Lignocellulosic biomass as renewable feedstock for biodegradable and recyclable plastics production: A sustainable approach

Rapid increment in fossil-derived single-use plastic disposal has led to human-made plastic mountains and leading to ecological imbalance. Therefore, the development of alternative environmentally friendly, biodegradable, and biobased plastics using lignocellulosic biomass renders sustainability. Li...

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Published inRenewable & sustainable energy reviews Vol. 158; p. 112130
Main Authors Raj, Tirath, Chandrasekhar, K., Naresh Kumar, A., Kim, Sang-Hyoun
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.04.2022
Subjects
Biocomposites
Bioplastic
Lactic acid
Polyhydroxyalkanoates
Pretreatment
FDA
AFEX
HBA
PHA
HBD
PHB
Bioplastic
PHH
TENS
PTT
NADH
CAGR
PHO
PHP
Pretreatment
Polyhydroxyalkanoates
Biocomposites
PHV
PBS
Bio-PE
IEA
EMP
PHBV
PGA
PEG
TMP
PEP
Lactic acid
PET
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Abstract Rapid increment in fossil-derived single-use plastic disposal has led to human-made plastic mountains and leading to ecological imbalance. Therefore, the development of alternative environmentally friendly, biodegradable, and biobased plastics using lignocellulosic biomass renders sustainability. Lignocellulosic biomass offers an unprecedented opportunity to produce renewable fuels, chemicals, and materials for the replacement of fossils-based derivatives. The present review comprehensively delineates the potential of lignocellulosic biomass to produce biodegradable and recyclable plastics and plastic composites. Initially, various available pretreatment methods for the deconstruction of natural recalcitrance for fuel and chemical production are summarized, along with the challenges and scope of the integrated biorefinery approach. Energy chemicals such as ethanol, hydrogen produced under biorefinery approach may serve as precursor for bioplastics productions for sustainable bio future. Recyclable and biodegradable polymers such as polyglycolic acid, polyhydroxyalkanoates, polylactic acid, polybutylene succinate, polyvinyl alcohol, biobased polyethylene, biobased polyethylene terephthalate and cellulose acetate have been critically reviewed. Furthermore, the limitations, hurdles, and future scope of commercially available biorefinery industries are deliberated. Thus, technical development and integration in current biorefinery could promote the economical production of biobased biodegradable and recyclable plastics, simultaneously addressing waste biomass utilization constraints. [Display omitted] •Lignocellulosic biomass (LCB) is a potential renewable feedstock for biopolymer.•Low-cost and efficient pretreatment is essential to overcome the recalcitrance.•LCB-derived polymer is either biodegradable (e.g., PHA) or recyclable (e.g., Bio-PE).•Biopolymer can be reinforced with cellulose, lignin, graphene and natural fibers.•Integration with biofuel production is recommended for economics and sustainability.
AbstractList Rapid increment in fossil-derived single-use plastic disposal has led to human-made plastic mountains and leading to ecological imbalance. Therefore, the development of alternative environmentally friendly, biodegradable, and biobased plastics using lignocellulosic biomass renders sustainability. Lignocellulosic biomass offers an unprecedented opportunity to produce renewable fuels, chemicals, and materials for the replacement of fossils-based derivatives. The present review comprehensively delineates the potential of lignocellulosic biomass to produce biodegradable and recyclable plastics and plastic composites. Initially, various available pretreatment methods for the deconstruction of natural recalcitrance for fuel and chemical production are summarized, along with the challenges and scope of the integrated biorefinery approach. Energy chemicals such as ethanol, hydrogen produced under biorefinery approach may serve as precursor for bioplastics productions for sustainable bio future. Recyclable and biodegradable polymers such as polyglycolic acid, polyhydroxyalkanoates, polylactic acid, polybutylene succinate, polyvinyl alcohol, biobased polyethylene, biobased polyethylene terephthalate and cellulose acetate have been critically reviewed. Furthermore, the limitations, hurdles, and future scope of commercially available biorefinery industries are deliberated. Thus, technical development and integration in current biorefinery could promote the economical production of biobased biodegradable and recyclable plastics, simultaneously addressing waste biomass utilization constraints. [Display omitted] •Lignocellulosic biomass (LCB) is a potential renewable feedstock for biopolymer.•Low-cost and efficient pretreatment is essential to overcome the recalcitrance.•LCB-derived polymer is either biodegradable (e.g., PHA) or recyclable (e.g., Bio-PE).•Biopolymer can be reinforced with cellulose, lignin, graphene and natural fibers.•Integration with biofuel production is recommended for economics and sustainability.
ArticleNumber 112130
Author Naresh Kumar, A.
Chandrasekhar, K.
Raj, Tirath
Kim, Sang-Hyoun
Author_xml – sequence: 1
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  orcidid: 0000-0003-2950-0458
  surname: Raj
  fullname: Raj, Tirath
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  surname: Chandrasekhar
  fullname: Chandrasekhar, K.
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  surname: Naresh Kumar
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  givenname: Sang-Hyoun
  orcidid: 0000-0003-3835-4077
  surname: Kim
  fullname: Kim, Sang-Hyoun
  email: sanghkim@yonsei.ac.kr
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– volume: 22
  start-page: 101393
  year: 2021
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  article-title: Can bioplastics be treated in conventional anaerobic digesters for food waste treatment?
  publication-title: Environ Technol Innovat
  doi: 10.1016/j.eti.2021.101393
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Snippet Rapid increment in fossil-derived single-use plastic disposal has led to human-made plastic mountains and leading to ecological imbalance. Therefore, the...
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elsevier
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StartPage 112130
SubjectTerms Biocomposites
Bioplastic
Lactic acid
Polyhydroxyalkanoates
Pretreatment
Title Lignocellulosic biomass as renewable feedstock for biodegradable and recyclable plastics production: A sustainable approach
URI https://dx.doi.org/10.1016/j.rser.2022.112130
Volume 158
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