BiOBr/Bi2S3 heterojunction with S-scheme structureand oxygen defects: In-situ construction and photocatalytic behavior for reduction of CO2 with H2O
[Display omitted] Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi2S3 heterojunction with surface oxygen vacancies (OVs) was synthesi...
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| Published in | Journal of colloid and interface science Vol. 620; pp. 407 - 418 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.08.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi2S3 heterojunction with surface oxygen vacancies (OVs) was synthesized in situ by a facile hydrothermal method. The as-prepared photocatalyst show high activity for CO2 photoreduction with pure water. The yields of product CO and CH4 are as high as 100.8 and 8.5 µmol g−1h−1, which are 17.5 and 13.5 times higher than that of the pristine Bi2S3, and 2.3 and 4.7 times higher than that of the pristine BiOBr respectively. The excellent activity of the BiOBr/Bi2S3 heterojunction is attributed to both the S-scheme electron structure and the surface OVs of the component BiOBr. The S-scheme structure can enhance utilization of sunlight and improve the separation and transfer of photogenerated electron/hole pairs. The surface OVs of BiOBr can serve as active sites of CO2 and H2O in the photocatalytic process. This work provides some novel insights of S-scheme heterojunction with defects for photocatalytic CO2 reduction. |
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| AbstractList | [Display omitted]
Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi2S3 heterojunction with surface oxygen vacancies (OVs) was synthesized in situ by a facile hydrothermal method. The as-prepared photocatalyst show high activity for CO2 photoreduction with pure water. The yields of product CO and CH4 are as high as 100.8 and 8.5 µmol g−1h−1, which are 17.5 and 13.5 times higher than that of the pristine Bi2S3, and 2.3 and 4.7 times higher than that of the pristine BiOBr respectively. The excellent activity of the BiOBr/Bi2S3 heterojunction is attributed to both the S-scheme electron structure and the surface OVs of the component BiOBr. The S-scheme structure can enhance utilization of sunlight and improve the separation and transfer of photogenerated electron/hole pairs. The surface OVs of BiOBr can serve as active sites of CO2 and H2O in the photocatalytic process. This work provides some novel insights of S-scheme heterojunction with defects for photocatalytic CO2 reduction. Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi₂S₃ heterojunction with surface oxygen vacancies (OVs) was synthesized in situ by a facile hydrothermal method. The as-prepared photocatalyst show high activity for CO₂ photoreduction with pure water. The yields of product CO and CH₄ are as high as 100.8 and 8.5 µmol g⁻¹h⁻¹, which are 17.5 and 13.5 times higher than that of the pristine Bi₂S₃, and 2.3 and 4.7 times higher than that of the pristine BiOBr respectively. The excellent activity of the BiOBr/Bi₂S₃ heterojunction is attributed to both the S-scheme electron structure and the surface OVs of the component BiOBr. The S-scheme structure can enhance utilization of sunlight and improve the separation and transfer of photogenerated electron/hole pairs. The surface OVs of BiOBr can serve as active sites of CO₂ and H₂O in the photocatalytic process. This work provides some novel insights of S-scheme heterojunction with defects for photocatalytic CO₂ reduction. Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi2S3 heterojunction with surface oxygen vacancies (OVs) was synthesized in situ by a facile hydrothermal method. The as-prepared photocatalyst show high activity for CO2 photoreduction with pure water. The yields of product CO and CH4 are as high as 100.8 and 8.5 µmol g-1h-1, which are 17.5 and 13.5 times higher than that of the pristine Bi2S3, and 2.3 and 4.7 times higher than that of the pristine BiOBr respectively. The excellent activity of the BiOBr/Bi2S3 heterojunction is attributed to both the S-scheme electron structure and the surface OVs of the component BiOBr. The S-scheme structure can enhance utilization of sunlight and improve the separation and transfer of photogenerated electron/hole pairs. The surface OVs of BiOBr can serve as active sites of CO2 and H2O in the photocatalytic process. This work provides some novel insights of S-scheme heterojunction with defects for photocatalytic CO2 reduction.Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox ability of single photocatalyst. Herein, S-scheme BiOBr/Bi2S3 heterojunction with surface oxygen vacancies (OVs) was synthesized in situ by a facile hydrothermal method. The as-prepared photocatalyst show high activity for CO2 photoreduction with pure water. The yields of product CO and CH4 are as high as 100.8 and 8.5 µmol g-1h-1, which are 17.5 and 13.5 times higher than that of the pristine Bi2S3, and 2.3 and 4.7 times higher than that of the pristine BiOBr respectively. The excellent activity of the BiOBr/Bi2S3 heterojunction is attributed to both the S-scheme electron structure and the surface OVs of the component BiOBr. The S-scheme structure can enhance utilization of sunlight and improve the separation and transfer of photogenerated electron/hole pairs. The surface OVs of BiOBr can serve as active sites of CO2 and H2O in the photocatalytic process. This work provides some novel insights of S-scheme heterojunction with defects for photocatalytic CO2 reduction. |
| Author | Wang, Ning Xu, Peng Wang, Xuxu Zhang, Yanfeng Miao, Zerui |
| Author_xml | – sequence: 1 givenname: Zerui surname: Miao fullname: Miao, Zerui organization: National Demonstration Center for Experimental Chemistry Education, Hebei Key Laboratory of Inorganic Nano-materials, College of Chemistry and Materials Science, Hebei Normal University, Shijiazhuang 050024, PR China – sequence: 2 givenname: Yanfeng surname: Zhang fullname: Zhang, Yanfeng email: zhangyanfeng@hebtu.edu.cn organization: National Demonstration Center for Experimental Chemistry Education, Hebei Key Laboratory of Inorganic Nano-materials, College of Chemistry and Materials Science, Hebei Normal University, Shijiazhuang 050024, PR China – sequence: 3 givenname: Ning surname: Wang fullname: Wang, Ning organization: National Demonstration Center for Experimental Chemistry Education, Hebei Key Laboratory of Inorganic Nano-materials, College of Chemistry and Materials Science, Hebei Normal University, Shijiazhuang 050024, PR China – sequence: 4 givenname: Peng surname: Xu fullname: Xu, Peng email: xup@nanoctr.cn organization: CAS Key Laboratory of Standardization and Measurement for Nanotechnology, National Center for Nanoscience and Technology, Beijing 100190, PR China – sequence: 5 givenname: Xuxu surname: Wang fullname: Wang, Xuxu email: zhangyanfeng@mail.hebtu.edu.cn, xwang@fzu.edu.cn organization: State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, Fuzhou 350108, PR China |
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Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers... Constructing heterojunction has been considered as an efficient strategy to promote the separation and transfer of photogenerated carriers and improve redox... |
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| SubjectTerms | Bi2S3 BiOBr carbon dioxide CO2 reduction hot water treatment oxygen photocatalysis photocatalysts Photocatalytic photoreduction S-scheme solar radiation |
| Title | BiOBr/Bi2S3 heterojunction with S-scheme structureand oxygen defects: In-situ construction and photocatalytic behavior for reduction of CO2 with H2O |
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