A multidimensional rational design of nickel–iron sulfide and carbon nanotubes on diatomite via synergistic modulation strategy for supercapacitors
[Display omitted] Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nicke...
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| Published in | Journal of colloid and interface science Vol. 603; pp. 799 - 809 |
|---|---|
| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
01.12.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nickel–iron sulfide nanosheets (NiFeSx) and carbon nanotubes (CNTs) were synthesized on diatomite using chemical vapor deposition and a two-step hydrothermal method to overcome these challenges. Synthesis of this composite successfully exploits the synergistic effect of multicomponent materials to improve the electrochemical performance. Diatomite is selected as a substrate to provide preferable surroundings for the uniform dispersion of nanomaterial on its surface, which enlarges the active sites that come in contact with the electrolytes, significantly improving the electrochemical properties. Combined with high conductivity and a synchronous sulfurization effect, the NiFeSx@CNTs@MnS@Diatomite electrode delivered a high specific capacitance of 552F g−1 at a current density of 1 A g−1, a good rate capability of 68.4% retention at 10 A g−1, and superior cycling stability of 89.8% capacitance retention after 5000 cycles at 5 A g−1. Furthermore, an asymmetric supercapacitor assembled via NiFeSx@CNTs@MnS@Diatomite and graphene delivered a maximum energy density of 28.9 Wh kg−1 and a maximum power density of 9375 W kg−1 at a potential of 1.5 V. This research lays the groundwork for ideal material preparation as well as a rational design for the electrode material, including property enhancement of diatomite-based material for use in supercapacitors. |
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| AbstractList | Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nickel-iron sulfide nanosheets (NiFeSx) and carbon nanotubes (CNTs) were synthesized on diatomite using chemical vapor deposition and a two-step hydrothermal method to overcome these challenges. Synthesis of this composite successfully exploits the synergistic effect of multicomponent materials to improve the electrochemical performance. Diatomite is selected as a substrate to provide preferable surroundings for the uniform dispersion of nanomaterial on its surface, which enlarges the active sites that come in contact with the electrolytes, significantly improving the electrochemical properties. Combined with high conductivity and a synchronous sulfurization effect, the NiFeSx@CNTs@MnS@Diatomite electrode delivered a high specific capacitance of 552F g-1 at a current density of 1 A g-1, a good rate capability of 68.4% retention at 10 A g-1, and superior cycling stability of 89.8% capacitance retention after 5000 cycles at 5 A g-1. Furthermore, an asymmetric supercapacitor assembled via NiFeSx@CNTs@MnS@Diatomite and graphene delivered a maximum energy density of 28.9 Wh kg-1 and a maximum power density of 9375 W kg-1 at a potential of 1.5 V. This research lays the groundwork for ideal material preparation as well as a rational design for the electrode material, including property enhancement of diatomite-based material for use in supercapacitors.Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nickel-iron sulfide nanosheets (NiFeSx) and carbon nanotubes (CNTs) were synthesized on diatomite using chemical vapor deposition and a two-step hydrothermal method to overcome these challenges. Synthesis of this composite successfully exploits the synergistic effect of multicomponent materials to improve the electrochemical performance. Diatomite is selected as a substrate to provide preferable surroundings for the uniform dispersion of nanomaterial on its surface, which enlarges the active sites that come in contact with the electrolytes, significantly improving the electrochemical properties. Combined with high conductivity and a synchronous sulfurization effect, the NiFeSx@CNTs@MnS@Diatomite electrode delivered a high specific capacitance of 552F g-1 at a current density of 1 A g-1, a good rate capability of 68.4% retention at 10 A g-1, and superior cycling stability of 89.8% capacitance retention after 5000 cycles at 5 A g-1. Furthermore, an asymmetric supercapacitor assembled via NiFeSx@CNTs@MnS@Diatomite and graphene delivered a maximum energy density of 28.9 Wh kg-1 and a maximum power density of 9375 W kg-1 at a potential of 1.5 V. This research lays the groundwork for ideal material preparation as well as a rational design for the electrode material, including property enhancement of diatomite-based material for use in supercapacitors. Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nickel–iron sulfide nanosheets (NiFeSx) and carbon nanotubes (CNTs) were synthesized on diatomite using chemical vapor deposition and a two-step hydrothermal method to overcome these challenges. Synthesis of this composite successfully exploits the synergistic effect of multicomponent materials to improve the electrochemical performance. Diatomite is selected as a substrate to provide preferable surroundings for the uniform dispersion of nanomaterial on its surface, which enlarges the active sites that come in contact with the electrolytes, significantly improving the electrochemical properties. Combined with high conductivity and a synchronous sulfurization effect, the NiFeSx@CNTs@MnS@Diatomite electrode delivered a high specific capacitance of 552F g⁻¹ at a current density of 1 A g⁻¹, a good rate capability of 68.4% retention at 10 A g⁻¹, and superior cycling stability of 89.8% capacitance retention after 5000 cycles