of cathodic areas for each material. In the case of AA5083, Al 6–(Mn,Fe,Cr) acts as permanent cathodic site whilst permanent cathodic sites do not exist in the galvanised steel. |
| Author | Botana, F.J Arenas, M.A de Damborenea, J Bethencourt, M Marcos, M |
| Author_xml | – sequence: 1 givenname: M.A surname: Arenas fullname: Arenas, M.A organization: Departamento de Corrosión y Protección, Centro Nacional de Investigaciones Metalúrgicas (CENIM/CSIC), Avenida de Gregorio del Amo 8, E-28040 Madrid, Spain – sequence: 2 givenname: M surname: Bethencourt fullname: Bethencourt, M organization: Departamento de Ciencia de los Materiales e Ingenierı́a Metalúrgica y Quı́mica Inorgánica, Facultad de Ciencias del Mar, Universidad de Cádiz, Polı́gono Rı́o San Pedro s/n, Apto. 40, Puerto Real, 11510 Cádiz, Spain – sequence: 3 givenname: F.J surname: Botana fullname: Botana, F.J organization: Departamento de Ciencia de los Materiales e Ingenierı́a Metalúrgica y Quı́mica Inorgánica, Facultad de Ciencias del Mar, Universidad de Cádiz, Polı́gono Rı́o San Pedro s/n, Apto. 40, Puerto Real, 11510 Cádiz, Spain – sequence: 4 givenname: J surname: de Damborenea fullname: de Damborenea, J email: jdambo@fresno.csic.es organization: Departamento de Corrosión y Protección, Centro Nacional de Investigaciones Metalúrgicas (CENIM/CSIC), Avenida de Gregorio del Amo 8, E-28040 Madrid, Spain – sequence: 5 givenname: M surname: Marcos fullname: Marcos, M organization: Departamento Ingenieria Mecánica y Diseño Industrial, Universidad de Cádiz, Escuela Superior de Ingenierı́a, c/Chile s/n, 11003 Cádiz, Spain |
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| Keywords | Cerium salts Green inhibitor Aluminium alloy Corrosion Galvanised steel Aluminium base alloys Galvanized steel Salt corrosion Corrosion inhibition Steel Experimental study Corrosion protection Sodium chloride Corrosion inhibitor Lanthanide compound Chlorides Cerium chloride Cesium compound |
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| Snippet | Lanthanide salts are being considered as an environmentally friendly alternative to the classic systems based on chromates. The inhibitor behaviour of CeCl
3... The use of rare earths has been proposed as non-contaminating alternatives to chromates for the process of anticorrosion treatments on metals. This paper... |
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| SubjectTerms | Aluminium alloy Applied sciences Cerium salts Corrosion Corrosion tests Exact sciences and technology Galvanised steel Green inhibitor Metals. Metallurgy |
| Title | Inhibition of 5083 aluminium alloy and galvanised steel by lanthanide salts |
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