Effects of random quenched impurities on wetting of solids: a Monte Carlo study
This paper presents the results of a Monte Carlo simulation study of the effects of randomly distributed quenched impurities on prewetting and wetting transitions in adsorbed layers. We concentrate on simple model systems with only two types of adsorption sites and investigate how the concentration...
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| Published in | Surface science Vol. 318; no. 3; pp. 413 - 420 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Lausanne
Elsevier B.V
20.10.1994
Amsterdam Elsevier Science New York, NY |
| Subjects | |
| Online Access | Get full text |
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| Abstract | This paper presents the results of a Monte Carlo simulation study of the effects of randomly distributed quenched impurities on prewetting and wetting transitions in adsorbed layers. We concentrate on simple model systems with only two types of adsorption sites and investigate how the concentration of impurities affects wettability of a surface. It is demonstrated that the impurities may change the character of the prewetting transition and considerably change the wetting temperature. In particular, it is shown that even very weak heterogeneity destroys the first-order character of the prewetting transition and may induce or exclude wetting of a solid substrate. |
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| AbstractList | This paper presents the results of a Monte Carlo simulation study of the effects of randomly distributed quenched impurities on prewetting and wetting transitions in adsorbed layers. We concentrate on simple model systems with only two types of adsorption sites and investigate how the concentration of impurities affects wettability of a surface. It is demonstrated that the impurities may change the character of the prewetting transition and considerably change the wetting temperature. In particular, it is shown that even very weak heterogeneity destroys the first-order character of the prewetting transition and may induce or exclude wetting of a solid substrate. |
| Author | Gac, W. Patrykiejew, A. Sokołowski, S. |
| Author_xml | – sequence: 1 givenname: W. surname: Gac fullname: Gac, W. organization: Department of Chemical Physics, Faculty of Chemistry, MCS University, 20031 Lublin, Poland – sequence: 2 givenname: A. surname: Patrykiejew fullname: Patrykiejew, A. organization: Department of Chemical Physics, Faculty of Chemistry, MCS University, 20031 Lublin, Poland – sequence: 3 givenname: S. surname: Sokołowski fullname: Sokołowski, S. organization: Department of Chemical Physics, Faculty of Chemistry, MCS University, 20031 Lublin, Poland |
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| Cites_doi | 10.1103/PhysRevB.28.2890 10.1103/PhysRevB.48.14454 10.1103/PhysRevB.26.5112 10.1016/0039-6028(90)90090-U 10.1103/PhysRevLett.35.1399 10.1016/0040-6090(93)90725-5 10.1103/PhysRevA.23.1925 10.1016/0378-4371(86)90234-7 10.1103/PhysRevB.32.4683 10.1103/PhysRevB.37.1745 10.1080/01411598808245480 10.1016/0039-6028(83)90456-9 10.1103/PhysRevLett.53.1747 10.1021/la00034a014 10.1088/0305-4470/18/14/012 10.1103/PhysRevB.26.1288 10.1103/PhysRevA.22.2776 10.1063/1.335494 10.1016/0040-6090(92)90641-N 10.1063/1.462180 10.1016/0039-6028(92)90078-K 10.1103/PhysRevLett.56.2272 10.1103/PhysRevB.24.295 |
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| Keywords | Monte Carlo method Fluid solid interface Quantity ratio Adsorption Impurities Wetting Simulation Theoretical study Lattice gas |
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| SubjectTerms | Condensed matter: structure, mechanical and thermal properties Exact sciences and technology Physics Solid-fluid interfaces Surfaces and interfaces; thin films and whiskers (structure and nonelectronic properties) Wetting |
| Title | Effects of random quenched impurities on wetting of solids: a Monte Carlo study |
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