Adsorption of BTX from aqueous solutions by Na-P1 zeolite obtained from fly ash

•BTX sorption on zeolite Na-P1 from F-class fly ash was studied.•Sorption efficiency was dependent on BTX initial concentration.•Sorption of BTX followed the order: xylenes>toluene>benzene. The adsorption of BTX (benzene, toluene, o- and p-xylene) from aqueous solution by synthetic zeolite Na-...

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Published inProcess safety and environmental protection Vol. 109; pp. 214 - 223
Main Authors Bandura, Lidia, Kołodyńska, Dorota, Franus, Wojciech
Format Journal Article
LanguageEnglish
Published Rugby Elsevier B.V 01.07.2017
Elsevier Science Ltd
Subjects
Adsorption
Adsorption isotherms
Adsorption kinetics
Aqueous solutions
Benzene
BTX removal
Chemical synthesis
Fly ash
Isotherms
Kinetics
p-Xylene
Reaction kinetics
Scanning electron microscopy
Sorption
Synthetic zeolites
Toluene
Ultrasonic testing
Water treatment
X-ray diffraction
Xylene
Zeolite Na-P1
Zeolites
Water treatment
Synthetic zeolites
Adsorption kinetics
Adsorption isotherms
Zeolite Na-P1
BTX removal
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Abstract •BTX sorption on zeolite Na-P1 from F-class fly ash was studied.•Sorption efficiency was dependent on BTX initial concentration.•Sorption of BTX followed the order: xylenes>toluene>benzene. The adsorption of BTX (benzene, toluene, o- and p-xylene) from aqueous solution by synthetic zeolite Na-P1 obtained from fly ash was examined. The adsorbent was characterized by scanning electron microscope (SEM-EDS) and X-ray diffraction (XRD). Surface area and pore volume distribution were determined using a nitrogen adsorption/desorption isotherm. BTX adsorption tests, including the influence of contact time, sorption isotherms and the influence of initial concentration, were performed in a batch multicomponent system. The sorption capacity followed the order xylenes>toluene>benzene, and the removal efficiency decreased with an increase in initial BTX concentration. The process kinetics was evaluated using pseudo-first-order, pseudo-second-order and intraparticle diffusion models. The adsorption equilibrium was reached within 24h and followed pseudo-second-order kinetics. The Langmuir, Freundlich and Temkin models were used to evaluate the adsorption capacity of Na-P1. The Langmuir model was found to be the most suitable for all BTX sorption from a multicomponent system. The calculated maximum adsorption capacities of Na-P1 (qmax) for benzene, toluene, o- and p-xylene were 0.032, 0.050, 0.147 and 0.129 respectively.
AbstractList •BTX sorption on zeolite Na-P1 from F-class fly ash was studied.•Sorption efficiency was dependent on BTX initial concentration.•Sorption of BTX followed the order: xylenes>toluene>benzene. The adsorption of BTX (benzene, toluene, o- and p-xylene) from aqueous solution by synthetic zeolite Na-P1 obtained from fly ash was examined. The adsorbent was characterized by scanning electron microscope (SEM-EDS) and X-ray diffraction (XRD). Surface area and pore volume distribution were determined using a nitrogen adsorption/desorption isotherm. BTX adsorption tests, including the influence of contact time, sorption isotherms and the influence of initial concentration, were performed in a batch multicomponent system. The sorption capacity followed the order xylenes>toluene>benzene, and the removal efficiency decreased with an increase in initial BTX concentration. The process kinetics was evaluated using pseudo-first-order, pseudo-second-order and intraparticle diffusion models. The adsorption equilibrium was reached within 24h and followed pseudo-second-order kinetics. The Langmuir, Freundlich and Temkin models were used to evaluate the adsorption capacity of Na-P1. The Langmuir model was found to be the most suitable for all BTX sorption from a multicomponent system. The calculated maximum adsorption capacities of Na-P1 (qmax) for benzene, toluene, o- and p-xylene were 0.032, 0.050, 0.147 and 0.129 respectively.
The adsorption of BTX (benzene, toluene, o- and p-xylene) from aqueous solution by synthetic zeolite Na-P1 obtained from fly ash was examined. The adsorbent was characterized by scanning electron microscope (SEM-EDS) and X-ray diffraction (XRD). Surface area and pore volume distribution were determined using a nitrogen adsorption/desorption isotherm. BTX adsorption tests, including the influence of contact time, sorption isotherms and the influence of initial concentration, were performed in a batch multicomponent system. The sorption capacity followed the order xylenes > toluene > benzene, and the removal efficiency decreased with an increase in initial BTX concentration. The process kinetics was evaluated using pseudo-first-order, pseudo-second-order and intraparticle diffusion models. The adsorption equilibrium was reached within 24 h and followed pseudo-second-order kinetics. The Langmuir, Freundlich and Temkin models were used to evaluate the adsorption capacity of Na-P1. The Langmuir model was found to be the most suitable for all BTX sorption from a multicomponent system. The calculated maximum adsorption capacities of Na-P1 (qmax) for benzene, toluene, o- and p-xylene were 0.032, 0.050, 0.147 and 0.129 respectively.
Author Franus, Wojciech
Kołodyńska, Dorota
Bandura, Lidia
Author_xml – sequence: 1
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  givenname: Dorota
  surname: Kołodyńska
  fullname: Kołodyńska, Dorota
  organization: Department of Inorganic Chemistry, Faculty of Chemistry, Maria Curie Skłodowska University, Maria Curie Skłodowska Sq. 2, 20-031 Lublin, Poland
– sequence: 3
  givenname: Wojciech
  surname: Franus
  fullname: Franus, Wojciech
  email: w.franus@pollub.pl
  organization: Department of Geotechnical Engineering, Faculty of Civil Engineering and Architecture, Lublin University of Technology, Nadbystrzycka 40, 20-618 Lublin, Poland
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Keywords Water treatment
Synthetic zeolites
Adsorption kinetics
Adsorption isotherms
Zeolite Na-P1
BTX removal
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Snippet •BTX sorption on zeolite Na-P1 from F-class fly ash was studied.•Sorption efficiency was dependent on BTX initial concentration.•Sorption of BTX followed the...
The adsorption of BTX (benzene, toluene, o- and p-xylene) from aqueous solution by synthetic zeolite Na-P1 obtained from fly ash was examined. The adsorbent...
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SubjectTerms Adsorption
Adsorption isotherms
Adsorption kinetics
Aqueous solutions
Benzene
BTX removal
Chemical synthesis
Fly ash
Isotherms
Kinetics
p-Xylene
Reaction kinetics
Scanning electron microscopy
Sorption
Synthetic zeolites
Toluene
Ultrasonic testing
Water treatment
X-ray diffraction
Xylene
Zeolite Na-P1
Zeolites
Title Adsorption of BTX from aqueous solutions by Na-P1 zeolite obtained from fly ash
URI https://dx.doi.org/10.1016/j.psep.2017.03.036
https://www.proquest.com/docview/2089732219
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