Three-dimensional conductive network constructed by in-situ preparation of sea urchin-like NiFe2O4 in expanded graphite for efficient microwave absorption
[Display omitted] Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap ca...
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| Published in | Journal of colloid and interface science Vol. 650; no. Pt A; pp. 710 - 718 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.11.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap cannot match microwave wavelength, and its single composition has less microwave loss. In this study, sea urchin-like NiFe2O4/EG composites are prepared in situ between expanded graphite layers by microwave treatment. The sea urchin-like NiFe2O4 grows between the expanded graphite to form a three-dimensional conductive network structure, which enhances conductive loss of composites and further increases the interlayer distance of EG. The extended interlayer distance promotes multiple reflections and scattering of electromagnetic waves in composites and improves dielectric properties. In addition, EG with a large specific surface area provides many active sites, further promoting interface and dipole polarization. Benefiting from synergistic effect of NiFe2O4 and EG, magnetic loss and dielectric loss of NiFe2O4/EG composites have been improved and impedance matching is further enhanced. The results indicate that the minimal reflection loss of NiFe2O4/EG-4 reaches −53.47 dB at 2.69 mm, and the effective absorption bandwidth reaches 2.97 GHz. In addition, based on the computer simulation technology results, NiFe2O4/EG can attenuate microwave energy under experimental conditions. This work provides a strategy for synthesizing carbon matrix composites with adjustable dielectric parameters and electromagnetic wave properties. |
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| AbstractList | Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap cannot match microwave wavelength, and its single composition has less microwave loss. In this study, sea urchin-like NiFe₂O₄/EG composites are prepared in situ between expanded graphite layers by microwave treatment. The sea urchin-like NiFe₂O₄ grows between the expanded graphite to form a three-dimensional conductive network structure, which enhances conductive loss of composites and further increases the interlayer distance of EG. The extended interlayer distance promotes multiple reflections and scattering of electromagnetic waves in composites and improves dielectric properties. In addition, EG with a large specific surface area provides many active sites, further promoting interface and dipole polarization. Benefiting from synergistic effect of NiFe₂O₄ and EG, magnetic loss and dielectric loss of NiFe₂O₄/EG composites have been improved and impedance matching is further enhanced. The results indicate that the minimal reflection loss of NiFe₂O₄/EG-4 reaches −53.47 dB at 2.69 mm, and the effective absorption bandwidth reaches 2.97 GHz. In addition, based on the computer simulation technology results, NiFe₂O₄/EG can attenuate microwave energy under experimental conditions. This work provides a strategy for synthesizing carbon matrix composites with adjustable dielectric parameters and electromagnetic wave properties. Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap cannot match microwave wavelength, and its single composition has less microwave loss. In this study, sea urchin-like NiFe2O4/EG composites are prepared in situ between expanded graphite layers by microwave treatment. The sea urchin-like NiFe2O4 grows between the expanded graphite to form a three-dimensional conductive network structure, which enhances conductive loss of composites and further increases the interlayer distance of EG. The extended interlayer distance promotes multiple reflections and scattering of electromagnetic waves in composites and improves dielectric properties. In addition, EG with a large specific surface area provides many active sites, further promoting interface and dipole polarization. Benefiting from synergistic effect of NiFe2O4 and EG, magnetic loss and dielectric loss of NiFe2O4/EG composites have been improved and impedance matching is further enhanced. The results indicate that the minimal reflection loss of NiFe2O4/EG-4 reaches -53.47 dB at 2.69 mm, and the effective absorption bandwidth reaches 2.97 GHz. In addition, based on the computer simulation technology results, NiFe2O4/EG can attenuate microwave energy under experimental conditions. This work provides a strategy for synthesizing carbon matrix composites with adjustable dielectric parameters and electromagnetic wave properties.Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap cannot match microwave wavelength, and its single composition has less microwave loss. In this study, sea urchin-like NiFe2O4/EG composites are prepared in situ between expanded graphite layers by microwave treatment. The sea urchin-like NiFe2O4 grows between the expanded graphite to form a three-dimensional conductive network structure, which enhances conductive loss of composites and further increases the interlayer distance of EG. The extended interlayer distance promotes multiple reflections and scattering of electromagnetic waves in composites and improves dielectric properties. In addition, EG with a large specific surface area provides many active sites, further promoting interface and dipole polarization. Benefiting from synergistic effect of NiFe2O4 and EG, magnetic loss and dielectric loss of NiFe2O4/EG composites have been improved and impedance matching is further enhanced. The results indicate that the minimal reflection loss of NiFe2O4/EG-4 reaches -53.47 dB at 2.69 mm, and the effective absorption bandwidth reaches 2.97 GHz. In addition, based on the computer simulation technology results, NiFe2O4/EG can attenuate microwave energy under experimental conditions. This work provides a strategy for synthesizing carbon matrix composites with adjustable dielectric parameters and electromagnetic wave properties. [Display omitted] Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low density, good electrical conductivity, and unique structure. However, its application is limited because the interlayer gap cannot match microwave wavelength, and its single composition has less microwave loss. In this study, sea urchin-like NiFe2O4/EG composites are prepared in situ between expanded graphite layers by microwave treatment. The sea urchin-like NiFe2O4 grows between the expanded graphite to form a three-dimensional conductive network structure, which enhances conductive loss of composites and further increases the interlayer distance of EG. The extended interlayer distance promotes multiple reflections and scattering of electromagnetic waves in composites and improves dielectric properties. In addition, EG with a large specific surface area provides many active sites, further promoting interface and dipole polarization. Benefiting from synergistic effect of NiFe2O4 and EG, magnetic loss and dielectric loss of NiFe2O4/EG composites have been improved and impedance matching is further enhanced. The results indicate that the minimal reflection loss of NiFe2O4/EG-4 reaches −53.47 dB at 2.69 mm, and the effective absorption bandwidth reaches 2.97 GHz. In addition, based on the computer simulation technology results, NiFe2O4/EG can attenuate microwave energy under experimental conditions. This work provides a strategy for synthesizing carbon matrix composites with adjustable dielectric parameters and electromagnetic wave properties. |
| Author | Wang, Yiqun Deng, Shuanglin Jiang, Jie He, Qinchuan Wu, Dan |
| Author_xml | – sequence: 1 givenname: Shuanglin surname: Deng fullname: Deng, Shuanglin organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China – sequence: 2 givenname: Jie surname: Jiang fullname: Jiang, Jie email: jiangjie13@cdut.edu.cn organization: School of Mechanical and Electrical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China – sequence: 3 givenname: Dan surname: Wu fullname: Wu, Dan organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China – sequence: 4 givenname: Qinchuan surname: He fullname: He, Qinchuan organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China – sequence: 5 givenname: Yiqun orcidid: 0000-0001-6145-1110 surname: Wang fullname: Wang, Yiqun email: wangyiqun17@cdut.edu.cn organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China |
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Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption... Expanded graphite (EG) is a modified conductive lamellar carbon that has been widely studied in the field of electromagnetic wave absorption due to its low... |
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| SubjectTerms | absorption computer simulation electrical conductivity electromagnetic radiation Electromagnetic wave absorption energy Expanded graphite graphene magnetism microwave treatment RCS simulation Sea urchin-like NiFe2O4 surface area synergism wavelengths |
| Title | Three-dimensional conductive network constructed by in-situ preparation of sea urchin-like NiFe2O4 in expanded graphite for efficient microwave absorption |
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