Mechanically strong, stretchable and self-healable silicone elastomers with designed dynamic networks for exceptional self-adhesion under harsh conditions
Silicone elastomers with wide-temperature stability and excellent mechanical flexibility have attracted considerable interest in both academic and industrial fields. However, the highly cross-linked networks cannot self-heal and usually show poor adhesion to other substrates, limiting their sustaina...
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| Published in | Advanced industrial and engineering polymer research Vol. 8; no. 3; pp. 422 - 432 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.07.2025
KeAi Communications Co., Ltd |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Silicone elastomers with wide-temperature stability and excellent mechanical flexibility have attracted considerable interest in both academic and industrial fields. However, the highly cross-linked networks cannot self-heal and usually show poor adhesion to other substrates, limiting their sustainable applications in emerging fields. Developing self-adhesive organosilicon elastomers with high mechanical strength, superior stretchability, and exceptional self-healing performance remains a significant challenge. Herein, we propose a facile method to synthesize self-adhesive organosilicon elastomers with high mechanical strength, flexibility, and self-healing performance by designing dynamic networks. Specifically, multiple reversible physical and chemical bonds, such as disulfide bonds, hydrogen bonds, and Zn2+ coordination bonds, are integrated into the organosilicon chains via click reactions, carboxylic acid-amine condensation, and ionic coordination. The optimized organosilicon elastomers exhibit exceptional stretchability and mechanical properties, including an elongation at break of ∼5600 %, high strength (2.2 MPa), and toughness (54.38 MJ/m3), outperforming traditional organosilicon elastomers. Additionally, the as-prepared elastomers demonstrate remarkable self-healing ability, with 80–93 % healing efficiency at 25–60 oC, and excellent self-adhesion to various substrates (0.3–1.0 MPa on aluminum, steel, and wood). These properties are maintained under harsh conditions, including low temperature (−10 oC), saltwater, and organic solvents. Clearly, the organosilicon elastomers developed in this work hold significant potential as green and sustainable candidates for various self-adhesive applications.
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| AbstractList | Silicone elastomers with wide-temperature stability and excellent mechanical flexibility have attracted considerable interest in both academic and industrial fields. However, the highly cross-linked networks cannot self-heal and usually show poor adhesion to other substrates, limiting their sustainable applications in emerging fields. Developing self-adhesive organosilicon elastomers with high mechanical strength, superior stretchability, and exceptional self-healing performance remains a significant challenge. Herein, we propose a facile method to synthesize self-adhesive organosilicon elastomers with high mechanical strength, flexibility, and self-healing performance by designing dynamic networks. Specifically, multiple reversible physical and chemical bonds, such as disulfide bonds, hydrogen bonds, and Zn2+ coordination bonds, are integrated into the organosilicon chains via click reactions, carboxylic acid-amine condensation, and ionic coordination. The optimized organosilicon elastomers exhibit exceptional stretchability and mechanical properties, including an elongation at break of ∼5600 %, high strength (2.2 MPa), and toughness (54.38 MJ/m3), outperforming traditional organosilicon elastomers. Additionally, the as-prepared elastomers demonstrate remarkable self-healing ability, with 80–93 % healing efficiency at 25–60 oC, and excellent self-adhesion to various substrates (0.3–1.0 MPa on aluminum, steel, and wood). These properties are maintained under harsh conditions, including low temperature (−10 oC), saltwater, and organic solvents. Clearly, the organosilicon elastomers developed in this work hold significant potential as green and sustainable candidates for various self-adhesive applications. Silicone elastomers with wide-temperature stability and excellent mechanical flexibility have attracted considerable interest in both academic and industrial fields. However, the highly cross-linked networks cannot self-heal and usually show poor adhesion to other substrates, limiting their sustainable applications in emerging fields. Developing self-adhesive organosilicon elastomers with high mechanical strength, superior stretchability, and exceptional self-healing performance remains a significant challenge. Herein, we propose a facile method to synthesize self-adhesive organosilicon elastomers with high mechanical strength, flexibility, and self-healing performance by designing dynamic networks. Specifically, multiple reversible physical and chemical bonds, such as disulfide bonds, hydrogen bonds, and Zn2+ coordination bonds, are integrated into the organosilicon chains via click reactions, carboxylic acid-amine condensation, and ionic coordination. The optimized organosilicon elastomers exhibit exceptional stretchability and mechanical properties, including an elongation at break of ∼5600 %, high strength (2.2 MPa), and toughness (54.38 MJ/m3), outperforming traditional organosilicon elastomers. Additionally, the as-prepared elastomers demonstrate remarkable self-healing ability, with 80–93 % healing efficiency at 25–60 oC, and excellent self-adhesion to various substrates (0.3–1.0 MPa on aluminum, steel, and wood). These properties are maintained under harsh conditions, including low temperature (−10 oC), saltwater, and organic solvents. Clearly, the organosilicon elastomers developed in this work hold significant potential as green and sustainable candidates for various self-adhesive applications. [Display omitted] |
| Author | Liu, Ji Cao, Cheng-Fei Li, Yu-Tong Qin, Yu-Qing Gong, Li-Xiu Li, Shi-Neng Tang, Long-Cheng Liu, Shuai-Chi Liu, Meng-Ying Zhang, Guo-Dong Li, Yang Yang, Ling |
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| Keywords | Mechanical flexibility Self-healing Dynamic networks Self-adhesion Silicone elastomer |
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| SubjectTerms | Dynamic networks Mechanical flexibility Self-adhesion Self-healing Silicone elastomer |
| Title | Mechanically strong, stretchable and self-healable silicone elastomers with designed dynamic networks for exceptional self-adhesion under harsh conditions |
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