Space-time contours to treat intense field-dressed molecular states

In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [ A. K. Paul , S. Adhikari , D. Mukhopadhyay , J. Phys. Chem. A 113 , 7331 ( 2009 ) ] in which a theory is presented that treats quantum effects due to non...

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Published inThe Journal of chemical physics Vol. 132; no. 3; pp. 034303 - 034303-10
Main Authors Paul, Amit K., Adhikari, Satrajit, Baer, Michael
Format Journal Article
LanguageEnglish
Published United States American Institute of Physics 21.01.2010
Subjects
ACCURACY
APPROXIMATIONS
BORN-OPPENHEIMER APPROXIMATION
BOSONS
CALCULATION METHODS
CATIONS
CHARGED PARTICLES
CHEMICAL REACTIONS
COLLISIONS
DECOMPOSITION
DISSOCIATION
ELEMENTARY PARTICLES
HYDROGEN IONS
HYDROGEN IONS 2 PLUS
INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY
IONS
KINETICS
MASSLESS PARTICLES
MOLECULAR IONS
MOLECULE COLLISIONS
PHOTOCHEMICAL REACTIONS
PHOTOLYSIS
PHOTON COLLISIONS
PHOTON-MOLECULE COLLISIONS
PHOTONS
REACTION KINETICS
SPACE-TIME
TIME DEPENDENCE
Online AccessGet full text
ISSN0021-9606
1089-7690
1089-7690
DOI10.1063/1.3282333

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Abstract In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [ A. K. Paul , S. Adhikari , D. Mukhopadhyay , J. Phys. Chem. A 113 , 7331 ( 2009 ) ] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H 2 + as caused by a laser field.
AbstractList In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul, S. Adhikari, D. Mukhopadhyay et al., J. Phys. Chem. A 113, 7331 (2009)] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H(2) (+) as caused by a laser field.
In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul, S. Adhikari, D. Mukhopadhyay et al., J. Phys. Chem. A 113, 7331 (2009)] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H(2) (+) as caused by a laser field.In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul, S. Adhikari, D. Mukhopadhyay et al., J. Phys. Chem. A 113, 7331 (2009)] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H(2) (+) as caused by a laser field.
In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul, S. Adhikari, D. Mukhopadhyay et al., J. Phys. Chem. A 113, 7331 (2009)] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H{sub 2}{sup +} as caused by a laser field.
In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [ A. K. Paul , S. Adhikari , D. Mukhopadhyay , J. Phys. Chem. A 113 , 7331 ( 2009 ) ] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born-Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H 2 + as caused by a laser field.
In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul, S. Adhikari, D. Mukhopadhyay et al., J. Phys. Chem. A 113, 7331 (2009)] in which a theory is presented that treats quantum effects due to nonclassical photon states (known also as Fock states). Since these states became recently a subject of intense experimental efforts we thought that they can be treated properly within the existing quantum formulation of dynamical processes. This was achieved by incorporating them in the Born–Oppenheimer (BO) treatment with time-dependent coefficients. The extension of the BO treatment to include the Fock states results in a formidable enhancement in numerical efforts expressed, in particular, in a significant increase in CPU time. In the present article we discuss an approach that yields an efficient and reliable approximation with only negligible losses in accuracy. The approximation is tested in detail for the dissociation process of H2+ as caused by a laser field.
Author Baer, Michael
Adhikari, Satrajit
Paul, Amit K.
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  givenname: Michael
  surname: Baer
  fullname: Baer, Michael
  email: michaelb@fh.huji.ac.il.
  organization: Department of Physical Chemistry, Indian Association for Cultivation of Science, Jadavpur,Kolkata 700 032, India
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CitedBy_id crossref_primary_10_1002_qua_24734
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crossref_primary_10_1140_epjd_e2017_80327_y
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Snippet In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [ A. K. Paul ,...
In this article we consider a molecular system exposed to an intense short-pulsed external field. It is a continuation of a previous publication [A. K. Paul,...
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SubjectTerms ACCURACY
APPROXIMATIONS
BORN-OPPENHEIMER APPROXIMATION
BOSONS
CALCULATION METHODS
CATIONS
CHARGED PARTICLES
CHEMICAL REACTIONS
COLLISIONS
DECOMPOSITION
DISSOCIATION
ELEMENTARY PARTICLES
HYDROGEN IONS
HYDROGEN IONS 2 PLUS
INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY
IONS
KINETICS
MASSLESS PARTICLES
MOLECULAR IONS
MOLECULE COLLISIONS
PHOTOCHEMICAL REACTIONS
PHOTOLYSIS
PHOTON COLLISIONS
PHOTON-MOLECULE COLLISIONS
PHOTONS
REACTION KINETICS
SPACE-TIME
TIME DEPENDENCE
Title Space-time contours to treat intense field-dressed molecular states
URI http://dx.doi.org/10.1063/1.3282333
https://www.ncbi.nlm.nih.gov/pubmed/20095735
https://www.proquest.com/docview/733807595
https://www.osti.gov/biblio/21559828
Volume 132
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