Iron, rhodium-codoped Ni2P nanosheets arrays supported on nickel foam as an efficient bifunctional electrocatalyst for overall water splitting
[Display omitted] •The Fe,Rh-Ni2P/NF were synthesized via hydrothermal treatment and sequential low-temperature phosphorization.•The unique nanosheets arrays effectively enriched the active sites with easy accessibility.•Fe,Rh-codoping had great effects on the electrocatalytic performances.•The elec...
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| Published in | Journal of colloid and interface science Vol. 605; pp. 888 - 896 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
01.01.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0021-9797 1095-7103 1095-7103 |
| DOI | 10.1016/j.jcis.2021.07.101 |
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| Abstract | [Display omitted]
•The Fe,Rh-Ni2P/NF were synthesized via hydrothermal treatment and sequential low-temperature phosphorization.•The unique nanosheets arrays effectively enriched the active sites with easy accessibility.•Fe,Rh-codoping had great effects on the electrocatalytic performances.•The electrocatalyst exhibited excellent OER, HER, and overall water splitting activity in the alkaline solutions.
To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional electrocatalysts towards oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). Herein, Fe,Rh-codoped Ni2P nanosheets arrays were in situ anchored on three-dimension (3D) Ni foam under hydrothermal condition and successive phosphorization, denoted as Fe,Rh-Ni2P/NF for simplicity. The unique nanosheets arrays effectively enriched the active sites with easy accessibility. By virtue of the unique sheet-like arrays and 3D porous conductive substrate, the prepared Fe,Rh-Ni2P/NF showed the low overpotentials of 226 mV at 30 mA cm−2 towards the OER and 73 mV at 10 mA cm−2 for the HER. Moreover, the electrocatalyst effectively worked as anode and cathode for overall water splitting system, showing a small voltage of 1.62 V to drive a current density of 10 mA cm−2. The present work provides alternative option for fabricating advanced catalysts in electrocatalysis and energy devices. |
|---|---|
| AbstractList | [Display omitted]
•The Fe,Rh-Ni2P/NF were synthesized via hydrothermal treatment and sequential low-temperature phosphorization.•The unique nanosheets arrays effectively enriched the active sites with easy accessibility.•Fe,Rh-codoping had great effects on the electrocatalytic performances.•The electrocatalyst exhibited excellent OER, HER, and overall water splitting activity in the alkaline solutions.
To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional electrocatalysts towards oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). Herein, Fe,Rh-codoped Ni2P nanosheets arrays were in situ anchored on three-dimension (3D) Ni foam under hydrothermal condition and successive phosphorization, denoted as Fe,Rh-Ni2P/NF for simplicity. The unique nanosheets arrays effectively enriched the active sites with easy accessibility. By virtue of the unique sheet-like arrays and 3D porous conductive substrate, the prepared Fe,Rh-Ni2P/NF showed the low overpotentials of 226 mV at 30 mA cm−2 towards the OER and 73 mV at 10 mA cm−2 for the HER. Moreover, the electrocatalyst effectively worked as anode and cathode for overall water splitting system, showing a small voltage of 1.62 V to drive a current density of 10 mA cm−2. The present work provides alternative option for fabricating advanced catalysts in electrocatalysis and energy devices. To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional electrocatalysts towards oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). Herein, Fe,Rh-codoped Ni₂P nanosheets arrays were in situ anchored on three-dimension (3D) Ni foam under hydrothermal condition and successive phosphorization, denoted as Fe,Rh-Ni₂P/NF for simplicity. The unique nanosheets arrays effectively enriched the active sites with easy accessibility. By virtue of the unique sheet-like arrays and 3D porous conductive substrate, the prepared Fe,Rh-Ni₂P/NF showed the low overpotentials of 226 mV at 30 mA cm⁻² towards the OER and 73 mV at 10 mA cm⁻² for the HER. Moreover, the electrocatalyst effectively worked as anode and cathode for overall water splitting system, showing a small voltage of 1.62 V to drive a current density of 10 mA cm⁻². The present work provides alternative option for fabricating advanced catalysts in electrocatalysis and energy devices. To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional electrocatalysts towards oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). Herein, Fe,Rh-codoped Ni2P nanosheets arrays were in situ anchored on three-dimension (3D) Ni foam under hydrothermal condition and successive phosphorization, denoted as Fe,Rh-Ni2P/NF for simplicity. The unique nanosheets arrays effectively enriched the active sites with easy accessibility. By virtue of the unique sheet-like arrays and 3D porous conductive substrate, the prepared Fe,Rh-Ni2P/NF showed the low overpotentials of 226 mV at 30 mA cm-2 towards the OER and 73 mV at 10 mA cm-2 for the HER. Moreover, the electrocatalyst effectively worked as anode and cathode for overall water splitting system, showing a small voltage of 1.62 V to drive a current density of 10 mA cm-2. The present work provides alternative option for fabricating advanced catalysts in electrocatalysis and energy devices.To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional electrocatalysts towards oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). Herein, Fe,Rh-codoped Ni2P nanosheets arrays were in situ anchored on three-dimension (3D) Ni foam under hydrothermal condition and successive phosphorization, denoted as Fe,Rh-Ni2P/NF for simplicity. The unique nanosheets arrays effectively enriched the active sites with easy accessibility. By virtue of the unique sheet-like arrays and 3D porous conductive substrate, the prepared Fe,Rh-Ni2P/NF showed the low overpotentials of 226 mV at 30 mA cm-2 towards the OER and 73 mV at 10 mA cm-2 for the HER. Moreover, the electrocatalyst effectively worked as anode and cathode for overall water splitting system, showing a small voltage of 1.62 V to drive a current density of 10 mA cm-2. The present work provides alternative option for fabricating advanced catalysts in electrocatalysis and energy devices. |
| Author | Chen, Meng-Ting Zhang, Lu Wang, Ai-Jun Jiao, Yang Duan, Jiao-Jiao Feng, Jiu-Ju Mei, Li-Ping |
| Author_xml | – sequence: 1 givenname: Meng-Ting surname: Chen fullname: Chen, Meng-Ting – sequence: 2 givenname: Jiao-Jiao surname: Duan fullname: Duan, Jiao-Jiao – sequence: 3 givenname: Jiu-Ju surname: Feng fullname: Feng, Jiu-Ju – sequence: 4 givenname: Li-Ping surname: Mei fullname: Mei, Li-Ping – sequence: 5 givenname: Yang surname: Jiao fullname: Jiao, Yang – sequence: 6 givenname: Lu surname: Zhang fullname: Zhang, Lu – sequence: 7 givenname: Ai-Jun surname: Wang fullname: Wang, Ai-Jun email: ajwang@zjnu.cn |
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| Copyright | 2021 Elsevier Inc. Copyright © 2021 Elsevier Inc. All rights reserved. |
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| Keywords | Bifunctional electrocatalyst Electrocatalysis Hydrogen evolution reaction Oxygen evolution reaction Overall water splitting |
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•The Fe,Rh-Ni2P/NF were synthesized via hydrothermal treatment and sequential low-temperature phosphorization.•The unique nanosheets arrays... To enhance the overall water splitting efficiency, it is widely attractive yet challenging to develop low price, abundance and efficient bifunctional... |
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| SubjectTerms | anodes Bifunctional electrocatalyst cathodes electric potential difference Electrocatalysis foams Hydrogen evolution reaction hydrogen production nanosheets nickel Overall water splitting Oxygen evolution reaction oxygen production prices |
| Title | Iron, rhodium-codoped Ni2P nanosheets arrays supported on nickel foam as an efficient bifunctional electrocatalyst for overall water splitting |
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