Highly efficient prismatic perovskite solar cells
Lead halide perovskites, such as methylammonium lead iodide (MAPbI 3 ) can reach near 100% internal quantum efficiency in single solar cells, but they still encounter significant thermodynamic losses in photon energy to offset device photovoltage and performance. Herein, a novel prismatic perovskite...
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| Published in | Energy & environmental science Vol. 12; no. 3; pp. 929 - 937 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
01.01.2019
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lead halide perovskites, such as methylammonium lead iodide (MAPbI
3
) can reach near 100% internal quantum efficiency in single solar cells, but they still encounter significant thermodynamic losses in photon energy to offset device photovoltage and performance. Herein, a novel prismatic perovskite solar cell with light trapping configuration, namely, Prim PVSC, is designed to mitigate such losses in devices, through modulating the pathway of light inside series cells, wherein incident high-to-low energy photons are separately captured by four horizontally aligned MAPbI
x
Br
3−x
subcells with varied bandgaps. This newly designed PVSC has remarkably led to a record open circuit voltage of 5.3 V in four series devices and power conversion efficiency of 21.3%, which could provide a new way to break the performance bottleneck of perovskites. Practically, this type of device architecture could also be applied in flexible modules for large-area application. |
|---|---|
| AbstractList | Lead halide perovskites, such as methylammonium lead iodide (MAPbI
3
) can reach near 100% internal quantum efficiency in single solar cells, but they still encounter significant thermodynamic losses in photon energy to offset device photovoltage and performance. Herein, a novel prismatic perovskite solar cell with light trapping configuration, namely, Prim PVSC, is designed to mitigate such losses in devices, through modulating the pathway of light inside series cells, wherein incident high-to-low energy photons are separately captured by four horizontally aligned MAPbI
x
Br
3−x
subcells with varied bandgaps. This newly designed PVSC has remarkably led to a record open circuit voltage of 5.3 V in four series devices and power conversion efficiency of 21.3%, which could provide a new way to break the performance bottleneck of perovskites. Practically, this type of device architecture could also be applied in flexible modules for large-area application. Lead halide perovskites, such as methylammonium lead iodide (MAPbI3) can reach near 100% internal quantum efficiency in single solar cells, but they still encounter significant thermodynamic losses in photon energy to offset device photovoltage and performance. Herein, a novel prismatic perovskite solar cell with light trapping configuration, namely, Prim PVSC, is designed to mitigate such losses in devices, through modulating the pathway of light inside series cells, wherein incident high-to-low energy photons are separately captured by four horizontally aligned MAPbIxBr3−x subcells with varied bandgaps. This newly designed PVSC has remarkably led to a record open circuit voltage of 5.3 V in four series devices and power conversion efficiency of 21.3%, which could provide a new way to break the performance bottleneck of perovskites. Practically, this type of device architecture could also be applied in flexible modules for large-area application. |
| Author | Huang, Jiang Xiang, Siheng Yu, Junsheng Li, Chang-Zhi |
| Author_xml | – sequence: 1 givenname: Jiang surname: Huang fullname: Huang, Jiang organization: State Key Laboratory of Electronic Thin Films and Integrated Devices, School of Optoelectronic Science and Engineering, University of Electronic Science and Technology of China (UESTC), Chengdu 610054, P. R. China – sequence: 2 givenname: Siheng surname: Xiang fullname: Xiang, Siheng organization: State Key Laboratory of Electronic Thin Films and Integrated Devices, School of Optoelectronic Science and Engineering, University of Electronic Science and Technology of China (UESTC), Chengdu 610054, P. R. China – sequence: 3 givenname: Junsheng orcidid: 0000-0002-7484-8114 surname: Yu fullname: Yu, Junsheng organization: State Key Laboratory of Electronic Thin Films and Integrated Devices, School of Optoelectronic Science and Engineering, University of Electronic Science and Technology of China (UESTC), Chengdu 610054, P. R. China – sequence: 4 givenname: Chang-Zhi orcidid: 0000-0003-1968-2032 surname: Li fullname: Li, Chang-Zhi organization: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou 310027 |
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) can reach near 100% internal quantum efficiency in single solar cells, but they still... Lead halide perovskites, such as methylammonium lead iodide (MAPbI3) can reach near 100% internal quantum efficiency in single solar cells, but they still... |
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| SubjectTerms | Circuit design Computer architecture Data processing Energy conversion efficiency Iodides Lead Open circuit voltage Perovskites Photons Photovoltaic cells Quantum efficiency Solar cells |
| Title | Highly efficient prismatic perovskite solar cells |
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