at 5 A g⁻¹. Furthermore, an asymmetric supercapacitor assembled via NiFeSx@CNTs@MnS@Diatomite and graphene delivered a maximum energy density of 28.9 Wh kg⁻¹ and a maximum power density of 9375 W kg⁻¹ at a potential of 1.5 V. This research lays the groundwork for ideal material preparation as well as a rational design for the electrode material, including property enhancement of diatomite-based material for use in supercapacitors. [Display omitted] Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until now, severe aggregation and low intrinsic conductivity have been the major hurdles for their application. In this work, nickel–iron sulfide nanosheets (NiFeSx) and carbon nanotubes (CNTs) were synthesized on diatomite using chemical vapor deposition and a two-step hydrothermal method to overcome these challenges. Synthesis of this composite successfully exploits the synergistic effect of multicomponent materials to improve the electrochemical performance. Diatomite is selected as a substrate to provide preferable surroundings for the uniform dispersion of nanomaterial on its surface, which enlarges the active sites that come in contact with the electrolytes, significantly improving the electrochemical properties. Combined with high conductivity and a synchronous sulfurization effect, the NiFeSx@CNTs@MnS@Diatomite electrode delivered a high specific capacitance of 552F g−1 at a current density of 1 A g−1, a good rate capability of 68.4% retention at 10 A g−1, and superior cycling stability of 89.8% capacitance retention after 5000 cycles at 5 A g−1. Furthermore, an asymmetric supercapacitor assembled via NiFeSx@CNTs@MnS@Diatomite and graphene delivered a maximum energy density of 28.9 Wh kg−1 and a maximum power density of 9375 W kg−1 at a potential of 1.5 V. This research lays the groundwork for ideal material preparation as well as a rational design for the electrode material, including property enhancement of diatomite-based material for use in supercapacitors. |
| Author | Hu, Zhufeng Dong, Biqin Zhao, Renjun Li, Kailin Liu, Xiaoying Sun, Qing Li, Haiyan Zhang, Yuxin Ji, Junyi Zhou, Jinfei Jing, Chuan Rao, Jinsong Yao, Kexin |
| Author_xml | – sequence: 1 givenname: Kailin surname: Li fullname: Li, Kailin organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 2 givenname: Zhufeng surname: Hu fullname: Hu, Zhufeng organization: School of Chemical Engineering, Sichuan University, Chengdu 610065, PR China – sequence: 3 givenname: Renjun surname: Zhao fullname: Zhao, Renjun organization: School of Chemical Engineering, Sichuan University, Chengdu 610065, PR China – sequence: 4 givenname: Jinfei surname: Zhou fullname: Zhou, Jinfei organization: Multi-scale Porous Materials Center, Institute of Advanced Interdisciplinary Studies, College of Chemistry and Chemical Engineering, Chongqing University, Chongqing 400044, China – sequence: 5 givenname: Chuan surname: Jing fullname: Jing, Chuan organization: College of Science, Chongqing University of Posts and Telecommunications, Chongqing 400065, PR China – sequence: 6 givenname: Qing surname: Sun fullname: Sun, Qing organization: Multi-scale Porous Materials Center, Institute of Advanced Interdisciplinary Studies, College of Chemistry and Chemical Engineering, Chongqing University, Chongqing 400044, China – sequence: 7 givenname: Jinsong surname: Rao fullname: Rao, Jinsong organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 8 givenname: Kexin orcidid: 0000-0002-5686-6909 surname: Yao fullname: Yao, Kexin organization: Multi-scale Porous Materials Center, Institute of Advanced Interdisciplinary Studies, College of Chemistry and Chemical Engineering, Chongqing University, Chongqing 400044, China – sequence: 9 givenname: Biqin surname: Dong fullname: Dong, Biqin organization: School of Civil Engineering, Guangdong Province Key Laboratory of Durability for Marine Civil Engineering, The Key Laboratory on Durability of Civil Engineering in Shenzhen, Shenzhen University, Shenzhen 518060, PR China – sequence: 10 givenname: Xiaoying surname: Liu fullname: Liu, Xiaoying organization: Chongqing Key Laboratory of Catalysis and New Environmental Materials, College of Environment and Resources, Chongqing Technology and Business University, Chongqing 400067, China – sequence: 11 givenname: Haiyan surname: Li fullname: Li, Haiyan organization: School of Chemistry & Chemical Engineering, Northeast Petroleum University, Daqing, 163318, PR China – sequence: 12 givenname: Yuxin surname: Zhang fullname: Zhang, Yuxin email: zhangyuxin@cqu.edu.cn organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 13 givenname: Junyi surname: Ji fullname: Ji, Junyi email: junyiji@scu.edu.cn organization: School of Chemical Engineering, Sichuan University, Chengdu 610065, PR China |
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| PublicationYear | 2021 |
| Publisher | Elsevier Inc |
| Publisher_xml | – name: Elsevier Inc |
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Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in... Based on their characteristics, transition metal layered double hydroxides have been of great scientific interest for their use in supercapacitors. Up until... |
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| SubjectTerms | capacitance Carbon nanotubes diatomaceous earth Diatomite electrochemical capacitors electrochemistry electrodes energy density graphene hot water treatment nanosheets Nickel iron sulfide sulfides Sulfurization process Supercapacitor synergism vapors |
| Title | A multidimensional rational design of nickel–iron sulfide and carbon nanotubes on diatomite via synergistic modulation strategy for supercapacitors |
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