Hierarchical Sb2S3/ZnIn2S4 core–shell heterostructure for highly efficient photocatalytic hydrogen production and pollutant degradation
A novel ZnIn2S4 decorated Sb2S3 hierarchical 1D/2D core–shell heterostructure was successfully fabricated by a simple hydrothermal method. It possessed highly efficient photocatalytic activities of hydrogen evolution and pollutant degradation. This work will provide a novel dual-function core–shell...
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| Published in | Journal of colloid and interface science Vol. 623; pp. 109 - 123 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
01.10.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A novel ZnIn2S4 decorated Sb2S3 hierarchical 1D/2D core–shell heterostructure was successfully fabricated by a simple hydrothermal method. It possessed highly efficient photocatalytic activities of hydrogen evolution and pollutant degradation. This work will provide a novel dual-function core–shell heterostructure photocatalyst to solve environmental pollution and produce hydrogen energy.
[Display omitted]
In this work, a novel hierarchical 1D/2D core/shell Sb2S3-ZnIn2S4 (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen production from water and organic pollutant degradation was designed and fabricated via a simple one-step hydrothermal method. The as-prepared SB-ZIS heterostructure, where ZnIn2S4 nanosheets uniformly grew onto Sb2S3 nanorod to form a tight and large intimate contacted interface, was conducive to improve the absorption capacity of light, increase the surface area, shorten the distance of electronic transmission channels and accelerate the separation and migration of photogenerated carriers. As a result, the presented SB-ZIS composites demonstrated significantly enhanced photocatalytic performances for H2 generation and Tetracycline Hydrochloride (TCH) photodegradation. The photocatalytic H2 production rate of optimal SB-ZIS-2 sample (1685.14 μmol·g−1·h−1) was about 12.24 times as large as that of pure ZnIn2S4 (137.63 μmol·g−1·h−1). The apparent quantum efficiency (AQE) at 420 nm was up to 3.8%. In addition, the highest rate constant for TCH removal (0.514 h−1) was 20.3 and 2.89 times larger than those of pure Sb2S3 and Znln2S4, respectively. The possible reaction routes of TCH and the photocatalytic reaction mechanism of SB-ZIS sample were also discussed in detail. This work will provide some useful information for the development of dual-functional Sb2S3-based type I core–shell heterostructure with an efficient photocatalytic activity for solving environmental pollution and producing clean hydrogen energy. |
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| AbstractList | A novel ZnIn2S4 decorated Sb2S3 hierarchical 1D/2D core–shell heterostructure was successfully fabricated by a simple hydrothermal method. It possessed highly efficient photocatalytic activities of hydrogen evolution and pollutant degradation. This work will provide a novel dual-function core–shell heterostructure photocatalyst to solve environmental pollution and produce hydrogen energy.
[Display omitted]
In this work, a novel hierarchical 1D/2D core/shell Sb2S3-ZnIn2S4 (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen production from water and organic pollutant degradation was designed and fabricated via a simple one-step hydrothermal method. The as-prepared SB-ZIS heterostructure, where ZnIn2S4 nanosheets uniformly grew onto Sb2S3 nanorod to form a tight and large intimate contacted interface, was conducive to improve the absorption capacity of light, increase the surface area, shorten the distance of electronic transmission channels and accelerate the separation and migration of photogenerated carriers. As a result, the presented SB-ZIS composites demonstrated significantly enhanced photocatalytic performances for H2 generation and Tetracycline Hydrochloride (TCH) photodegradation. The photocatalytic H2 production rate of optimal SB-ZIS-2 sample (1685.14 μmol·g−1·h−1) was about 12.24 times as large as that of pure ZnIn2S4 (137.63 μmol·g−1·h−1). The apparent quantum efficiency (AQE) at 420 nm was up to 3.8%. In addition, the highest rate constant for TCH removal (0.514 h−1) was 20.3 and 2.89 times larger than those of pure Sb2S3 and Znln2S4, respectively. The possible reaction routes of TCH and the photocatalytic reaction mechanism of SB-ZIS sample were also discussed in detail. This work will provide some useful information for the development of dual-functional Sb2S3-based type I core–shell heterostructure with an efficient photocatalytic activity for solving environmental pollution and producing clean hydrogen energy. In this work, a novel hierarchical 1D/2D core/shell Sb₂S₃-ZnIn₂S₄ (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen production from water and organic pollutant degradation was designed and fabricated via a simple one-step hydrothermal method. The as-prepared SB-ZIS heterostructure, where ZnIn₂S₄ nanosheets uniformly grew onto Sb₂S₃ nanorod to form a tight and large intimate contacted interface, was conducive to improve the absorption capacity of light, increase the surface area, shorten the distance of electronic transmission channels and accelerate the separation and migration of photogenerated carriers. As a result, the presented SB-ZIS composites demonstrated significantly enhanced photocatalytic performances for H₂ generation and Tetracycline Hydrochloride (TCH) photodegradation. The photocatalytic H₂ production rate of optimal SB-ZIS-2 sample (1685.14 μmol·g⁻¹·h⁻¹) was about 12.24 times as large as that of pure ZnIn₂S₄ (137.63 μmol·g⁻¹·h⁻¹). The apparent quantum efficiency (AQE) at 420 nm was up to 3.8%. In addition, the highest rate constant for TCH removal (0.514 h⁻¹) was 20.3 and 2.89 times larger than those of pure Sb₂S₃ and Znln₂S₄, respectively. The possible reaction routes of TCH and the photocatalytic reaction mechanism of SB-ZIS sample were also discussed in