Surface tension and interfacial tension of polyolefins and polyolefin blends
This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and high‐density polyethylene with syndiotactic polypropylene. For this, three methods to measure the interfacial tension are compared: the use of Palierne's mo...
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Published in | Journal of applied polymer science Vol. 139; no. 14 |
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Main Authors | , , , |
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Hoboken, USA
John Wiley & Sons, Inc
10.04.2022
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Abstract | This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and high‐density polyethylene with syndiotactic polypropylene. For this, three methods to measure the interfacial tension are compared: the use of Palierne's model, and Gramespacher and Meissner's model, both based on additional elasticity or long relaxation times brought by shape recovery of dispersed phase, and ab‐initio calculation, which requires the knowledge of the surface tension of the neat polymer measured at the same temperature. For that, a database collected from the literature is built in the first section of this paper, whether for the studied systems or for other systems of various olefinic homopolymers or copolymers with polypropylene. The results show the effectiveness of the Gramespacher and Meissner's model to calculate the interfacial tension of the studied systems for which the results were in agreement with ab‐initio calculation and Palierne's model. Extension of the ab‐initio calculation to olefinic copolymers was proposed. |
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AbstractList | This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and high‐density polyethylene with syndiotactic polypropylene. For this, three methods to measure the interfacial tension are compared: the use of Palierne's model, and Gramespacher and Meissner's model, both based on additional elasticity or long relaxation times brought by shape recovery of dispersed phase, and ab‐initio calculation, which requires the knowledge of the surface tension of the neat polymer measured at the same temperature. For that, a database collected from the literature is built in the first section of this paper, whether for the studied systems or for other systems of various olefinic homopolymers or copolymers with polypropylene. The results show the effectiveness of the Gramespacher and Meissner's model to calculate the interfacial tension of the studied systems for which the results were in agreement with ab‐initio calculation and Palierne's model. Extension of the ab‐initio calculation to olefinic copolymers was proposed. Abstract This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and high‐density polyethylene with syndiotactic polypropylene. For this, three methods to measure the interfacial tension are compared: the use of Palierne's model, and Gramespacher and Meissner's model, both based on additional elasticity or long relaxation times brought by shape recovery of dispersed phase, and ab‐initio calculation, which requires the knowledge of the surface tension of the neat polymer measured at the same temperature. For that, a database collected from the literature is built in the first section of this paper, whether for the studied systems or for other systems of various olefinic homopolymers or copolymers with polypropylene. The results show the effectiveness of the Gramespacher and Meissner's model to calculate the interfacial tension of the studied systems for which the results were in agreement with ab‐initio calculation and Palierne's model. Extension of the ab‐initio calculation to olefinic copolymers was proposed. |
Author | Charfeddine, Ilhem Carrot, Christian Majesté, Jean‐Charles Lhost, Olivier |
Author_xml | – sequence: 1 givenname: Ilhem surname: Charfeddine fullname: Charfeddine, Ilhem organization: TOTAL Research and Technology Feluy – sequence: 2 givenname: Jean‐Charles surname: Majesté fullname: Majesté, Jean‐Charles organization: Univ Lyon, UJM‐Saint‐Etienne, CNRS, IMP UMR5223 – sequence: 3 givenname: Christian orcidid: 0000-0001-8928-828X surname: Carrot fullname: Carrot, Christian email: carrot@univ-st-etienne.fr organization: Univ Lyon, UJM‐Saint‐Etienne, CNRS, IMP UMR5223 – sequence: 4 givenname: Olivier surname: Lhost fullname: Lhost, Olivier organization: TOTAL Research and Technology Feluy |
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Snippet | This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and high‐density... Abstract This paper focuses on the calculation of the interfacial tension of two systems: low‐density polyethylene with isotactic polypropylene and... This paper focuses on the calculation of the interfacial tension of two systems: low-density polyethylene with isotactic polypropylene and high-density... |
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SubjectTerms | Chemical Sciences Copolymers Density Materials science Mathematical models Polyethylenes Polymer blends Polymers Polyolefins Polypropylene structure‐property relationships Surface tension surfaces and interfaces Syndiotacticity |
Title | Surface tension and interfacial tension of polyolefins and polyolefin blends |
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