detail. This work will provide some useful information for the development of dual-functional Sb₂S₃-based type I core–shell heterostructure with an efficient photocatalytic activity for solving environmental pollution and producing clean hydrogen energy. In this work, a novel hierarchical 1D/2D core/shell Sb2S3-ZnIn2S4 (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen production from water and organic pollutant degradation was designed and fabricated via a simple one-step hydrothermal method. The as-prepared SB-ZIS heterostructure, where ZnIn2S4 nanosheets uniformly grew onto Sb2S3 nanorod to form a tight and large intimate contacted interface, was conducive to improve the absorption capacity of light, increase the surface area, shorten the distance of electronic transmission channels and accelerate the separation and migration of photogenerated carriers. As a result, the presented SB-ZIS composites demonstrated significantly enhanced photocatalytic performances for H2 generation and Tetracycline Hydrochloride (TCH) photodegradation. The photocatalytic H2 production rate of optimal SB-ZIS-2 sample (1685.14 μmol·g-1·h-1) was about 12.24 times as large as that of pure ZnIn2S4 (137.63 μmol·g-1·h-1). The apparent quantum efficiency (AQE) at 420 nm was up to 3.8%. In addition, the highest rate constant for TCH removal (0.514 h-1) was 20.3 and 2.89 times larger than those of pure Sb2S3 and Znln2S4, respectively. The possible reaction routes of TCH and the photocatalytic reaction mechanism of SB-ZIS sample were also discussed in detail. This work will provide some useful information for the development of dual-functional Sb2S3-based type I core-shell heterostructure with an efficient photocatalytic activity for solving environmental pollution and producing clean hydrogen energy.In this work, a novel hierarchical 1D/2D core/shell Sb2S3-ZnIn2S4 (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen production from water and organic pollutant degradation was designed and fabricated via a simple one-step hydrothermal method. The as-prepared SB-ZIS heterostructure, where ZnIn2S4 nanosheets uniformly grew onto Sb2S3 nanorod to form a tight and large intimate contacted interface, was conducive to improve the absorption capacity of light, increase the surface area, shorten the distance of electronic transmission channels and accelerate the separation and migration of photogenerated carriers. As a result, the presented SB-ZIS composites demonstrated significantly enhanced photocatalytic performances for H2 generation and Tetracycline Hydrochloride (TCH) photodegradation. The photocatalytic H2 production rate of optimal SB-ZIS-2 sample (1685.14 μmol·g-1·h-1) was about 12.24 times as large as that of pure ZnIn2S4 (137.63 μmol·g-1·h-1). The apparent quantum efficiency (AQE) at 420 nm was up to 3.8%. In addition, the highest rate constant for TCH removal (0.514 h-1) was 20.3 and 2.89 times larger than those of pure Sb2S3 and Znln2S4, respectively. The possible reaction routes of TCH and the photocatalytic reaction mechanism of SB-ZIS sample were also discussed in detail. This work will provide some useful information for the development of dual-functional Sb2S3-based type I core-shell heterostructure with an efficient photocatalytic activity for solving environmental pollution and producing clean hydrogen energy. |
| Author | Xiao, Yan Liu, Zhanchao Wu, Xiangyang Jiang, Yinhua Zhang, Jianming Zhang, Wenli Deng, Wei Wang, Hao |
| Author_xml | – sequence: 1 givenname: Yan surname: Xiao fullname: Xiao, Yan organization: Institute of Environmental Health and Ecological Security, School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 2 givenname: Hao surname: Wang fullname: Wang, Hao organization: School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 3 givenname: Yinhua surname: Jiang fullname: Jiang, Yinhua email: jyhua@ujs.edu.cn organization: School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 4 givenname: Wenli surname: Zhang fullname: Zhang, Wenli organization: School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 5 givenname: Jianming surname: Zhang fullname: Zhang, Jianming organization: School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 6 givenname: Xiangyang surname: Wu fullname: Wu, Xiangyang email: wuxy@ujs.edu.cn organization: Institute of Environmental Health and Ecological Security, School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, PR China – sequence: 7 givenname: Zhanchao surname: Liu fullname: Liu, Zhanchao organization: School of Materials Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, PR China – sequence: 8 givenname: Wei surname: Deng fullname: Deng, Wei organization: Foshan (Southern China) Institute for New Materials, Foshan, Guangdong 528200, China |
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| Snippet | A novel ZnIn2S4 decorated Sb2S3 hierarchical 1D/2D core–shell heterostructure was successfully fabricated by a simple hydrothermal method. It possessed highly... In this work, a novel hierarchical 1D/2D core/shell Sb2S3-ZnIn2S4 (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen... In this work, a novel hierarchical 1D/2D core/shell Sb₂S₃-ZnIn₂S₄ (SB-ZIS) heterostructure with highly efficient photocatalytic activities for both hydrogen... |
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| SubjectTerms | absorption Dual-functional energy hierarchical 1D/2D heterostructure hot water treatment hydrogen hydrogen production nanorods nanosheets photocatalysis photolysis pollutants pollution reaction mechanisms Sb2S3 nanorod surface area tetracycline ZnIn2S4 nanosheet |
| Title | Hierarchical Sb2S3/ZnIn2S4 core–shell heterostructure for highly efficient photocatalytic hydrogen production and pollutant degradation |
| URI | https://dx.doi.org/10.1016/j.jcis.2022.04.137 https://www.proquest.com/docview/2665108345 https://www.proquest.com/docview/2675560087 |
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